Skip to main content
PLOS One logoLink to PLOS One
. 2023 Mar 22;18(3):e0283199. doi: 10.1371/journal.pone.0283199

Variation and internal-external driving forces of grey water footprint efficiency in China’s Yellow River Basin

Yun Li 1, Yu Liu 1,*, Lihua Yang 1, Tianbo Fu 2
Editor: Xianzhong Cao3
PMCID: PMC10032503  PMID: 36947510

Abstract

Grey water footprint (GWF) efficiency is a reflection of both water pollution and the economy. The assessment of GWF and its efficiency is conducive to improving water environment quality and achieving sustainable development. This study introduces a comprehensive approach to assessing and analyzing the GWF efficiency. Based on the measurement of the GWF efficiency, the kernel density estimation and the Dagum Gini coefficient method are introduced to investigate the spatial and temporal variation of the GWF efficiency. The Geodetector method is also innovatively used to investigate the internal and external driving forces of GWF efficiency, not only revealing the effects of individual factors, but also probing the interaction between different drivers. For demonstrating this assessment approach, nine provinces in China’s Yellow River Basin from 2005 to 2020 are chosen for the study. The results show that: (1) the GWF efficiency of the basin increases from 23.92 yuan/m3 in 2005 to 164.87 yuan/m3 in 2020, showing a distribution pattern of "low in the western and high in the eastern". Agricultural GWF is the main contributor to the GWF. (2) The temporal variation of the GWF efficiency shows a rising trend, and the kernel density curve has noticeable left trailing and polarization characteristics. The spatial variation of the GWF efficiency fluctuates upwards, accompanied by a rise in the overall Gini coefficient from 0.25 to 0.28. Inter-regional variation of the GWF efficiency is the primary source of spatial variation, with an average contribution of 73.39%. (3) For internal driving forces, economic development is the main driver of the GWF efficiency, and the interaction of any two internal factors enhances the explanatory power. For external driving forces, capital stock reflects the greatest impact. The interaction combinations with the highest q statistics for upstream, midstream and downstream are capital stock and population density, technological innovation and population density, and industrial structure and population density, respectively.

Introduction

Water serves as a crucial material basis that sustains the human society. During rapid economic and social development, problems such as the over-consumption of water resources and damage to the water environment have occurred frequently, resulting in the water crisis around the world [1,2]. A quantitative assessment of water pollution is an important prerequisite for alleviating the water crisis [3]. The grey water footprint (GWF) theory, first proposed by Hoekstra and Chapagain [4], provides a new approach to measuring the quality of polluted water. GWF is defined as the volume of freshwater required to absorb a given pollutant [57]. However, sustainable development needs to accommodate both economic and environmental co-benefits [8,9]. The simple concept of the GWF expresses the impact of pollution on the volume of water resources, but does not capture the economic role. As a result, some scholars have further incorporated the role of the economy into the measurement of water pollution by combining the GWF with GDP, which constitutes the GWF efficiency [1013]. A comprehensive analysis of the GWF and its efficiency is an essential basis for reconciling the relationship between the environment and the economy.

As the second longest river in Asia and the " mother river " of China, the Yellow River supplies water to Asia’s major agricultural production areas, such as the Hetao Plain and the Fenwei Plain. Moreover, the Yellow River Basin is an important economic belt for the energy industry [14]. However, over the years, the water quality of the basin has been heavily polluted. With the rise of industry and the accelerated urbanization of the population, wastewater from industry and urban dwellers has increased dramatically [15]. In addition, the over-application of pesticides and fertilizers in the growing areas of the basin is also a severe problem [16]. Consequently, the Yellow River carries about 6% of wastewater and 7% of chemical oxygen demand with 2% of China’s water resources, significantly exceeding the carrying capacity of the water environment [17]. At the same time, problems such as unbalanced economic development also pose a huge challenge to the sustainable development of the Yellow River Basin [18]. Therefore, this study takes the Yellow River Basin as an example to measure the GWF and its efficiency, and to accurately grasp the variation and driving forces of water pollution and economic development in the basin at the spatial and temporal levels, which is representative and relevant.

A series of studies have been conducted on the GWF of the agricultural [7,1921], industrial [22,23] or domestic sectors [24,25]. Many scholars have analyzed the GWF or its efficiency at the national [3,10,26,27], regional [2831] or river basin level [1113,32,33] from the perspective of quantitative measurements. According to the results, it is not difficult to find that the GWF and its efficiency show some numerical variability at the spatial and temporal levels. However, these simple comparisons of visual data often ignore the specific spatial and temporal distribution of subsamples. Few studies have been conducted to quantitatively and methodologically investigate the spatial and temporal variation of the GWF and its efficiency. In this study, the kernel density estimation and the Dagum Gini coefficient method are used to systematically and comprehensively investigate the spatial and temporal variation of the GWF efficiency in the Yellow River Basin. In terms of temporal variation, the kernel density estimation method is able to reflect the continuous distribution characteristics of the data by obtaining estimates of each point of the density function [34,35]. In terms of spatial variation, existing researches tend to use the traditional Gini coefficient method or the Thiel index method to analyze the evolution of the GWF, which cannot solve the overlap problem between sub-samples [36,37]. In contrast, the Dagum Gini coefficient method can effectively overcome this problem and decompose the spatial differences, thus accurately reflecting the spatial variation and its sources [18].

In addition, exploring the driving forces of spatial and temporal changes in the GWF efficiency is a priority for reconciling economic and social development with ecological conservation. Currently, there is a wealth of research related to the driving force of GWF or its efficiency. For example, Zhang and Sun [38], Han et al. [10], Zhang et al. [3], and Feng et al. [27] all use the Kaya equation and LMDI model to dissect the effects of multiple factors on the GWF or its efficiency of different provinces in China. On this basis, Fu et al. [12], Chen et al. [11], and Xu et al. [13] decompose the GWF efficiency into several driving factors by the same method with different watersheds as the object of their study. Bai and Sun combine the Thiel index and the extended Kaya equation to explore the regional differences and driving factors of the GWF per capita [37]. However, the Kaya equation and the LMDI decomposition method used in most studies can quantify the contribution of driving factors to the GWF efficiency, but cannot investigate the interaction of different driving factors. In contrast, the Geodetector method is able to identify the driving factors and their interaction relationships behind the spatial and temporal variation [18,39]. Therefore, this method is selected in this study to analyze the internal-external driving forces of spatial and temporal variation in the GWF efficiency in the Yellow River Basin.

This study aims to introduce an integrated assessment approach for the GWF efficiency. Based on the measurement of the GWF and its efficiency in the 9 provinces of the Yellow River Basin from 2005 to 2020, the temporal and spatial variation of GWF efficiency is investigated by the kernel density estimation and the Dagum Gini coefficient method, respectively. The internal and external driving forces and their interaction of the GWF efficiency are also discussed with the help of the Geodetector. Finally, targeted suggestions are put forward for improving the GWF efficiency. The contributions of this study are: on the one hand, a comprehensive assessment of GWF efficiency is provided at the watershed scale. It also takes into account both temporal and spatial dimensions to reveal the variation in the evolution of GWF efficiency, which can be used to clearly observe the pollution and economic development of the Yellow River Basin. This not only expands the research thinking on GWF efficiency but also contributes to the integrated management of the river basin. On the other hand, the Geodetector method has been innovatively applied to investigate the individual and interactive driving forces of the internal and external factors on GWF efficiency, with a view to finding the main driving factors for the variation of GWF efficiency in different regions. It is useful for the zoning control of water pollution, optimal regulation of water resources and sustainable ecological development.

Overview of the study area

The Yellow River Basin in China spans nine provinces, connecting the Qinghai-Tibet Plateau, the Loess Plateau and the North China Plain, making it an important ecological and economic zone. With only 27% of China’s average per capita water resources, the Yellow River Basin is responsible for supplying water to 12% of the country’s population, 17% of its arable land and more than 50 large and medium-sized cities. In addition, the Yellow River Basin is an important industrial production area in China, with abundant traditional resources such as coal, oil, natural gas and non-ferrous metals. However, the rough development has led to excessive consumption of resources and severe water pollution problems in the river basin. In 2022, the report of the 20th National Congress of the Communist Party of China (CPC) put forward "promoting the ecological protection and high-quality development of the Yellow River basin" as a major strategy to facilitate coordinated regional development. Although the Yellow River has been managed to a certain extent, the problem of fragile water ecology in the basin is still prominent. Coordinating the relationship between water pollution and economic development is a must for the implementation of high-quality development in the Yellow River Basin.

Therefore, nine provinces in China’s Yellow River Basin, including Qinghai, Sichuan, Gansu, Ningxia, Inner Mongolia, Shanxi, Shaanxi, Henan and Shandong, are taken as the research objects. The GWF and its efficiency are measured for the nine provinces between 2005 and 2020. Fig 1 shows an overview of the study area.

Fig 1. Overview of the study area.

Fig 1

Methods and data

GWF efficiency accounting

This study measures the GWF efficiency of the Yellow River Basin in China following the evaluation methodology presented in the Water Footprint Assessment Manual by Hoekstra et al. [40]. The accounting is based on three aspects: agricultural, industrial and domestic GWF.

Agricultural GWF

The GWF from planting and breeding are measured separately to obtain the agricultural GWF. The improper use of pesticides and fertilizers in the planting process has caused serious pollution of water. In this study, the degree of water pollution by nitrogen fertilizers is chosen as the evaluation indicator for the GWF from planting. The specific formula is as follows.

GWFpla=α*ApplCmaxCnat (1)

Where GWFpla is the GWF from planting; α represents the proportion of nitrogen fertilizer entering the water; Appl is the annual use of nitrogen fertilizer; Cmax and Cnat indicate the concentration of the pollutant required in the standard and the background concentration of the pollutant, respectively.

The pollutants chemical oxygen demand (COD) and total nitrogen (TN) are both used as the basis for the evaluation of the GWF from breeding, calculated as follows.

GWFbre=max(GWFbre(COD),GWFbre(TN)) (2)
GWFbre(i)=Lbre(i)CmaxCnat (3)
Lbre(i)=h=14Nh*Dh*(fh*phf*βhf+uh*phu*βhu) (4)

Where GWFbre is the GWF from breeding; i is the pollutant COD or TN; GWFbre(i) represents the GWF from the breeding of different pollutants; Lbre(i) represents the pollutant load of breeding pollutants; h is different livestock (pigs, cattle, sheep, poultry); Nh and Dh are the number and the breeding cycle of h; fh and uh are the daily manure discharge and the daily urine discharge of h; phf and phu are the pollutant content per unit of manure and urine for h; βhf and βhu represent the pollutant loss rate per unit of manure and urine for h, respectively.

According to the metric model for the GWF from planting and breeding, the agricultural GWF (GWFagr) can be calculated by the following equation:

GWFagr=max(GWFbre(COD),GWFpla+GWFbre(TN)) (5)

Industrial GWF

Chemical oxygen demand (COD) and ammonia nitrogen (NH4+N) are the main pollutants in the industrial effluent, which are selected as indicators to measure the industrial GWF. Then

GWFind=max(GWFind(COD),GWFind(NH4+N)) (6)
GWFind(i)=Lind(i)CmaxCnat (7)

Where GWFind(i) represents the industrial GWF of the pollutant i (COD or NH4+N). Lind(i) is the discharge load of the pollutant i.

Domestic GWF

Domestic wastewater is similar to industrial wastewater in that COD and NH4+N are the main pollutants, so the domestic GWF (GWFdom(i)) is calculated in the same way as for industry.

GWF efficiency

The total GWF (TGWF) can be obtained by summing the agricultural, industrial and domestic GWF.

TGWF=GWFagr+GWFind+GWFdom (8)

On this basis, the GWF efficiency (g), i.e., the GDP that can be generated from one unit of GWF, can be further calculated as:

g=GDPTGWF (9)

Kernel density estimation

In this study, kernel density estimation is used to explore the dynamic evolution of GWF efficiency in the temporal dimension. As one of the non-parametric estimation methods, the core idea of kernel density estimation is to characterize the distribution pattern of random variables through a continuous density profile [34,35]. The density function equation is as follows.

f(x)=1Nhi=1NK(XiX¯h) (10)

Where N is the number of sample observations; Xi is the independent and identically distributed observations, i.e., the GWF efficiency of the 9 provinces in the Yellow River Basin; X¯ is the mean of the GWF efficiency; h represents the bandwidth, reflecting the degree of smoothness and estimation accuracy of the density function curve; K represents the kernel density and the kernel function K(•) is expressed as follows.

K(x)=12πexp(x22) (11)
{limxK(x)*x=0K(x)0,+K(x)dx=1supK(x)<+,+K2(x)dx=1 (12)

Dagum Gini coefficient and its decomposition

The Dagum Gini coefficient reflects the changes in the relative variation of indicators. It is used in this study to measure the regional variation of the GWF efficiency in the Yellow River Basin. Drawing on Dagum and Alvaredo [41,42], the 9 provinces are divided into three sub-regions: upstream, midstream and downstream. Among them, upstream includes Qinghai, Sichuan, Gansu and Ningxia; midstream includes Inner Mongolia, Shanxi and Shaanxi; and downstream includes Henan and Shandong. j and h denote different sub-regions; nj and nh represent the number of provinces in sub-regions j and h; yji and yhr represent the GWF efficiency of the province i in region j, and the GWF efficiency of province r in region h, respectively; y¯ is the mean of GWF efficiency. Then, the overall Gini coefficient can be expressed as:

G=j=1kh=1ki=1njr=1nh|yjiyhr|2n2y¯ (13)

On this basis, the Dagum Gini coefficient is decomposed to investigate the sources of variation in the GWF efficiency of different sub-regions. According to the sub-sample decomposition method, the sources of overall variation can be decomposed into three components: the contribution of intra-regional variation (Gw), inter-regional variation (Gnb), and hypervariable density (Gt). G = Gw+Gnb+Gt. Gjj and Gjh represent the Gini coefficient within the sub-region j, and the Gini coefficient between sub-region j and h, respectively. The specific formulas are as follows.

Gjj=i=1njr=1nh|yjiyjr|2nj2yj¯ (14)
Gjh=i=1njr=1nh|yjiyhr|njnh(yj¯+yh¯) (15)
Gw=j=1kGjjpjsj (16)
Gnb=j=2kh=1j1Gjh(phsj+pjsh)Djh (17)
Gt=j=2kh=1j1Gjh(phsj+pjsh)(1Djh) (18)

Where pj = nj/n, sj=njyj¯/ny¯, j = 1,2,⋯,k; Djh represents the relative effect of GWF efficiency between sub-region j and h; djh represents the difference in GWF efficiency between regions and qjh is the hypervariable first order moment. Then

djh=0dFj(y)0y(yx)dFh(x) (19)
qjh=0dFh(y)0y(yx)dFj(x) (20)

Where Fj and Fh represent the cumulative density distribution functions for the region j and h.

Decomposition of driving factors

Geodetectors include factor detection, interaction detection, risk detection and ecological detection [43]. In this study, factor detection and interaction detection are used to explore the internal-external driving forces of the single factor alone and the interaction between different factors on the variation of GWF efficiency, respectively.

Factor detection. q values reflect the effect on grey water footprint efficiency, q∈[0,1]. q values indicate that Xi explains 100*q% of Y, i.e., the higher the q value, the greater the explanatory power of variable Xi on the variation in GWF efficiency. q is expressed as:

q=11Nσ2h=1mNh*σh2 (21)

Where h = 1,2,⋯,m, is the strata of the independent or dependent variable. N and Nh are the sample sizes for the whole basin and strata, respectively. σ2 and σh2 represent the variance of the dependent variable for the whole basin and strata, respectively.

Interaction detection. Interactions between different factors are identified by assessing whether factors Xi and Xj acting together increase or decrease the explanatory power (q value) of the dependent variable Y. Specifically, if q(XiXj)<min(q(Xi),q(Xj)), the interaction of Xi and Xj is non-linearly weakened; if min(q(Xi),q(Xj))<q(XiXj)<max(q(Xi),q(Xj)), the interaction of Xi and Xj is one-way non-linearly weakened; if max(q(Xi),q(Xj))<q(XiXj)<q(Xi)+q(Xj), the interaction of Xi and Xj is two-way strengthened; if q(XiXj)=q(Xi)+q(Xj), it means that Xi and Xj are independent of each other; if q(XiXj)>q(Xi)+q(Xj), the interaction of Xi and Xj is non-linearly strengthened.

Data sources

Variables of GWF efficiency

This study measures the GWF efficiency of different sectors based on the statistical data from 2005–2020 in the 9 provinces of the Yellow River Basin. Among them, data on the annual use of nitrogen fertilizer in the agricultural sector are obtained from the Agricultural Statistics of New China in the Past Fifty Years, and the proportion of nitrogen fertilizer entering water bodies is 7%; data on the number of livestock, breeding cycle, daily manure and urine discharge, pollutant content per unit of manure and urine, and pollutant loss rate per unit of manure and urine are obtained from the China Rural Statistical Yearbook and the China Pollution Technical Report of the Survey of Large-scale Livestock and Poultry Breeding Industry; data of industrial and domestic pollutant discharges and GDP can be obtained from the China Environmental Statistical Yearbook and China Statistical Yearbook. In addition, with reference to Hoekstra et al. [40], Han et al. [10], Zhang et al. [3] and the Integrated Pollutant Discharge Standard (GB8978-1996), the background concentration of the pollutant is set at 0, and the concentrations of COD and nitrogen required in the standard are 60 mg/L and 15 mg/L, respectively.

Variables of the driving forces

This study investigates the key driving forces of the spatial and temporal variation of GWF efficiency in the Yellow River Basin from both internal and external perspectives. On the one hand, the underlying cause of the variation in GWF efficiency is the correlation and mutual feedback between the internal forces that constitute the GWF efficiency. The economic development factor, represented by GDP, is one of the significant drivers of GWF efficiency. As the measurement of GWF efficiency is dependent on water use and pollution emissions, the factors of water consumption and pollution levels should also be included as internal driving forces. In addition, labour and environmental capital inputs can influence grey water output in different industries which are also critical internal drivers that cannot be ignored. Therefore, in this study, economic development (ED), water consumption (WC), pollution level (PL), labour input (LI) and environmental capital input (EI) are selected as internal driving forces affecting GWF efficiency. The economic development is measured by the GDP of each province; the water consumption is represented by the ratio of water consumption to total water resources; the pollution level is based on the ratio of total COD and ammonia nitrogen emissions to water consumption in different sectors; the labour input is measured by the employment rate of the urban population; and the environmental capital investment is measured by the amount of investment in pollution control as a proportion of GDP.

On the other hand, according to existing studies, external factors such as industrial structure (IS), population density (PD), technological innovation (TI), urban-rural structure (UR), and capital stock (CS) can also influence the spatial and temporal variation of GWF efficiency [3,12,30,38]. In this study, the industrial structure is represented by the share of tertiary industry in GDP; population density is tabulated as the ratio of total population to administrative district land area; technological innovation is represented by the number of patents granted; urban-rural structure is represented by the share of urban population in total population; the level of capital stock is represented by the fixed capital stock. The data on the above driving forces are obtained from the China Statistical Yearbook.

Results

Measurement of GWF efficiency

The GWF of different sectors and the corresponding GWF efficiency in the Yellow River Basin can be calculated, as shown in Fig 2. As a whole, the GWF efficiency of the Yellow River Basin increases from 23.92 yuan/m3 in 2005 to 164.87 yuan/m3 in 2020. It is mainly due to the reduction of the GWF and the rapid growth of GDP. On the one hand, GDP rises from 570.26 billion yuan in 2005 to 2820.69 billion yuan in 2020. It indicates that the economy of the Yellow River Basin has achieved substantial development in recent years. On the other hand, the total GWF shows a fluctuating downward trend with a decline from 20.75 billion m3 to 15.74 billion m3 during the observation period. The year 2007 is a significant turning point, and since then, the GWF has switched from rising to gradually declining, with a rebound in 2020. This result is consistent with the studies by Zhang and Sun [38], and Lin et al. [44]. It is mainly associated with the implementation of "basin restrictions" since 2007, i.e., limiting the number of polluting enterprises and strengthening water quality supervision [45]. With the strengthening of environmental regulation and the upgrading of industrial standards, sewage discharge has been controlled. This result also indirectly reflects the effectiveness of China’s environmental regulation policy. In addition, both the GWF and its efficiency change abruptly in 2020. Compared to 2019, the domestic GWF is significantly higher in 2020, leading to an increase in the total GWF. However, due to macro factors such as the New Crown epidemic, the growth in GDP of 2020 is slight, which results in a significant decrease in the GWF efficiency. It indicates that urban wastewater treatment in the basin needs to be strengthened. In response, in 2021, China’s Development and Reform Commission and Ministry of Housing and Construction jointly issue the Implementation Plan for the Urban Sewage and Waste Treatment in the Yellow River Basin during the "14th Five-Year Plan" period to improve the domestic sewage treatment rate.

Fig 2. Changes in the GWF and its efficiency in the Yellow River Basin from 2005 to 2020.

Fig 2

To observe the changes in GWF efficiency of different provinces, Fig 3 reports the GWF efficiency and the proportion of the GWF of different sectors at four-time points: 2005, 2010, 2015 and 2020. As can be seen, the GWF efficiency varies considerably between provinces, showing a spatial distribution pattern of "low in the western and high in the eastern". The GWF efficiency of Shandong province in the downstream remains the highest, while Qinghai province in the upstream is the lowest. Qinghai is the source of the Yellow River and has a relatively good water environment, with a low GWF of 6.82 billion m3, which is around 2/5 of the average GWF of the basin as a whole. However, as an economically underdeveloped region, Qinghai is still in the early stages of industrial development, and this situation has not been effectively improved over the years. The average GDP of Qinghai is only 186.14 billion yuan, much lower than the overall basin average GDP of 1733.16 billion yuan, which causes the GWF efficiency to be small. This result is also reflected in the study by Han et al. [10]. Differently, the other upstream provinces (Sichuan, Gansu and Ningxia) have received a faster increase in GWF efficiency, due to a slight decrease in grey water emissions and a rapid rise in GDP. In comparison, Shandong province in the downstream has secured an increase in GWF efficiency from 46.82 yuan/m3 to 294.63 yuan/m3 in parallel with stable socio-economic development. The reason is that Shandong, as an estuary province of the Yellow River, has a comparative advantage and is better developed in terms of economy, industry and technology [3]. Especially, core cities in Shandong, such as Jinan, have made efforts to promote high-quality development, with the growth rate of major economic indicators remaining in the top echelon of the province and strategic emerging industries showing strong and resilient development trends.

Fig 3. GWF efficiency and the decomposition of GWF by province.

Fig 3

In addition, the downstream province of Henan also experiences significant growth in GWF efficiency during the observation period, with an 8.24-fold increase. As a central agricultural province in the Yellow River Basin, Henan has accelerated its agricultural emission reduction efforts in recent years, and has been effective in controlling greywater emissions, decreasing from 45.01 billion m3 to 28.38 billion m3. Similarly, the GWF efficiency of Shanxi and Shaanxi in the midstream has risen rapidly, with increases of 230.85 yuan/m3 and 206.64 yuan/m3, respectively. However, Inner Mongolia, another midstream province, has seen relatively little improvement in the GWF efficiency. Despite its economic growth over the years, there has been no significant reduction in grey water emissions. Inner Mongolia has a sizeable east-west span, with a highly uneven distribution of resources and economic development. The western economic zone of Inner Mongolia, centered on Hohhot, Ordos and Baotou, is the main source of the province’s economy, while the other regions have experienced very slow economic growth. Moreover, the industry based on energy sources such as coal has led to serious water pollution.

To further explore the heterogeneous role of different sectors, this study provides a detailed insight into the changes in agricultural, industrial and domestic GWF. Combining Figs 2 and 3, it is clear that the share of agricultural GWF is consistently the largest. From 2005 to 2020, the agricultural and industrial GWF fluctuate downwards, while the domestic GWF increases significantly. It indicates that agricultural grey water is the main source of grey water discharge in the Yellow River Basin. And over the years, grey water discharges from agriculture and industry have been controlled to some extent. In contrast to the actual situation, agricultural production in the Yellow River Basin is large in scale, with a wide distribution of rural areas, a concentrated population and a great number of livestock and poultry, which lead to severe non-point source pollution and a significant contribution to water pollutants [46,47]. It has caused the characteristic that agricultural GWF accounts for the largest share.

Spatial and temporal variation of GWF efficiency

Temporal variation

After the above analysis, it can be initially recognized that there is a certain variation in grey water footprint efficiency in the Yellow River Basin at the spatial and temporal dimensions. This study considers 2005, 2008, 2011, 2014, 2017 and 2020 as typical years and further explores the dynamics of temporal variation in GWF efficiency through the kernel density estimation method, as shown in Fig 4.

Fig 4. Kernel density estimation of GWF efficiency.

Fig 4

In terms of distribution position, the kernel density curve for GWF efficiency shifts to the right as a whole, showing a left-skewed distribution. It indicates that the GWF efficiency of the basin tends to be in an upward trend. In terms of the distribution pattern, the height of the main peak of the GWF efficiency curve decreases in a fluctuating manner, and the width becomes wider from 2005 to 2020. It means that the absolute difference in GWF efficiency is increasing and indirectly reflects the imbalanced development of the Yellow River Basin. For a long time, the Yellow River Basin has been characterized by a development pattern of "strong in the downstream and weak in the upstream". These findings reaffirm the significance of coordinated development in the Yellow River Basin. In terms of distribution extension, the curve of GWF efficiency has a clear left trailing feature. It demonstrates the existence of provinces with very poor GWF efficiency that should be controlled locally. In terms of polarization trends, the kernel density curve of GWF efficiency shows a multi-peaked pattern, with the main peak significantly higher than the side peaks. Although the pattern of the side peaks has gradually smoothed out in recent years, the overall trend has not changed. It suggests that the GWF efficiency in the Yellow River Basin is multi-polar. The variation between high and low provinces has decreased over the years, but the gradient effect is still significant. Therefore, it is necessary to implement differentiated water management in response to regional realities.

Spatial variation

To characterize the spatial variation of GWF efficiency in the Yellow River Basin, regional differences and sources of GWF efficiency are analyzed using the Dagum Gini coefficient and its decomposition method, and the results are presented in Table 1.

Table 1. Dagum Gini coefficient and decomposition.
year Basin-wide Gini
Coefficient
Intra-regional variation Inter-regional variation Contribution rate (%)
Upstream Midstream Downstream Up-Mid Up-Down Mid-Down Intra-regional Inter-regional Hypervariable density
2005 0.25 0.17 0.10 0.15 0.18 0.41 0.32 17.17 76.38 6.46
2006 0.26 0.18 0.08 0.15 0.20 0.42 0.32 16.60 76.72 6.68
2007 0.27 0.17 0.10 0.17 0.20 0.45 0.35 16.73 77.45 5.82
2008 0.28 0.18 0.11 0.16 0.21 0.47 0.37 16.27 77.50 6.23
2009 0.28 0.19 0.08 0.14 0.21 0.46 0.38 14.83 76.98 8.19
2010 0.28 0.19 0.09 0.15 0.20 0.44 0.38 15.63 74.79 9.58
2011 0.28 0.19 0.10 0.15 0.19 0.44 0.41 15.88 73.26 10.87
2012 0.27 0.18 0.09 0.15 0.19 0.43 0.40 15.85 73.07 11.09
2013 0.27 0.19 0.09 0.16 0.19 0.43 0.39 16.00 73.34 10.66
2014 0.28 0.19 0.09 0.16 0.21 0.44 0.38 16.00 74.35 9.65
2015 0.28 0.19 0.11 0.17 0.20 0.44 0.37 17.15 73.64 9.21
2016 0.28 0.19 0.14 0.18 0.20 0.42 0.39 18.92 69.27 11.81
2017 0.30 0.14 0.20 0.22 0.20 0.43 0.41 20.63 67.63 11.73
2018 0.30 0.13 0.19 0.21 0.19 0.43 0.42 20.31 68.28 11.41
2019 0.30 0.09 0.19 0.24 0.17 0.44 0.42 20.39 68.91 10.69
2020 0.28 0.10 0.16 0.23 0.17 0.44 0.38 19.81 72.66 7.53

According to the results, the overall Gini coefficient of GWF efficiency in the Yellow River Basin shows a fluctuating upward trend during the observation period, rising from 0.25 in 2005 to 0.28 in 2020, with an increase of 12.83%. It indicates that the regional variation in GWF efficiency has become greater. Specifically, the average contribution of intra-regional variation, inter-regional variation and hypervariable density is 17.39%, 73.39% and 9.23%, respectively, with significant stratification. It can be seen that inter-regional variation is the main source of spatial variation in GWF efficiency in the Yellow River Basin. This result emphasizes the objective fact that the development of the Yellow River Basin is imbalanced once again. From the perspective of the contribution of variation, the contribution of inter-regional variation decreases from 76.38% to 72.66%. On the contrary, the contribution of intra-regional variation and hypervariable density rises, with an increase of 15.39% and 16.63%, respectively. It indicates a slight decrease in the inter-regional variation of GWF efficiency. However, it is still at a high level, far exceeding the sum of the other contributions.

This study further analyzes intra-regional and inter-regional variation separately. The intra-regional variation in both the upstream and midstream during the observation period is slight, with corresponding average Gini coefficients of 16.70%, 12.08% and 17.37%, respectively. Between 2005 and 2015, the intra-regional variation is consistently greatest in the upstream and smallest in the midstream. After 2015, the intra-regional Gini coefficient in the downstream rises significantly, leapfrogging the upstream. It indicates that the variation between Shandong Province and Henan Province in the downstream has been expanding in recent years. Inter-regional variation exhibits different characteristics. The average value of the inter-regional Gini coefficient for GWF efficiency in the Yellow River Basin is high and fluctuates very slightly. The inter-regional variation between the upstream and downstream is consistently the largest, while the variation between the upstream and midstream is the smallest. It is due to the large environmental and economic differences between the upper and lower reaches of the Yellow River Basin. Therefore, the integrated management of the Yellow River Basin should pay more attention to differentiation and develop relevant policies for different regions.

Analysis of driving forces

Internal driving forces

In this study, q statistics and significance levels for each driving factor are calculated with the help of a factor detector (as seen in Table 2). The driving force of the internal factors of the GWF efficiency in the Yellow River Basin is then investigated. Fig 5 shows the driving force of the different internal factors at the spatial and temporal dimensions. It is seen in Fig 5(A) that economic development is the dominant factor in the evolution of GWF efficiency in the Yellow River Basin as a whole and the three major regions. It is mainly due to the fact that areas with poor economic development have smaller GDPs and are often accompanied by problems such as sloppy production practices and high pollutant emissions, which inhibit GWF efficiency [10]. In addition, the pollution level is also a driving factor for the spatial and temporal variation of GWF efficiency that cannot be ignored. Specifically by region, for the basin as a whole and the upstream region, water consumption, labour input and environmental capital input contribute to improving GWF efficiency while the driving force is relatively small. In the midstream, labour input also has a significant role in the change of GWF efficiency except for economic development and pollution level. For the downstream, attention should also be paid to the water consumption factor. The downstream of the Yellow River suffers from severe water scarcity. Over the years, poor irrigation practices, rapid population growth and artificial diversions have led to reduced water availability and degradation of the water environment in the lower reaches, especially at the mouth of the delta [48,49]. Thus, improving the GWF efficiency in the downstream also requires rational water consumption management. According to the temporal evolution of the driving effects of different internal factors depicted in Fig 5(B), economic development has long been the main driver of the spatial and temporal variation in GWF efficiency, with the corresponding q statistics remaining high despite a significant decline after 2015. Except for the economic development factor, all other factors show relatively significant fluctuating changes.

Table 2. The driving force of internal factors on the GWF efficiency.
Region Driving force ED WC PL LI EI
Basin-wide q statistic 0.59 0.16 0.35 0.18 0.11
p value 0.00 0.00 0.00 0.00 0.01
Upstream q statistic 0.61 0.20 0.47 0.21 0.27
p value 0.00 0.05 0.00 0.04 0.01
Midstream q statistic 0.82 0.11 0.64 0.55 0.30
p value 0.00 0.49 0.00 0.00 0.03
Downstream q statistic 0.94 0.38 0.78 0.09 0.11
p value 0.00 0.10 0.00 0.72 0.69
Fig 5. Spatial and temporal evolution of the driving force of internal factors.

Fig 5

The interaction detector is also used to explore the superimposed effects of the different internal driving factors, with the specific results shown in Fig 6. It can be found that the interaction of any two factors enhances the driving force of individual factors on changes of GWF efficiency, and that all combinations of interactions are either non-linearly strengthened or two-way strengthened. It suggests that the spatial and temporal variation in GWF efficiency receives the combined effect of multiple internal factors. By coordinating the relationship between the different factors, GWF efficiency can be effectively promoted. The interaction between economic development and other factors is always the highest for both the basin as a whole and the three sub-regions, especially in the downstream areas, where the driving force is over 90%. At the same time, the q statistics for the interaction between pollution level and other factors are all above 0.35. For the basin as a whole, the interaction between economic development and pollution level is the most significant, further suggesting that these two factors are critical to the GWF efficiency. Regarding the sub-region, the interaction between economic development and weakly driven labour input in the upstream has a significantly higher q statistic than the other combinations. It indicates that the improvement of GWF efficiency in the upstream should not only consider economic aspects, but also increase labour input and promote employment. For the midstream and downstream, when the water consumption factor with a weak driving force is combined with other factors, especially pollution level, the impact on GWF efficiency will be very significant. Therefore, controlling pollution emissions while using water resources wisely is also an effective initiative to promote GWF efficiency in the middle and lower reaches.

Fig 6. Detection results of the interaction of internal factors.

Fig 6

External driving forces

To explore the driving forces of the spatial and temporal variation in GWF efficiency, it is necessary to consider not only the direct effect of internal factors, but also the indirect driving force of external factors. As a result, this study further calculates the q statistics of the external factors and judges the interaction of different external factors. All the external driving forces reported in Table 3 have passed the 10% significance level test, confirming the high explanatory power of each external factor on the variation of GWF efficiency.

Table 3. The driving force of external factors on the GWF efficiency.
Region Driving force IS PD TI UR CS
Basin-wide q statistic 0.07 0.34 0.63 0.54 0.70
p value 0.08 0.00 0.00 0.00 0.00
Upstream q statistic 0.26 0.44 0.62 0.39 0.66
p value 0.02 0.00 0.00 0.00 0.00
Midstream q statistic 0.31 0.50 0.79 0.53 0.82
p value 0.03 0.00 0.00 0.00 0.00
Downstream q statistic 0.92 0.74 0.93 0.91 0.82
p value 0.00 0.00 0.00 0.00 0.00

Similarly, Fig 7 illustrates the spatial and temporal evolution of the driving forces of external factors. It can be seen that capital stock is the main external driver of the variation in GWF efficiency, and its contribution remains at the highest position throughout the period 2005–2020. For all regions of the Yellow River Basin, it is important to use the power of capital to promote GWF efficiency. The driving force of technological innovation is also vital. The effect of technological innovation is not only reflected in the ability to improve the treatment rate of domestic and industrial wastewater, but also to improve fertilizer uptake and reduce fertilizer application, thereby mitigating agricultural pollution [27]. Furthermore, based on the temporal evolutionary characteristics of the driving forces of external factors, it is also clear that the driving force of population density on GWF efficiency increases rapidly after 2011. This is because areas with higher population accommodation capacity can effectively avoid the problem of excessive resource use or pollution emissions in zones of a certain size, reducing the environmental load on water bodies [50]. For the basin as a whole, the driving forces of the industrial structure and urban-rural structure are relatively weak; while in the downstream, the effect of these two factors is significant.

Fig 7. Spatial and temporal evolution of the driving force of external factors.

Fig 7

Similar to the internal factors, the interaction of any two external factors is significantly greater than the effect of individual factors (as shown in Fig 8). For the downstream region, the mean value of the q-statistic is as high as 0.93, indicating that the synergistic effect of external driving factors significantly enhances the explanation of the spatial and temporal variation in GWF efficiency in the Yellow River Basin. In terms of specific factors, the interaction of capital stock and technological innovation with other drivers is significant for the basin as a whole and for the three sub-regions. The dominant role of these two factors is again affirmed. In terms of sub-regions, the strongest combinations of q statistics corresponding to the upstream, midstream and downstream are capital stock and population density, technological innovation and population density, and industrial structure and population density, respectively. Therefore, each region should take locally appropriate measures to improve the GWF efficiency.

Fig 8. Detection results of the interaction of external factors.

Fig 8

Discussion

Comparison with previous researches

This study measures the GWF and its efficiency for 9 provinces in the Yellow River Basin. The results have some commonalities with previous research which indicates the reasonableness of this study. For example, the GWF in this study decreases from 20.75 billion m3 in 2005 to 15.74 billion m3 in 2020. The year 2007 is a significant split point, and since then, the GWF has gradually changed from increasing to decreasing. Such results are consistent with the studies by Zhang and Sun [38], and Lin et al. [44]. They measure the GWF of 31 Chinese provinces and cities from 2000–2014 and 1998–2016, respectively, and similarly find that the GWF shifts from an increasing to a decreasing trend from the year 2007 onwards. This change mainly stems from the implementation of environmental regulation policies at that time. In addition, Han et al. [10], Fu et al. [12], and Xu et al. [13] show that the GWF efficiency in China or the Yangtze River Basin is generally low in the west and high in the east, indirectly confirming the reliability of the results in this study.

However, the differences between the results of this study and other existing studies cannot be ignored. Specifically, Zhang et al. find that the domestic GWF makes the most considerable contribution to the total GWF, averaging about 69% [3], while this study concludes that agricultural GWF is the primary source of GWF in the Yellow River Basin. The reason for this discrepancy is that, on the one hand, the difference in study samples and intervals leads to some bias in the specific values measured. On the other hand, the Yellow River Basin is an important agricultural production area with a wide rural distribution, population concentration and a large number of livestock and poultry. It has led to serious non-point source pollution and water pollution [46,47].

Using the Geodetector method, this study also explores the internal and external driving forces of the spatial and temporal variation in GWF efficiency. It is found that economic development is the main internal driver of the variation in GWF efficiency. Han et al. [10], Zhang et al. [3], Fu et al. [12], Feng et al. [27], and Xu et al. [13] decompose the GWF or its efficiency using the Kaya equation and the LMDI model, and similarly find that the economic effect is an essential driving factor. In terms of external driving factors, capital stock and technological innovation are the primary drivers of GWF efficiency. Similar conclusions can be obtained in the studies by Zhang and Sun [38], Fu et al. [12], and Feng et al. [27]. Distinguishing from the existing literature, this study further investigates the interaction of different internal or external factors on the variation of GWF efficiency. It can be found that the interaction of any two internal or external factors is more significant than the effect of a single factor. Furthermore, the combinations of interactions with the highest q statistics vary for different regions. Therefore, it is necessary to take differentiated measures to improve grey water footprint efficiency for different regions.

Policy implications

Based on the above analysis, this study suggests that synergistically improving the GWF efficiency of the Yellow River Basin requires not only a basin-wide perspective, but also disaggregated measures according to regional advantages.

Firstly, a region-wide coordinated development mechanism should be established to gradually reduce the absolute variation of GWF efficiency in the basin. Regions with high GWF efficiency should play a leading role, while low-efficiency regions should seek a new balance between environmental protection and economic development that is adapted to their demands. Secondly, the temporal and spatial differences in economic development and water pollution status among the three major regions of the basin should be fully considered, and initiatives should be differentiated to improve the GWF efficiency. For the upstream region, on the one hand, water environment regulation should be strengthened to enhance water containment capacity; on the other hand, for the main grain-producing areas such as the Hetao Plain and the Fenwei Plain, modern agriculture should be developed through technological innovation. Measures in the midstream region should be centered on pollution control and soil and water conservation. For example, controlling industrial pollution emissions, building silt dams and developing dry terracing. In the downstream, the focus can be on the protection of the delta area. Thirdly, the role of different internal and external driving forces should be brought into play. On the one hand, pay attention to the interaction between economic development and other factors. At the same time, it is necessary to accelerate the cultivation of strategic new industries and promote the rational allocation of water resources and the upgrading of energy structures. On the other hand, the focus should be on safeguarding capital stock and resolving the conflict between people and land.

Conclusion

This study introduces a comprehensive methodology for assessing and analyzing the GWF efficiency. Firstly, the GWF and its efficiency are calculated for the nine provinces of the Yellow River Basin from 2005 to 2020 from the agricultural, industrial and domestic perspectives. On this basis, the spatial and temporal variation in GWF efficiency is comprehensively investigated by the kernel density estimation and the Dagum Gini coefficient method, and the internal and external driving factors of the GWF efficiency are identified by the Geodetector method. The findings of the study are as follows.

  1. Between 2005 and 2020, the GWF of the Yellow River Basin decreases from 20.75 billion m3 to 15.74 billion m3, and the agricultural GWF is the main contributor to GWF. In addition, the GWF efficiency increases from 23.92 yuan/m3 to 164.87 yuan/m3, showing a distribution pattern of "low in the western and high in the eastern". The GWF efficiency of Shandong province in the downstream remains at the highest level, while Qinghai province in the upstream is at the lowest.

  2. The absolute temporal variation of GWF efficiency shows a rising trend. The kernel density curve is characterized by a significant left trailing and polarization, indicating the existence of areas with very low GWF efficiency and significant multi-polar differentiation in the Yellow River Basin. The spatial variation of GWF efficiency fluctuates upwards, accompanied by an increase in the overall Dagum Gini coefficient from 0.25 to 0.28. Inter-regional variation is the main source of spatial variation in GWF efficiency, with an average contribution of 73.39%. By sub-region, intra-regional variation is consistently higher in the upstream than in the midstream and downstream; the most serious spatial variation in GWF efficiency is found between the upstream and downstream.

  3. In terms of internal driving forces, economic development is the primary driver of spatial and temporal variation in GWF efficiency in both the Yellow River Basin as a whole and the three regions. The interaction of any two internal factors is more significant than the effect of individual factors; in terms of external driving forces, the capital stock has the greatest impact on GWF efficiency. The corresponding interaction combinations with the highest q statistics for upstream, midstream and downstream are capital stock and population density, technological innovation and population density, and industrial structure and population density, respectively.

Supporting information

S1 File

(TXT)

S1 Data

(XLSX)

Acknowledgments

We would like to express our sincere thanks to the editors and anonymous reviewers for their constructive comments and suggestions.

Data Availability

All relevant data and the sources have been provided in the paper and the Supporting Information file.

Funding Statement

This study is supported by the “Graduate Research and Innovation Projects of Jiangsu Province” (grant number: KYCX21_0441) and the “Fundamental Research Funds for the Central Universities” (grant number: B220203024). The funder has played an important role in study design, data collection and analysis, decision to publish, and preparation of the manuscript.

References

  • 1.Rijsberman FR. Water scarcity: Fact or fiction?. Agricultural Water Management. 2006; 80(1–3):5–22. doi: 10.1016/j.agwat.2005.07.001 [DOI] [Google Scholar]
  • 2.Jiang Y. China’s water scarcity. Journal of Environmental Management. 2009; 90(11):3185–3196. doi: 10.1016/j.jenvman.2009.04.016 [DOI] [PubMed] [Google Scholar]
  • 3.Zhang L, Dong H, Geng Y, Francisco M. China’s provincial grey water footprint characteristic and driving forces. Science of The Total Environment. 2019; 677:427–435. doi: 10.1016/j.scitotenv.2019.04.318 [DOI] [PubMed] [Google Scholar]
  • 4.Hoekstra AY, Chapagain AK. Globalization of water: Sharing the planet’s freshwater resources. Blackwell Publishing, Oxford, UK. 2008. [Google Scholar]
  • 5.Franke NA, Boyacioglu H, Hoekstra AY. Grey water footprint accounting: Tier 1 supporting guidelines. Unesco-IHE Institute dor Water Education. 2013. [Google Scholar]
  • 6.Girolamo AMD, Miscioscia P, Politi T, Barca E. Improving grey water footprint assessment: Accounting for uncertainty. Ecological Indicators. 2019; 102:822–833. doi: 10.1016/j.ecolind.2019.03.040 [DOI] [Google Scholar]
  • 7.Jamshidi S, Imani S, Delavar M. An approach to quantifying the grey water footprint of agricultural productions in basins with impaired environment. Journal of Hydrology. 2022; 606:127458. doi: 10.1016/j.jhydrol.2022.127458 [DOI] [Google Scholar]
  • 8.Strange T, Bayley A. Sustainable development: Linking economy, society, environment. OECD. 2008. [Google Scholar]
  • 9.Han Z, Jiao S, Zhang X, Xie F, Ran J, Jin R, et al. Seeking sustainable development policies at the municipal level based on the triad of city, economy and environment: Evidence from Hunan province, China. Journal of Environmental Management. 2021; 290:112554. doi: 10.1016/j.jenvman.2021.112554 [DOI] [PubMed] [Google Scholar]
  • 10.Han Q, Sun C, Zou W. Grey water footprint efficiency measure and its driving pattern analysis on provincial scale in China from 1998 to 2012. Resources Science. 2016; 38(6):1179–1191. doi: 10.18402/resci.2016.06.17 [DOI] [Google Scholar]
  • 11.Chen Y, Tong G, Wang L. Spatial-temporal distribution and driving models of agricultural grey water footprint efficiency in the Huai River Basin. Water Resources Protection. 2020; 36(6):60–66+85. doi: 10.3880/j.issn.1004-6933.2020.06.010 [DOI] [Google Scholar]
  • 12.Fu T, Xu C, Yang L, Hou S, Xia Q. Measurement and driving factors of grey water footprint efficiency in Yangtze River Basin. Science of The Total Environment. 2022; 802:149587. doi: 10.1016/j.scitotenv.2021.149587 [DOI] [PubMed] [Google Scholar]
  • 13.Xu C, Liu Y, Fu T. Spatial-temporal evolution and driving factors of grey water footprint efficiency in the Yangtze River Economic Belt. Science of The Total Environment. 2022; 844:156930. doi: 10.1016/j.scitotenv.2022.156930 [DOI] [PubMed] [Google Scholar]
  • 14.Cai X, Rosegrant MW. Optional water development strategies for the Yellow River Basin: Balancing agricultural and ecological water demands. Water Resources Research. 2004; 40(8):1–11. doi: 10.1029/2003wr002488 [DOI] [Google Scholar]
  • 15.Feng K, Siu YL, Guan D, Hubacek K. Assessing regional virtual water flows and water footprints in the Yellow River Basin, China: A consumption based approach. Applied Geography, 2012; 32(2):691–701. doi: 10.1016/j.apgeog.2011.08.004 [DOI] [Google Scholar]
  • 16.Zhuo L, Mekonnen MM, Hoekstra AY, Wada Y. Inter- and intra-annual variation of water footprint of crops and blue water scarcity in the Yellow River basin (1961–2009). Advances in Water Resources. 2016; 87:29–41. doi: 10.1016/j.advwatres.2015.11.002 [DOI] [Google Scholar]
  • 17.Lv Z, Mu J. Study on the spatial and temporal evolution of water quality pollution in the Yellow River Basin. Yellow River. 2017; 39(4):66–70+77. doi: 10.3969/j.issn.1000-1379.2017.04.015 [DOI] [Google Scholar]
  • 18.Chen M, Yue H, Hao Y, Liu W. Spatial variation, dynamic evolution and drivers of eco-efficiency in the Yellow River Basin. Quantitative and technical economic research. 2021; 38(9):25–44. doi: 10.13653/j.cnki.jqte.2021.09.002 [DOI] [Google Scholar]
  • 19.Wu M, Chiu Y, Demissie Y. Quantifying the regional water footprint of biofuel production by incorporating hydrologic modeling. Water Resources Research. 2012; 48(10):W10518. doi: 10.1029/2011WR011809 [DOI] [Google Scholar]
  • 20.Jamshidi S. An approach to develop grey water footprint accounting. Ecological Indicators. 2019; 106:105477. doi: 10.1016/j.ecolind.2019.105477 [DOI] [Google Scholar]
  • 21.Karandish F, Hoekstra AY, Hogeboom RJ. Reducing food waste and changing cropping patterns to reduce water consumption and pollution in cereal production in Iran. Journal of Hydrology. 2020; 586:124881. doi: 10.1016/j.jhydrol.2020.124881 [DOI] [Google Scholar]
  • 22.Wang L, Ding X, Wu X, Yu J. Textiles industrial water footprint: Methodology and study. Journal of Scientific & Industrial Research. 2013; 72(11):710–715. [Google Scholar]
  • 23.Chini CM, Logan LH, Stillwell AS. Grey water footprints of U.S. thermoelectric power plants from 2010–2016. Advances in Water Resources. 2020; 145:103733. doi: 10.1016/j.advwatres.2020.103733 [DOI] [Google Scholar]
  • 24.Mian HR, Hu G, Hewage K, Sadiq R. Drinking water quality assessment in distribution networks: A water footprint approach. Science of The Total Environment. 2021; 775(4):145844. doi: 10.1016/j.scitotenv.2021.145844 [DOI] [Google Scholar]
  • 25.Liao X, Chai L, Liang Y. Income impacts on household consumption’s grey water footprint in China. Science of The Total Environment. 2021; 755:142584. doi: 10.1016/j.scitotenv.2020.142584 [DOI] [PubMed] [Google Scholar]
  • 26.Muratoglu A. Grey water footprint of agricultural production: An assessment based on nitrogen surplus and high-resolution leaching runoff fractions in Turkey. Science of The Total Environment. 2020; 742:140553. doi: 10.1016/j.scitotenv.2020.140553 [DOI] [PubMed] [Google Scholar]
  • 27.Feng H, Sun F, Liu Y, Zeng P, Che Y. Mapping multiple water pollutants across China using the grey water footprint. Science of The Total Environment. 2021; 785:147255. doi: 10.1016/j.scitotenv.2021.147255 [DOI] [PubMed] [Google Scholar]
  • 28.Serio F, Miglietta PP, Lamastra L, Ficocelli S, Intini F, Leo FD, et al. Groundwater nitrate contamination and agricultural land use: A grey water footprint perspective in Southern Apulia Region (Italy). Science of The Total Environment. 2018; 645:1425–1431. doi: 10.1016/j.scitotenv.2018.07.241 [DOI] [PubMed] [Google Scholar]
  • 29.Aldaya MM, Rodriguez CI, Fernandez-Poulussen A, Merchan D, Beriain MJ, Llamas R. Grey water footprint as an indicator for diffuse nitrogen pollution: The case of Navarra, Spain. Science of The Total Environment. 2020; 698:134338. doi: 10.1016/j.scitotenv.2019.134338 [DOI] [PubMed] [Google Scholar]
  • 30.Li S, Wang Y, Luo J, Jiang P, Chen H. Spatio⁃temporal variations and driving factors of grey water footprint in Fujian Province. Acta Ecologica Sinica. 2020; 40(21):7952–7965. doi: 10.5846/stxb201910292274 [DOI] [Google Scholar]
  • 31.Wang X, Dong Z, Wang W, Luo Y, Tan Y. Stochastic grey water footprint model based on uncertainty analysis theory. Ecological Indicators. 2021; 124:107444. doi: 10.1016/j.ecolind.2021.107444 [DOI] [Google Scholar]
  • 32.Pellicer-Martínez F, Martínez-Paz JM. Grey water footprint assessment at the river basin level: Accounting method and case study in the Segura River Basin, Spain. Ecological Indicators. 2016; 60:1173–1183. doi: 10.1016/j.ecolind.2015.08.032 [DOI] [Google Scholar]
  • 33.Whler L, Brouwer P, Augustijn DCM, Hoekstra AY, Hogeboom RJ, Irvine B, et al. An integrated modelling approach to derive the grey water footprint of veterinary antibiotics. Environmental Pollution. 2021; 288:117746. doi: 10.1016/j.envpol.2021.117746 [DOI] [PubMed] [Google Scholar]
  • 34.Kerm PV. Adaptive kernel density estimation. Stata Journal. 2003; 3(2):148–156. doi: 10.1177/1536867X0300300204 [DOI] [Google Scholar]
  • 35.Wang S, Li A, Wen K, Wu X. Robust kernels for kernel density estimation. Economics Letters. 2020; 191:109138. doi: 10.1016/j.econlet.2020.109138 [DOI] [Google Scholar]
  • 36.Sun C, Bai T, Han Q. The regional and structural equilibrium analysis of grey water footprint in China based on Gini coefficient. Journal of Natural Resources. 2016; 31(12):2047–2059. CNKI:SUN:ZRZX.0.2016-12-007. [Google Scholar]
  • 37.Bai T, Sun C. Regional inequality and factor decomposition of the per capita grey water footprint in China. Acta Ecologica Sinica. 2018; 38(17):6314–6325. doi: 10.5846/stxb201709291764 [DOI] [Google Scholar]
  • 38.Zhang Z, Sun C. Driving effect measurements and spatial-temporal variation of the per capita gray water ecological footprint in China. Acta Ecologica Sinica. 2018; 38(13):4596–4608. doi: 10.5846/stxb201706221136 [DOI] [Google Scholar]
  • 39.Lv M, Song Y, Li X, Wang M, Qu Y. Spatiotemporal characteristics and driving factors of global planetary albedo: An analysis using the Geodetector method. Theoretical and Applied Climatology. 2022; 147(1):737–752. doi: 10.1007/s00704-021-03858-9 [DOI] [Google Scholar]
  • 40.Hoekstra AY, Chapagain AK, Aldaya MM, Hoekstra MMM. The water footprint assessment manual: Setting the global standard. Earthscan. 2011. [Google Scholar]
  • 41.Dagum C. A new approach to the decomposition of the Gini income inequality ratio. Income Inequality, Poverty, and Economic Welfare. 1998; 47–63. doi: 10.1007/978-3-642-51073-1_4 [DOI] [Google Scholar]
  • 42.Alvaredo F. A note on the relationship between top income shares and the Gini coefficient. Economics Letters. 2011; 110(3):274–277. doi: 10.1016/j.econlet.2010.10.008 [DOI] [Google Scholar]
  • 43.Wang J, Xu C. Geodetector: Principle and perspective. Acta Geographica Sinica. 2017; 72(1):116–134. doi: 10.11821/dlxb201701010 [DOI] [Google Scholar]
  • 44.Lin J, Weng L, Dai Y. Study on the spatial and temporal patterns of grey water footprints and its decoupling relationship in China. Water Conservancy Science and Technology and Economy. 2019; 25(9):14–21. CNKI:SUN:SLKY.0.2019-09-003. [Google Scholar]
  • 45.Sun Y. "Watershed Restrictions" to explore new ways to control pollution in watersheds. Environmental Protection. 2007; (14):51–52. CNKI:SUN:HJBU.0.2007-14-018. [Google Scholar]
  • 46.Yang Y, Yan L, Cheng W. Estimation of non-point source pollution in the Yellow River Basin. Yellow River. 2011; 33(11):66–68. doi: 10.3969/j.issn.1000-1379.2011.11.025 [DOI] [Google Scholar]
  • 47.Li J, Peng K, Hao G, Li H, Li S. Research progress on quantification and control of non-point source pollution load in the Yellow River Basin. Water Resources Protection. 2021; 37(1):90–102. doi: 10.3880/j.issn.1004-6933.2021.01.014 [DOI] [Google Scholar]
  • 48.Kong D, Miao C, Wu J, Duan Q, Sun Q, Ye A, et al. The hydro-environmental response on the lower Yellow River to the water–sediment regulation scheme. Ecological Engineering. 2015; 79:69–79. doi: 10.1016/j.ecoleng.2015.03.009 [DOI] [Google Scholar]
  • 49.Chen Q, Guo B, Zhao C, Xing B. Characteristics of CH4 and CO2 emissions and influence of water and salinity in the Yellow River delta wetland, China. Environmental Pollution. 2018; 239:289–299. doi: 10.1016/j.envpol.2018.04.043 [DOI] [PubMed] [Google Scholar]
  • 50.Teklehaimanot GZ, Kamika I, Coetzee MAA, Momba MNB. Population growth and its impact on the design capacity and performance of the wastewater treatment plants in Sedibeng and Soshanguve, South Africa. Environmental Management. 2015; 56:984–997. doi: 10.1007/s00267-015-0564-3 [DOI] [PubMed] [Google Scholar]

Decision Letter 0

Xianzhong Cao

6 Dec 2022

PONE-D-22-25102Variation and internal-external driving forces of grey water footprint efficiency in China's Yellow River BasinPLOS ONE

Dear Dr. Liu,

Thank you for submitting your manuscript to PLOS ONE. After careful consideration, we feel that it has merit but does not fully meet PLOS ONE’s publication criteria as it currently stands. Therefore, we invite you to submit a revised version of the manuscript that addresses the points raised during the review process.

Please submit your revised manuscript by Jan 20 2023 11:59PM. If you will need more time than this to complete your revisions, please reply to this message or contact the journal office at plosone@plos.org. When you're ready to submit your revision, log on to https://www.editorialmanager.com/pone/ and select the 'Submissions Needing Revision' folder to locate your manuscript file.

Please include the following items when submitting your revised manuscript:

  • A rebuttal letter that responds to each point raised by the academic editor and reviewer(s). You should upload this letter as a separate file labeled 'Response to Reviewers'.

  • A marked-up copy of your manuscript that highlights changes made to the original version. You should upload this as a separate file labeled 'Revised Manuscript with Track Changes'.

  • An unmarked version of your revised paper without tracked changes. You should upload this as a separate file labeled 'Manuscript'.

If you would like to make changes to your financial disclosure, please include your updated statement in your cover letter. Guidelines for resubmitting your figure files are available below the reviewer comments at the end of this letter.

If applicable, we recommend that you deposit your laboratory protocols in protocols.io to enhance the reproducibility of your results. Protocols.io assigns your protocol its own identifier (DOI) so that it can be cited independently in the future. For instructions see: https://journals.plos.org/plosone/s/submission-guidelines#loc-laboratory-protocols. Additionally, PLOS ONE offers an option for publishing peer-reviewed Lab Protocol articles, which describe protocols hosted on protocols.io. Read more information on sharing protocols at https://plos.org/protocols?utm_medium=editorial-email&utm_source=authorletters&utm_campaign=protocols.

We look forward to receiving your revised manuscript.

Kind regards,

Xianzhong Cao

Academic Editor

PLOS ONE

Journal Requirements:

When submitting your revision, we need you to address these additional requirements.

1. Please ensure that your manuscript meets PLOS ONE's style requirements, including those for file naming. The PLOS ONE style templates can be found at

https://journals.plos.org/plosone/s/file?id=wjVg/PLOSOne_formatting_sample_main_body.pdf  and

https://journals.plos.org/plosone/s/file?id=ba62/PLOSOne_formatting_sample_title_authors_affiliations.pdf

2. Please note that PLOS ONE has specific guidelines on code sharing for submissions in which author-generated code underpins the findings in the manuscript. In these cases, all author-generated code must be made available without restrictions upon publication of the work. Please review our guidelines at https://journals.plos.org/plosone/s/materials-and-software-sharing#loc-sharing-code and ensure that your code is shared in a way that follows best practice and facilitates reproducibility and reuse. New software must comply with the Open Source Definition.

3. Thank you for stating the following financial disclosure:

“This work is supported by “the Graduate Research and Innovation Projects of Jiangsu Province” (grant number KYCX21_0441) and “the Fundamental Research Funds for the Central Universities” (grant number B220203024).”

Please state what role the funders took in the study.  If the funders had no role, please state: "The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript."

If this statement is not correct you must amend it as needed.

Please include this amended Role of Funder statement in your cover letter; we will change the online submission form on your behalf.

4. Thank you for stating the following in the Acknowledgments Section of your manuscript:

“This work is supported by “the Graduate Research and Innovation Projects of Jiangsu Province” (grant number KYCX21_0441) and “the Fundamental Research Funds for the Central Universities” (grant number B220203024).”

We note that you have provided additional information within the Acknowledgements Section that is not currently declared in your Funding Statement. Please note that funding information should not appear in the Acknowledgments section or other areas of your manuscript. We will only publish funding information present in the Funding Statement section of the online submission form.

Please remove any funding-related text from the manuscript and let us know how you would like to update your Funding Statement. Currently, your Funding Statement reads as follows:

“This work is supported by “the Graduate Research and Innovation Projects of Jiangsu Province” (grant number: KYCX21_0441; funder: Lihua Yang) and “the Fundamental Research Funds for the Central Universities” (grant number: B220203024; funder: Lihua Yang).Lihua Yang is the first author of this manuscript.”

Please include your amended statements within your cover letter; we will change the online submission form on your behalf.

5. PLOS requires an ORCID iD for the corresponding author in Editorial Manager on papers submitted after December 6th, 2016. Please ensure that you have an ORCID iD and that it is validated in Editorial Manager. To do this, go to ‘Update my Information’ (in the upper left-hand corner of the main menu), and click on the Fetch/Validate link next to the ORCID field. This will take you to the ORCID site and allow you to create a new iD or authenticate a pre-existing iD in Editorial Manager. Please see the following video for instructions on linking an ORCID iD to your Editorial Manager account: https://www.youtube.com/watch?v=_xcclfuvtxQ

6. In your Data Availability statement, you have not specified where the minimal data set underlying the results described in your manuscript can be found. PLOS defines a study's minimal data set as the underlying data used to reach the conclusions drawn in the manuscript and any additional data required to replicate the reported study findings in their entirety. All PLOS journals require that the minimal data set be made fully available. For more information about our data policy, please see http://journals.plos.org/plosone/s/data-availability.

Upon re-submitting your revised manuscript, please upload your study’s minimal underlying data set as either Supporting Information files or to a stable, public repository and include the relevant URLs, DOIs, or accession numbers within your revised cover letter. For a list of acceptable repositories, please see http://journals.plos.org/plosone/s/data-availability#loc-recommended-repositories. Any potentially identifying patient information must be fully anonymized.

Important: If there are ethical or legal restrictions to sharing your data publicly, please explain these restrictions in detail. Please see our guidelines for more information on what we consider unacceptable restrictions to publicly sharing data: http://journals.plos.org/plosone/s/data-availability#loc-unacceptable-data-access-restrictions. Note that it is not acceptable for the authors to be the sole named individuals responsible for ensuring data access.

We will update your Data Availability statement to reflect the information you provide in your cover letter.

7. We note that  Figure 3 in your submission contain map images which may be copyrighted. All PLOS content is published under the Creative Commons Attribution License (CC BY 4.0), which means that the manuscript, images, and Supporting Information files will be freely available online, and any third party is permitted to access, download, copy, distribute, and use these materials in any way, even commercially, with proper attribution. For these reasons, we cannot publish previously copyrighted maps or satellite images created using proprietary data, such as Google software (Google Maps, Street View, and Earth). For more information, see our copyright guidelines: http://journals.plos.org/plosone/s/licenses-and-copyright.

 We require you to either (1) present written permission from the copyright holder to publish these figures specifically under the CC BY 4.0 license, or (2) remove the figures from your submission:

      1. You may seek permission from the original copyright holder of Figure 3 to publish the content specifically under the CC BY 4.0 license. 

We recommend that you contact the original copyright holder with the Content Permission Form (http://journals.plos.org/plosone/s/file?id=7c09/content-permission-form.pdf) and the following text:

“I request permission for the open-access journal PLOS ONE to publish XXX under the Creative Commons Attribution License (CCAL) CC BY 4.0 (http://creativecommons.org/licenses/by/4.0/). Please be aware that this license allows unrestricted use and distribution, even commercially, by third parties. Please reply and provide explicit written permission to publish XXX under a CC BY license and complete the attached form.”

 Please upload the completed Content Permission Form or other proof of granted permissions as an "Other" file with your submission.

In the figure caption of the copyrighted figure, please include the following text: “Reprinted from [ref] under a CC BY license, with permission from [name of publisher], original copyright [original copyright year].”

       2. If you are unable to obtain permission from the original copyright holder to publish these figures under the CC BY 4.0 license or if the copyright holder’s requirements are incompatible with the CC BY 4.0 license, please either i) remove the figure or ii) supply a replacement figure that complies with the CC BY 4.0 license. Please check copyright information on all replacement figures and update the figure caption with source information. If applicable, please specify in the figure caption text when a figure is similar but not identical to the original image and is therefore for illustrative purposes only.

The following resources for replacing copyrighted map figures may be helpful:

 USGS National Map Viewer (public domain): http://viewer.nationalmap.gov/viewer/

The Gateway to Astronaut Photography of Earth (public domain):  http://eol.jsc.nasa.gov/sseop/clickmap/

Maps at the CIA (public domain): https://www.cia.gov/library/publications/the-world-factbook/index.html and https://www.cia.gov/library/publications/cia-maps-publications/index.html

NASA Earth Observatory (public domain): http://earthobservatory.nasa.gov/

Landsat: http://landsat.visibleearth.nasa.gov/

USGS EROS (Earth Resources Observatory and Science (EROS) Center) (public domain): http://eros.usgs.gov/#

Natural Earth (public domain): http://www.naturalearthdata.com/

[Note: HTML markup is below. Please do not edit.]

Reviewers' comments:

Reviewer's Responses to Questions

Comments to the Author

1. Is the manuscript technically sound, and do the data support the conclusions?

The manuscript must describe a technically sound piece of scientific research with data that supports the conclusions. Experiments must have been conducted rigorously, with appropriate controls, replication, and sample sizes. The conclusions must be drawn appropriately based on the data presented.

Reviewer #1: Yes

**********

2. Has the statistical analysis been performed appropriately and rigorously?

Reviewer #1: Yes

**********

3. Have the authors made all data underlying the findings in their manuscript fully available?

The PLOS Data policy requires authors to make all data underlying the findings described in their manuscript fully available without restriction, with rare exception (please refer to the Data Availability Statement in the manuscript PDF file). The data should be provided as part of the manuscript or its supporting information, or deposited to a public repository. For example, in addition to summary statistics, the data points behind means, medians and variance measures should be available. If there are restrictions on publicly sharing data—e.g. participant privacy or use of data from a third party—those must be specified.

Reviewer #1: Yes

**********

4. Is the manuscript presented in an intelligible fashion and written in standard English?

PLOS ONE does not copyedit accepted manuscripts, so the language in submitted articles must be clear, correct, and unambiguous. Any typographical or grammatical errors should be corrected at revision, so please note any specific errors here.

Reviewer #1: Yes

**********

5. Review Comments to the Author

Please use the space provided to explain your answers to the questions above. You may also include additional comments for the author, including concerns about dual publication, research ethics, or publication ethics. (Please upload your review as an attachment if it exceeds 20,000 characters)

Reviewer #1: This manuscript investigated the spatial and temporal variation of the grey water footprint (GWF) efficiency based on the measurement of the GWF efficiency, the kernel density estimation and the Dagum Gini coefficient method. The paper is written in sound English, but with some grammar errors. Detailed comments are as follows:

1. “For demonstrating this assessment approach, China's Yellow River Basin is chosen as an example.”, spatial and temporal scales should be clarified for the empirical study in this sentence.

2. “Inter-regional variation is the 41 primary source of spatial variation, with an average contribution of 73.39%.”, please clarify inter-regional variation of what?

3. A map should be added to provide a detailed description of the study area.

4. As to the numbers in the text and tables, I suggest the authors keep only two decimal places in a number.

5. In methods and data, the use of operator signs in formulas should be uniform.

6. Natural and social conditions differ significantly within provinces, such as Inner Mongolia. Is the provincial-scale analysis too general? If possible, analysis at a more precise scale could be more convincing.

7. According to Fig. 1, both TGWF and GWF efficiency were mutated in 2020. An analysis of this phenomenon can be added to the text.

8. The graphic style of Fig. 3 does not show well the three-dimensional distribution of information. Try adjusting the angle or changing the layout to make the information clear.

9. Some grammar problems can be checked.

**********

6. PLOS authors have the option to publish the peer review history of their article (what does this mean?). If published, this will include your full peer review and any attached files.

If you choose “no”, your identity will remain anonymous but your review may still be made public.

Do you want your identity to be public for this peer review? For information about this choice, including consent withdrawal, please see our Privacy Policy.

Reviewer #1: No

**********

[NOTE: If reviewer comments were submitted as an attachment file, they will be attached to this email and accessible via the submission site. Please log into your account, locate the manuscript record, and check for the action link "View Attachments". If this link does not appear, there are no attachment files.]

While revising your submission, please upload your figure files to the Preflight Analysis and Conversion Engine (PACE) digital diagnostic tool, https://pacev2.apexcovantage.com/. PACE helps ensure that figures meet PLOS requirements. To use PACE, you must first register as a user. Registration is free. Then, login and navigate to the UPLOAD tab, where you will find detailed instructions on how to use the tool. If you encounter any issues or have any questions when using PACE, please email PLOS at figures@plos.org. Please note that Supporting Information files do not need this step.

Decision Letter 1

Xianzhong Cao

6 Mar 2023

Variation and internal-external driving forces of grey water footprint efficiency in China's Yellow River Basin

PONE-D-22-25102R1

Dear Dr. Liu,

We’re pleased to inform you that your manuscript has been judged scientifically suitable for publication and will be formally accepted for publication once it meets all outstanding technical requirements.

Within one week, you’ll receive an e-mail detailing the required amendments. When these have been addressed, you’ll receive a formal acceptance letter and your manuscript will be scheduled for publication.

An invoice for payment will follow shortly after the formal acceptance. To ensure an efficient process, please log into Editorial Manager at http://www.editorialmanager.com/pone/, click the 'Update My Information' link at the top of the page, and double check that your user information is up-to-date. If you have any billing related questions, please contact our Author Billing department directly at authorbilling@plos.org.

If your institution or institutions have a press office, please notify them about your upcoming paper to help maximize its impact. If they’ll be preparing press materials, please inform our press team as soon as possible -- no later than 48 hours after receiving the formal acceptance. Your manuscript will remain under strict press embargo until 2 pm Eastern Time on the date of publication. For more information, please contact onepress@plos.org.

Kind regards,

Xianzhong Cao

Academic Editor

PLOS ONE

Additional Editor Comments (optional):

Reviewers' comments:

Reviewer's Responses to Questions

Comments to the Author

1. If the authors have adequately addressed your comments raised in a previous round of review and you feel that this manuscript is now acceptable for publication, you may indicate that here to bypass the “Comments to the Author” section, enter your conflict of interest statement in the “Confidential to Editor” section, and submit your "Accept" recommendation.

Reviewer #2: (No Response)

**********

2. Is the manuscript technically sound, and do the data support the conclusions?

The manuscript must describe a technically sound piece of scientific research with data that supports the conclusions. Experiments must have been conducted rigorously, with appropriate controls, replication, and sample sizes. The conclusions must be drawn appropriately based on the data presented.

Reviewer #2: Yes

**********

3. Has the statistical analysis been performed appropriately and rigorously?

Reviewer #2: Yes

**********

4. Have the authors made all data underlying the findings in their manuscript fully available?

The PLOS Data policy requires authors to make all data underlying the findings described in their manuscript fully available without restriction, with rare exception (please refer to the Data Availability Statement in the manuscript PDF file). The data should be provided as part of the manuscript or its supporting information, or deposited to a public repository. For example, in addition to summary statistics, the data points behind means, medians and variance measures should be available. If there are restrictions on publicly sharing data—e.g. participant privacy or use of data from a third party—those must be specified.

Reviewer #2: Yes

**********

5. Is the manuscript presented in an intelligible fashion and written in standard English?

PLOS ONE does not copyedit accepted manuscripts, so the language in submitted articles must be clear, correct, and unambiguous. Any typographical or grammatical errors should be corrected at revision, so please note any specific errors here.

Reviewer #2: Yes

**********

6. Review Comments to the Author

Please use the space provided to explain your answers to the questions above. You may also include additional comments for the author, including concerns about dual publication, research ethics, or publication ethics. (Please upload your review as an attachment if it exceeds 20,000 characters)

Reviewer #2: The authors comprehensively revised the manuscript according to the comments of reviewers. I have only small suggestions for the manuscript as follows:

1. Please indicate the units of variables in the method and data parth.

2. In the results section, it can be seen from Figure 2 that in 2016, GWF decreased significantly and the efficiency of GWF increased significantly. Please explain the reason briefly.

3. Line 425, 76.37% should be 76.38%.

4. In the internal driving forces section, Please describe the p value in Table 2.

**********

7. PLOS authors have the option to publish the peer review history of their article (what does this mean?). If published, this will include your full peer review and any attached files.

If you choose “no”, your identity will remain anonymous but your review may still be made public.

Do you want your identity to be public for this peer review? For information about this choice, including consent withdrawal, please see our Privacy Policy.

Reviewer #2: No

**********

Acceptance letter

Xianzhong Cao

14 Mar 2023

PONE-D-22-25102R1

Variation and internal-external driving forces of grey water footprint efficiency in China's Yellow River Basin

Dear Dr. Liu:

I'm pleased to inform you that your manuscript has been deemed suitable for publication in PLOS ONE. Congratulations! Your manuscript is now with our production department.

If your institution or institutions have a press office, please let them know about your upcoming paper now to help maximize its impact. If they'll be preparing press materials, please inform our press team within the next 48 hours. Your manuscript will remain under strict press embargo until 2 pm Eastern Time on the date of publication. For more information please contact onepress@plos.org.

If we can help with anything else, please email us at plosone@plos.org.

Thank you for submitting your work to PLOS ONE and supporting open access.

Kind regards,

PLOS ONE Editorial Office Staff

on behalf of

Professor Xianzhong Cao

Academic Editor

PLOS ONE

Associated Data

    This section collects any data citations, data availability statements, or supplementary materials included in this article.

    Supplementary Materials

    S1 File

    (TXT)

    S1 Data

    (XLSX)

    Attachment

    Submitted filename: Response to Reviewers.docx

    Data Availability Statement

    All relevant data and the sources have been provided in the paper and the Supporting Information file.


    Articles from PLOS ONE are provided here courtesy of PLOS

    RESOURCES