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• Fig. S1. Optical image of a 45-nm-thick exfoliated single-crystal 1T-TaS₂ sample supported on a standard 1000-mesh gold TEM grid.
• Fig. S2. Steady-state and dynamical diffraction patterns of 1T-TaS₂ in the NCCDW state taken at room temperature.
• Fig. S3. The selected CDW patterns under different optical excitation fluences for constructing the optical doping–induced phase diagram obtained at T_B = 150 K using the 800-nm femtosecond photons for optical doping.
• Fig. S4. The determination of CDW phase boundaries based on the presence of a step or a slope change.
• References (50–54)

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