This PDF file includes:

• Fig. S1. Correlation of PdBT to starting materials on ¹H and ¹³C NMR.
• Fig. S2. Measurement of biomolecule incorporation using DMMB and Coomassie blue assays.
• Fig. S3. Modulation of PdBT degradation kinetics by PGA block length.
• Fig. S4. GPC standard curve.
• Table S1. An overview of PdBT compared to several commonly used in situ hydrogel cross-linkers.
• References (38–40)

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