Abstract
Current-induced spin–orbit torques (SOTs) enable fast and efficient manipulation of the magnetic state of magnetic tunnel junctions (MTJs), making them attractive for memory, in-memory computing, and logic applications. However, the requirement of the external magnetic field to achieve deterministic switching in perpendicularly magnetized SOT-MTJs limits its implementation for practical applications. Here, we introduce a field-free switching (FFS) solution for the SOT-MTJ device by shaping the SOT channel to create a “bend” in the SOT current. The resulting bend in the charge current creates a spatially nonuniform spin current, which translates into inhomogeneous SOT on an adjacent magnetic free layer enabling deterministic switching. We demonstrate FFS experimentally on scaled SOT-MTJs at nanosecond time scales. This proposed scheme is scalable, material-agnostic, and readily compatible with wafer-scale manufacturing, thus creating a pathway for developing purely current-driven SOT systems.
Keywords: field-free switching, spin−orbit torques, magnetic tunnel junction, memories, MRAM, spintronics
Electrical manipulation of magnetic tunnel junctions (MTJs) is gaining importance for embedded memory applications and spin-based logic due to the nonvolatile nature of ferromagnets, CMOS compatibility, and high operational speed.1 In particular, MTJs switched with spin–orbit torque (SOT) are promising owing to their high endurance (>1014), large energy efficiency (<1 fJ), and fast switching speed (<1 ns) characteristics.2−7 In SOT-MTJs, the spin Hall effect in the SOT channel (heavy metal) and the interfacial Rashba interaction at the SOT channel/ferromagnetic free layer (FL) interface creates a spin current with in-plane spin polarization, which induces an instantaneous torque on the magnetization. To enable ultrafast SOT-induced switching, perpendicularly magnetized MTJs (pMTJs) are preferred.4 However, in such a configuration, the generated torques cannot intrinsically differentiate between the two states of pMTJs, thus resulting in nondeterministic switching.8 To enable SOT-induced deterministic switching, the time-reversal symmetry needs to be broken; this is traditionally achieved with an external in-plane magnetic field (Bip) along the electric current direction. However, using this external field hinders the potential of SOT-MTJs for embedded memory applications.
Various alternatives have been proposed in the literature to remove or substitute this external field, which can be broadly grouped into four categories:9 (i) built-in magnetic fields by exchange bias10 or a decoupled in-plane magnet grown in the pMTJ structure;11−13 (ii) additional spin currents are produced with either crystalline materials (PtCu,14,15 WTe216−18), Rashba field modulation,19,20 or competing spin Hall angle;21 (iii) hybrid approaches combining domain wall motion,22 spin-transfer torque,23 Dzyaloshinskii–Moriya interaction (DMI) modulation,24 the spin current generated from an in-plane magnetized ferromagnetic layer25 or coupled nanomagnets26 with SOT-induced switching; (iv) structural asymmetry created by a gradient of the FL thickness27,28 or the SOT channel thickness,29 tilting the easy axis of the FL,30 and engineering the FL geometry.31
In this study, we propose a new field-free switching (FFS) scheme for SOT-pMTJs by introducing a geometric curvature in the SOT channel (Figure 1a). This curvature creates a structural asymmetry in the system with the flow of inhomogeneous charge current in the SOT channel, which modifies the flow and polarization of spin current. These modifications in spin current further cause an inhomogeneous SOT on the FL, thus breaking the time-reversal symmetry. We demonstrate deterministic FFS for current pulses down to 5 ns and elucidate the underlying mechanism with micromagnetic and finite-element simulations. Importantly, this approach has no additional restriction on the material choices for the SOT channel or the FL. Manipulating magnets by inducing a curvature in the SOT channel holds exciting potential for practical application due to its scalability, integration friendliness, and reproducibility.
In this work, we performed the experiments on our baseline top-pinned SOT-MTJs fabricated on 300 mm wafers and annealed to 300 °C, as reported in ref (6). The MTJ consists of a 0.9 nm CoFeB free layer, a MgO barrier with a resistance area product of ∼51 Ω μm2, and a 1.1 nm CoFeB reference layer, which is pinned to a synthetic antiferromagnetic (SAF) hard layer. The hard layer pins the reference layer in the −z direction such that the MTJ is in a low resistive parallel (P) or high resistive antiparallel (AP) state when the FL magnetization points toward the −z (+z) direction, respectively. MTJ pillars have a circular cross-section with nominal diameters of 60, 80, and 100 nm. The MTJs are deposited on a 3.5 nm thick β-W SOT channel with a resistivity of 160 μΩ cm and an effective spin Hall angle (θSH) estimated to be −0.43 from our second-harmonic measurement.32 All properties for each dimension are summarized in section I in the Supporting Information. Henceforth, in this article, we focus on the results from 60 nm MTJs.
The device design used in our study (Figure 1a) is a standard straight-line SOT channel with MTJ positioned at the center of the channel, referred to as a straight structure (as a reference structure), and a cornered SOT channel with a MTJ positioned on the corner, referred to as a bending structure. Both structures have a SOT channel width of 140 nm; meanwhile, the length in the bending structure is longer than that in the straight structure. This longer length in bending structures causes higher resistance (4350 Ω) than in straight structures (500 Ω). The MTJ shows a square hysteresis loop (Figure 1b) with similar magnetic properties for both structures. The median values for over 20 structures of each type are a tunnel magnetoresistance ratio (TMR) of ∼73 ± 4%, a coercive field (Bc) of ∼60 ± 6 mT, an offset field along the z direction |Boff| ≈ 6.8 ± 4 mT (favoring AP state), and an anisotropy field Bk ≈ 180 ± 3.4 mT.
The surface profile of the magnitude of the spin current (JS) along z and the direction of spin current polarization (σ) for both structures are simulated using COMSOL (section II in the Supporting Information). For straight structures, when a charge current is applied along +x, due to the spin Hall effect, a constant JS and a homogeneous distribution of σ in the −y direction is observed (Figure 1c). In the bending structures, the reorientation of electron flow at the inner corner causes a rotation of σ(r), which modifies the SOT direction across the FL.33 Additionally, the spatial distribution of charge current (JC(r)) results in a nonuniform amplitude of JS (Figure 1d), as , which results in a gradient of JS(r) in the xy plane with the highest amplitude of JS(r) at the inner corner. This generated spin current gradient is independent of the direction of charge current due to higher current accumulation at the inner corner of the SOT channel. Importantly, due to the inhomogeneous σ(r) and JS(r), a spatially varying SOT is experienced by the FL; thus, it breaks the time-reversal symmetry, and it allows deterministic switching.
We perform SOT-induced magnetization switching by passing direct current (DC) of variable amplitudes (ISOT) through the SOT channel. A postpulse readout of the FL state is sensed by applying a low read current (Iread ≈ 5 μA) through the MTJ. During the switching, Bip can be applied in the xy plane with a maximum amplitude of 40 mT. Figure 1e shows typical RMTJ–ISOT switching loops for straight structures obtained at different Bip applied along the x direction. The switching conditions are as expected for a negative spin Hall angle; at zero external fields, the device does not switch deterministically, and a minimum Bip ≈ ±10 mT is required to define the switching polarity. When a positive ISOT is applied, the MTJ state switches from an antiparallel (AP) to a parallel (P) state for Bip < −10 mT, whereas the P–AP transition for Bip > 10 mT. Thus, SOT switching for straight structures with positive or negative Bip generates clockwise (CW) or counterclockwise (CCW) switching loops, respectively. The average switching current (ISW) over our devices is ∼500 μA, corresponding to a switching current density (JSW) of 9.5 × 107 A cm–2 for Bip = −10 mT.
Remarkably, for the bending structures shown in Figure 1f, deterministic bipolar switching occurs at Bip = 0 mT, thus confirming the proposed concept of time-reversal symmetry breaking due to inhomogeneous SOT below the FL and JS gradient. FFS loops in bending structures have CW polarity, the same as the straight structures with Bip < 0, indicating the direction of the effective SOT field (Beff) created by bending the SOT channel. When applying Bip ≈ 10 mT (at −45° in the xy plane, which is the effective JC direction), the device shows stochastic switching, whereas a further increase of Bip causes the switching polarity to reverse from CW to CCW loops. This change in switching polarity suggests that for Bip > 15 mT, Bip dominates over Beff. The average ISW of the bending structure is like that for straight structures, with ∼530 μA, corresponding to JSW = 1 × 108 A cm–2 at Bip = 0 mT. We observe FFS using MTJ sizes of 80 and 100 nm on a W-based SOT channel. Importantly, we observe FFS with Pt-based MTJs, but with opposite switching polarities. Since Pt has an opposite spin Hall angle to W, this validates that SOT physics dominates the FFS in bending structures (section III in the Supporting Information).
To investigate the direction and the magnitude of Beff in the bending structure, we perform switching measurements with an angular variation of Bip and compare it to straight structures. We record average switching loops in the presence of |Bip| = 25 mT with varying directions in the xy plane from −180° ≤ Φ ≤ 180°. We observe a cosine angular dependence of ISW with Φ, which is due to the variation of angle between Bip and the antidamping SOT field (BAD).8,34 The opposite trend in variation of ISW for P–AP and AP–P transitions relates to the interplay between the field-like field (BFL) and Bip, which add or subtract from each other.35 The direction of Beff can be identified by the angular variation of Bip since the interplay among Bip, BAD, and BFL determines the region for the lowest switching current and stochastic (random) switching.36 In the straight structure (Figure 2a), the region for stochastic switching occurs at ∼±90°, and the least switching current occurs at 180° for CW (0° for CCW switching loop). Beff is determined by the sum of BFL(34) or BAD(35) in SOT-induced switching in the presence of Bip and is along the direction of current (180° for CW switching loops).
For the bending structure (Figure 2b), the region showing the CW switching loop is for angles between −140° and 50°. The minimum switching current required for both transitions are at 135° and −30° for CW and CCW switching loops, respectively. Using the same analogy for bending structures, we can conclude that Beff contributing to FFS will be along 135°. We have used this understanding for measuring the average RMTJ−ISOT switching loop in Figure 1e,f.
To gain insight into the underlying switching mechanism, we performed micromagnetic simulations for the bending and straight structures. In the micromagnetic framework, we consider the exchange interaction, anisotropy, damping parameter, generated antidamping and field-like SOT, Oersted field, magnetostatic interaction, and DMI. We first perform a finite-element simulation to calculate the spatial distribution of JC induced by the bent SOT channel, resulting in the gradient in JS, inhomogeneous σ (Figure 1d), and the Oersted field. The magnetization trajectory in our simulation is recorded by initializing the FL along +z (or −z) and followed by a relaxation of 0.1 ns. Then, the ISOT switching pulse is applied to 1 ns (indicated by the yellow region in Figure 3a,b), and the system is allowed to relax for another 6 ns with the current pulse turned off. For both the straight structure (Figure 3a) and bending structure (Figure 3b), deterministic switching occurs with an AP–P transition for ISOT > 0 (inset graph shows the P–AP transition for ISOT< 0), in the presence of Bip = −20 mT and absence of field, respectively. The FFS is reliable and shows fixed switching polarity, confirming the CW loops observed in the experiments. Notably, there is no switching when the FL is forced to have opposite switched polarity (setting initial P (AP) state for ISOT > 0 (ISOT < 0)).
In Figure 3c, the snapshots of magnetic configuration at different times for straight structures show the reversal by chiral domain nucleation at the edge followed by domain wall propagation across the FL, typical for SOT-MTJs of diameter ≥50 nm with perpendicular magnetic anisotropy (PMA).7,37 The nucleation point is different for both transitions, as it is mainly driven by DMI35 and SOT fields, and it has a 4-fold symmetry that depends on the interplay of the in-plane field and current polarities. Interestingly, nucleation occurs on the spot closer to the inner corner in bending structures (Figure 3d) regardless of the initial magnetization or current direction in the SOT channel. Given the spatial current distribution, nucleation is always favored at the inner corner of FL due to the higher spin current density for both polarities, and it is followed by a domain wall propagation until the current pulse is turned off. The domain wall propagation is attributed to an inhomogeneous SOT31 due to the continuous spin polarization direction change. Once the pulse is turned off, with the support of exchange interaction, anisotropy, and DMI, the magnetization relaxes to a uniform ground state determined by the initial nucleated domain orientation. We further investigated the roles of spin current gradient, inhomogeneous spin polarization, and DMI on the switching of bending structure (section IV.i in the Supporting Information). Notably, the spin current gradient contributes to fixing the nucleation point at the inner corner of the SOT channel for both current polarities. The domain wall dynamics are dictated by the direction of spin polarization and the strength and direction of DMI. The domain wall magnetization experiences an inhomogeneous SOT due to spatially varying spin polarization; its magnetization orientation depends on the direction of current and initial magnetization of the FL, thus enabling the differentiation between the two transitions. The DMI strength and chirality impacts the postnucleation dynamics with only positive DMI (promoting right-handed domain wall chirality), enabling switching for our current bending structure design. The switching polarity is determined by the combination of DMI chirality and SOT induced on the domain wall magnetization due to spatially varying spin polarization. The fixed nucleation point determined by the spin current gradient and followed by complete switching can also be observed for different pulse parameters, MTJ sizes, and MTJ locations on the SOT channel, indicating reliable operations (details are discussed in section IV.ii in the Supporting Information). We also simulate the reversal dynamics at an elevated temperature and observe no impact on the nucleation site or the switching trajectory compared to the 0 K simulations, indicating that the switching is reliable against random thermal fluctuation. This corroborates our assumption that the deterministic nature of the FFS process is due to the spatially varying SOT assisted by DMI.
In addition, we investigated the role of inhomogeneous BFL and the Oersted field generated due to the curvature of the SOT channel by performing simulation in the presence and absence of these parameters, there is little change between the magnetization trajectory (Supporting Information IV.iii). The damping parameter is varied in magnitude; there is no significant variation in the switching trace recorded in the simulations. Meanwhile, the spatial variation of the magnetic parameters due to inhomogeneous Joule heating of the SOT channel has a moderate influence; we observe that it only lowers the critical switching current and does not impact the switching dynamics for the bending structure. The magnetization reversal in bending structure is mainly influenced by inhomogeneous current distribution below the SOT and chirality of the DMI; other factors such as the Oersted field, BFL, damping parameter, and inhomogeneous Joule heating of the SOT channel play no role in time-reversal symmetry breaking but only contribute toward enhancing (reducing) the switching reliability.
Notably, we experimentally compare the pulsed switching of the bending structure at Bip = 0 mT and the switching of the straight structure at various in-plane fields in Figure 4a (more details on the experimental setup are given in section III in the Supporting Information). The pulsed switching confirms that the proposed FFS mechanism seems not limited by switching speed, as we can deterministically switch at 5 ns with JSW = 1.5 × 108 A cm–2. Unfortunately, for a pulse width (τp) shorter than 5 ns, switching is limited by the large SOT channel resistance of the bending structures and our experimental setup voltage delivery. At longer τp (>50 ns), the ISW for the bending structure (Bip = 0 mT) is like that of straight structure (Bip = −12.8 mT along the x direction) as the stochastic thermal fluctuations contribute to lowering the required Beff (∝JS) for bending structures. The difference in switching current increases at shorter pulses between both structures as the Beff in bending structures is current-amplitude-dependent; in contrast, Beff is static (Beff=Bip) for straight structures. We also note that reliable switching at 10 ns is possible for bending structures with larger MTJ diameters of 80 and 100 nm (section III in the Supporting Information).
Given the switching dynamics observed in the simulations, and the importance of a z field on DW displacement,38 we measured the switching as a function of the direction of the stray field produced by the hard layer and the out-of-plane field (Bz), as shown in Figure 4b. The bending structure device with a hard layer magnetized in +z (SAF-up) shows reliable switching for a wide range of z fields, whereas SAF-down structures show switching only for a large positive z field. This shows that the stray field generated from the hard layer impacts the switching dynamics by either assisting or competing with BAD on the domain wall magnetization during the reversal38 (more details are given in section V in the Supporting Information). This effect is more pronounced in bending structures than in straight structures as the magnetization of the domain wall in the bending structure is determined by the DMI (intrinsic property), whereas for the straight structure, it is controlled by the magnitude and direction of Bip.
Finally, to access the impact of bending structures on the architecture design, we performed a design-to-technology co-optimization (DTCO) analysis for bending structures and compared it to other embedded memory technologies such as static-RAM, STT-MRAM, and SOT-MRAM at the 5 nm technology node39 (section VI in the Supporting Information). Notably, we observed that bending the SOT channel does not impact the area per bit compared to the standard SOT-MRAM, with the added advantage of field-free switching and no penalty on the switching current.
However, various aspects need to be investigated to improve the switching performance of bending structures in terms of design and material characteristics for making it a promising FFS solution. First, understanding the impact of the stray field generated from the SAF hard layer on FFS and engineering the hard layer to assist in the domain wall dynamics is required. Second, optimizing interface properties between the FL and SOT channel, such as DMI and θSH, will cause an increase in spin current gradient and improve the domain wall dynamics. Third, redesigning the structure by shortening the SOT channel will reduce the resistance, limit the breakdown of the device, and give the opportunity to study a shorter pulse regime. Lastly, placing the MTJ closer to the inner corner will cause a larger gradient in the current below the MTJ. The expected reduction in the critical current is ∼25%, if the MTJ is closer to the inner corner of the SOT channel by 18 nm compared to our current design. The DTCO analysis for this optimized location of MTJ shows properties similar to that of the straight structure.
To conclude, we proposed and demonstrated a new FFS concept by introducing a curvature in the SOT channel in a SOT-pMTJ with no impact on the static properties of the MTJ stack. Deterministic field-free switching is achieved down to nanosecond pulses due to time-reversal symmetry breaking created by inhomogeneous SOT below the free layer. The switching mechanism can be explained by the creation of a fixed point for nucleation determined by the geometry of the SOT channel, followed by a complex domain wall propagation supported by inhomogeneous SOT. Bending structure design opens a new route for realizing FFS in SOT-pMTJs: it is scalable, material agnostic, and suitable for large-scale integration.
Methods
Sample Fabrication
The devices were fabricated on IMEC’s 300 mm MRAM pilot line. SOT-MTJ stacks are deposited on preprocessed wafers made of W-VIA bottom electrodes embedded in SiO2. The SOT-MTJs were deposited in situ at room temperature by physical vapor deposition in a 300 mm cluster EC7800 Canon-Anelva tool and subsequently annealed for 30 min at 300 °C in the presence of a perpendicular magnetic field of 1 T. The material composition of the top-pinned MTJ stack for W/CoFeB is W(3.5)/Co20Fe60B20(0.9)/MgO (∼1)/Co17.5Fe52.5B30(1.1)/W(0.3)/Co(1.2)/Ru(0.85)/Co(0.6)/Pt(0.8)[Co(0.3)/Pt(0.8)]6Ru(5) (units in nm). Then, the MTJ pillar was patterned using 193 nm immersion lithography followed by ion-beam etching at normal incidence with the etch stop condition optimized. The SOT channel is intact without producing a side wall short across the barrier. The copper electrodes were fabricated using a dual damascene process to make the top and bottom electrical connections.
Acknowledgments
This work was supported by IMEC’s Industrial Affiliation Program on MRAM devices, ECSEL Joint Undertaking Program (grant No. 876925-project ANDANTE), and the Swiss National Science Foundation (Grant No. 200020_200465).
Data Availability Statement
The data that support the plots within this paper and other findings of this study are available from the corresponding author upon reasonable request.
Supporting Information Available
The Supporting Information is available free of charge at https://pubs.acs.org/doi/10.1021/acs.nanolett.3c00639.
Magnetic properties of bending structure, finite element method simulation, SOT-induced switching in bending structures, experimental setup for DC SOT switching, experimental setup for pulsed SOT switching, field-free switching, micromagnetic simulation, switching mechanism of bending structures, switching robustness of bending structures, change in simulation parameters, influence of SAF hard layer, and bending structure design analysis (PDF)
Author Contributions
K.G. planned and supervised the project. Va.Ka. performed the measurement on devices designed by K.G. F.Y. was in charge of the device integration process. The experimental data were analyzed by Va.Ka., S.R., K.C., and K.G. Micromagnetic simulations were performed by Vi.Kr. and M.G.M. M.G. performed the design-to-technology co-optimization analysis. Va.Ka., S.R., and K.G. wrote the manuscript. All the authors discussed the data and commented on the manuscript.
The authors declare no competing financial interest.
Supplementary Material
References
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Supplementary Materials
Data Availability Statement
The data that support the plots within this paper and other findings of this study are available from the corresponding author upon reasonable request.