Abstract
Reaching net zero emissions and limiting global warming to 2 °C requires the widespread introduction of technology-based solutions to draw down existing atmospheric levels and future emissions of CO2. One such approach is direct air CO2 capture and storage (DACCS), a readily available, yet energy-intensive process. The combination of DACCS and ocean thermal energy conversion (OTEC) allows for independently powered carbon capture plants to inject concentrated carbon into deep marine sediments where storage is generally safe and permanent. OTEC is a form of electricity production that exploits the temperature difference between deep and shallow ocean waters, and can power DACCS on floating platforms at a price competitive with coal-generated electricity. Here we highlight the scale of the challenge facing society. We show that a safe and sustainable level of OTEC-generated electricity powering DACCS for 70 years could result in up to a 35% decrease in the relative global mean temperature warming compared to a business-as-usual emissions scenario.
Subject terms: Climate change, Climate and Earth system modelling, Physical oceanography
Introduction
The 2018 Intergovernmental Panel on Climate Change report noted the need for widespread negative emission technologies in order to meet the goal of the 2015 Paris Accord and limit warming to 1.5 °C since preindustrial times1. This is largely because natural greenhouse gas sinks cannot keep up with the rate of anthropogenic greenhouse gas emissions. In direct air CO2 capture and storage (DACCS) atmospheric CO2 is captured through a series of chemical processes using liquid solvents or solid sorbents2 and subsequently liquidized. Following compression into a supercritical liquid, the CO2 can be injected into suitable intact marine sediments where storage is generally safe and permanent3. Ocean floor sedimentary basins along passive continental shelves, such as depleted or semi-depleted oil and gas fields, are the most geologically sound choice for this4. In these basins, the liquidized CO2 is injected into available pore space below an impermeable capstone. Depleted oil and gas fields make ideal sites for long-term CO2 storage as geologic data suggest these areas have good storage and trapping characteristics4,5.
Ocean thermal energy conversion (OTEC) is a form of marine renewable energy that uses the natural thermal gradient between cold deep ocean water and warm surface ocean water to power a heat engine6. It was conceived in 1881 by Jacques-Arsène D’Arsonval, who recognized the net power depended on the magnitude of the temperature difference between the warm and cold water. To maximize its potential, he proposed warm water be drawn from the surface near the equator and cold water from the same latitude but at great depths7. In 1930, D’Arsonval’s student, Georges Claude, set this idea into practice in Cuba by building the first pilot plant.
OTEC consists of pumping warm surface water from the mixed layer and using its heat to evaporate a working fluid inside a heat exchanger. The working fluid in vapour form then passes through a turbine where it expands, converting thermal energy into kinetic energy and then electrical energy by way of a generator. The working fluid then proceeds to a second heat exchanger where it is cooled by cold deep seawater, pumped in from approximately 1000 m deep, and condensed back into liquid form before restarting the cycle. After the warm and cold water have passed through their respective heat exchangers, the two are mixed and discharged at the level of neutral buoyancy. While the use of a non-seawater working fluid improves the process’ efficiency, it can also be conducted using seawater, producing freshwater as a by-product.
While initial and ongoing studies consider OTEC as a method of clean electricity generation8,9, more recently OTEC has also been suggested as a clean energy source for CO2 negative emissions technology6. OTEC generated electricity could be used to power liquid solvent based DACCS in terrestrial facilities or solid sorbent based DACCS in marine conditions. The captured CO2 could then be transported and sequestered in offshore storage sites.
The levelized cost of electricity (LCOE) of OTEC is competitive with that of coal-fired electricity production. The inflation adjusted (using the U.S. Bureau of Labor Statistics online CPI inflation calculator) LCOE of OTEC ranges from 0.04 to 0.24 USD2023/kWh10–12 prior to considering any discounts or subsidization. The 2020 LCOE of coal-generated electricity in the US is between 0.075 and 0.116 USD2020/kWh (Table 3.12 in 13) assuming a 3% discount rate, or equivalently and adjusted for inflation, between 0.09 and 0.14 USD2023/kWh.
Approximations of how much power OTEC is able to produce per year without significant environmental impact vary greatly. The discrepancy comes mainly from the large amount of uncertainty surrounding the limiting factor for reservoir renewal. Other concerns include deep water formation14, environmentally safe levels of OTEC production density15, and possible disruptions of the oceanic thermohaline circulation6,16.
Consistent with17, the sensitivity analysis we performed using the UVic Earth System Climate Model (UVic ESCM) revealed that 3 TW of OTEC electricity production a year could be sustained for at least 500 years without substantial adverse effects on the ocean circulation or its physical and chemical properties. The combination therefore of DACCS and OTEC offers an exciting new approach for independently powered carbon capture plants to inject concentrated supercritical CO2 into the deep ocean in an economically and environmentally beneficial approach.
In this report, we use the UVic ESCM to explore the feasibility of fueling negative emission technology with aqueous clean energy, in order to significantly decrease the global temperature increase that would otherwise occur.
Methodology
The UVic ESCM consists of an energy-moisture balance atmospheric model, a dynamic-thermodynamic sea-ice model18–20, and a primitive equation oceanic general circulation model21. The UVic ESCM has fully coupled representations of the oceanic and terrestrial carbon cycles and global coverage with a horizontal resolution of 3.6 degrees (zonal) by 1.8 degrees (meridional) (see ref. 22 for details). The model was initialized with a 10,000-year spin-up at the year 850. From 850 to the year 2005, historical forcing (land cover change, solar, volcanic, aerosol, CO2 and other GHGs) was used to force the model. In addition, over the period 2005 to 2100 changing CO2, land surface, aerosol and other greenhouse gas forcing followed the Intergovernmental Panel on Climate Change Representative Concentration Pathway 8.5 (IPCC RCP 8.5; 23). From 2000 to 2100, the equivalent CO2 emissions were diagnosed24 and then used in the subsequent sensitivity experiments. This allowed the model to react to the sequestration of CO2 rather than be constrained by specific concentrations.
To determine useful OTEC plant locations, the vertical temperature gradient in each viable ocean grid cell was calculated and OTEC plants were placed first in locations with the greatest temperature gradient. This is because OTEC is most efficient in areas with large temperature gradients. OTEC requires a thermal gradient of at least 18 to 20 °C between where surface water uptake occurs and where the deep-water uptake occurs17,25. If the temperature gradient fell below 18 °C or the power generated by each OTEC plant fell below 75 MW the plant in our model was “decommissioned” and relocated. Each OTEC plant was assumed to require a minimum area of 50 km2. The net power generated by each deployed OTEC plant was determined as follows (see ref. 26 for more details):
where
The calculated emission reduction was incorporated by factoring it into transient CO2 atmospheric forcing where all available OTEC-generated electricity was used to power DACCS. Two approaches were taken. First, we used estimations of energy required for DACCS from the Squamish Carbon Engineering plant, where 366 kWh of electricity and 5.6 GJ of natural gas are needed to sequester one tonne of CO2 (see ref. 27 for more details). Here we note that the Carbon Engineering plant uses a liquid solvent system and so natural gas combustion is required to create the very high temperatures needed. While we recognize technological barriers exist in creating such high temperatures from renewable energy, research and development in overcoming these barriers is advancing28. In the two experiments discussed below, we assume in one case (ODLMit — OTEC/DACCS Low Mitigation) that all energy is produced from OTEC (1921 kWh per tonne of CO2 sequestered). In the other case (ODHMit — OTEC/DACCS High Mitigation), we assume that local reserves of natural gas are available so OTEC is solely used to provide the required electricity (366 kWh per tonne of CO2 sequestered). In this case the emissions from natural gas combustion are also sequestered.
Two deep ocean CO2 storage sites were selected: (1) off the east coast of Oman in the Arabian Sea; (2) off the northern coast of Venezuela in the western equatorial Atlantic (Fig. 1). Both sites are excellent target basins for long-term CO2 storage because of their stability and structural integrity29. This is in large part due to their location on the passive edge of stable continental plates. This and their location within the suitable latitude range for OTEC is why these sites were selected. While there is a need to obtain more information on the storage capacity of these selected areas, their known large amounts of oil and gas reserves suggest that there would be the capacity to store large amounts of CO2.
In this report, three model integrations are compared. All experiments use the diagnosed emissions from the 21st century integration driven by RCP 8.5. The IPCC RCPs were used extensively in models run for the IPCC AR5 and include a time series of emissions and GHG concentrations from 2005 to 2100 with extensions to 23001. RCP 8.5 represents a business-as-usual scenario where there are high emissions without effective climate change mitigation practices. In this scenario, the radiative forcing reaches 8.5 W/m2 by 21001.
Results
To explore the climate effects of widespread OTEC deployment coupled with DACCS, we first conducted a Control experiment where the model was integrated from 2000 to 2100 using the diagnosed emissions from the RCP 8.5 spin-up (Fig. 2a). In this Control experiment the atmospheric CO2 concentration increases to 922 ppm in 2100, 553 ppm higher than in year 2000. Concomitant with the increase in greenhouse gas forcing, the global mean surface air temperature increased by 3.5 °C from 14.1 °C in year 2000 to 17.6 °C in year 2100 (Fig. 2b). In ODLMit, OTEC power production was initiated in year 2030 and grew following a raised negative cosine function until the number of plants deployed (~ 30,700 plants producing on average 98 MW each) at year 2100 met the requested power demand of 3 TW (see Fig. 1b). All OTEC power is directed towards DACCS and in year 2100, at peak OTEC production, 14 GtCO2 is being sequestered annually (Fig. 2a).
ODHMit follows the same experimental design as ODLMit with the difference being that OTEC energy is used to only power the required 366kwh of electrical energy per tonne of captured CO2. In this case, ~ 33,000 plants, each producing on average 90 MW, met the requested 3TW power demand at 2100 (see Fig. 1b). In 2100, 72 GtCO2 is being sequestered annually in ODHMit (Fig. 2a). This is nearly twice the anthropogenic CO2 emissions in year 2030 diagnosed from the RCP 8.5 spin-up (41 GtCO2) and twice present-day anthropogenic emissions of CO2 (37 GtCO2). In total, 471 GtCO2 and 2,446 GtCO2 were sequestered from 2030 to 2100 in ODLMit and ODHMit, respectively. These are well within estimates of available capacity for CO2 storage in deep saline formations and available oil and gas fields29.
In the ODHMit experiment, global CO2 emissions continue to rise from 2030 to 2050, before beginning to decline. This occurs because OTEC power production, and therefore the amount of DACCS that is powered, increases with time. By 2100, net CO2 emissions in the ODHMit experiment are reduced to only 17 GtCO2/year (Fig. 2a) and the resulting atmospheric CO2 concentration is 645 ppm (Fig. 2b). Compared to the results from Control, this represents a 278 ppm reduction in atmospheric CO2 and a 72 Gt reduction in annual anthropogenic CO2 emissions. In the case of ODLMit, where the majority of OTEC energy is used to replace the natural gas energy component in ODHMit, net CO2 emissions did not drop to the same extent. In ODLMit, CO2 emissions only reduced to 74.8 GtCO2/year and the atmospheric CO2 concentration reached 855.6 ppm at year 2100. Compared to the results from Control, this represents a 66.8 ppm reduction in atmospheric CO2 and a 13.6 Gt reduction in annual anthropogenic CO2 emissions.
The growing reduction in net 21st -century anthropogenic CO2 emissions after the deployment of OTEC and DACCS leads to a concomitant increasing reduction in atmospheric surface temperature warming (Fig. 2c) compared to the case with no CO2 sequestration. The resulting 2100 globally-averaged atmospheric surface air temperature in ODLMit (ODHMit) is 17.1 °C (16.4 ºC), a 0.5 °C (1.2 °C) reduction from Control, the experiment without any CO2 sequestration (Figs. 2c and 3). Nevertheless, global mean surface air temperatures still rose 2.3 °C in ODLMit and 1.5 °C in ODHMit more than the 2030 average (14.8 °C), although the rise is significantly lower than in Control where the increase above 2030 was 2.7 °C. This relative temperature decrease is felt across the globe but is concentrated in the areas where OTEC is operational and over the Arctic, where climate feedbacks are strongest (Fig. 3).
Discussion
Based on the potential for mitigating anthropogenic climate change suggested by our analysis, we chose to perform initial calculations estimating the economic feasibility of implementing OTEC coupled with DACCS at the suggested scale. While we recognize that such estimates are highly uncertain and far too general to be definitive, emerging literature can help guide us. Below we first explore the cost of deploying OTEC, followed by the cost of installing DACCS in association with OTEC.
The cost of OTEC
The cost to build OTEC plants varies greatly depending on the location, scale, and technology used to build these plants. At this time there is limited quantitative cost data available for OTEC, with most cost references based on feasibility studies from limited sources. Ref.10 attempted to provide an overview of the available cost projections for a range of OTEC plants, spanning 5 to 250 MW capacity, based on data from12. They found that due to the large overhead cost, small-scale OTEC plants (those capable of producing less than 10 MW power) have comparatively higher capital costs per kW than larger (10 to 100 MW) OTEC plants. They suggested that the capital cost of an OTEC plant with 100 MW capacity would range from USD2010 5,000/kW to 15,000/kW. These capital costs include plant components such as pumps, heat exchangers, and components for thermodynamic cycles which are considered predictable costs since these components are commercially available for other offshore operations. Other costs, such as labour, were estimated based on USD2010 prices. Therefore, for an OTEC plant with 90 MW capacity, the capital cost per plant would be USD2010 500 million to 1.5 billion10. Using inflation-adjusted conversion rates from the U.S. Bureau of Labor Statistics, this is equivalent to 700 million to 2.1 billion USD2023. To produce 3 TW of electricity in ODHMit using 90 MW OTEC plants, we needed 33,000 plants, whereas 30,700 plants producing on average 98 MW, were needed in ODLMit.
Using the lower and the upper bound of these estimates (500 million USD2023 and 2.1 billion USD2023, respectively), the required 33,000 OTEC plants in ODHMit would cost between 17 trillion USD2023 and 69 trillion USD2023, respectively. The 30,700 plants in ODLMit would cost between 15 trillion USD2023 and 64 trillion USD2023. These numbers do not consider the decrease in price that would occur as the OTEC plants become more standardized (economy of scale) or the possibility of attaching OTEC plants to decommissioned oil and gas platforms. Ref.10 estimated that closed-cycle OTEC plants (where ammonia with a low boiling point is used as the working fluid) are less expensive than open-cycle (where seawater is used as the working fluid) designs. However, open-cycle OTEC plants produce fresh water as a by-product whereas closed-cycle plants do not, so the economic benefits of freshwater production may make open-cycle OTEC systems more economically viable in the long term, particularly for plants located near small island nations or the coast.
Once OTEC is operational, the LCOE also depends on interest rates and subsidies. For a ~ 100 MW plant, it has been estimated that the LCOE could range from 0.09 to 0.24 USD2023/kWh10–12. Additionally11, estimated that obtaining financing from government bonds (with lower interest rates than commercial loans) could reduce the LCOE of OTEC power generation to around 0.04 USD2023/kWh for a ~ 100 MW OTEC plant. For comparison, ref.13 recently estimated the LCOE for US-based coal-powered electricity as 0.09 to 0.14 USD2023/kWh. Therefore, the LCOE of OTEC-generated electricity could be considered competitive with the LCOE of coal-generated electricity.
The cost of DACCS
One of the major factors in determining the cost of DACCS is the cost of electricity and thermal energy used to power the system. Since the energy requirement for CO2 capture and storage can be significantly larger than for other emission control systems, how DACCS is powered is an important consideration to ensure the process is both economically profitable and environmentally beneficial. Due to the number of factors influencing the cost of DACCS, there is little consensus on estimates of the technology’s cost. Cost estimates based on simple scaling relationships, yield results from ~ 50 to ~ 1,200 USD2023 per tonne CO2 sequestered27,30–34.
In April 2022 the International Energy Agency published a report28 exploring the role that direct air capture could play in assisting the world reach net zero emission targets. They noted that only 18 such plants existed at the time of publication, although governments and industry had committed billions in direct air capture technology investment in the years ahead. While the cost per tonne of CO2 removed is presently high, the IEA estimated that for a large-scale plant built in 2022, the cost would be between 125 and 335 USD per tonne CO2 captured. They further argued that by 2030, costs for DAC could fall to below $100 per ton of CO2 capture.
Carbon Engineering, based in British Columbia in Canada suggested that direct air capture on land could be achieved for 94 to 232 USD2018 per tonne (equivalent to 114 to 280 USD2023; 27). This is much lower than the previous American Physical Society estimate35 of 600 USD2011 per tonne CO2 (equivalent to 830 USD2023), suggesting, and consistent with ref.28, that the price of direct air CO2 capture is rapidly decreasing with technological advances and will continue to do so.
If we use the range of land-based direct air capture costs from the IEA report (between 125 USD2023 and 335 USD2023 per ton of CO2 captured, respectively), the cost to extract the 2,446 Gt of CO2 in ODHMit through direct air capture converts to between 305 trillion and 819 trillion USD2023. In the case of ODLMit, the cost to extract the 471 GtCO2 would be between 59 trillion and 158 trillion USD2023. Considering the decrease in price that would occur with electricity coming from OTEC rather than the electrical grid, these costs would decrease further. We recognize that the above estimates are for land-based direct air capture and that these costs could be expected to be different in the marine environment.
The technology for injecting CO2 into depleted or nearly depleted oil and gas reservoirs is mature and has been successfully used for decades for enhanced oil recovery. This method of carbon injection occurs when liquidized CO2 is injected into the oil-bearing formation to lower the viscosity of the oil, therefore allowing the oil to flow more easily to the oil well36. The 2019 cost for land-based enhanced oil recovery CO2 injection was estimated to be about 40 USD2019 per tonne of CO2 stored37,38, although the IEA report28 notes that in the US, land-based storage can be achieved for less than 10 USD while offshore storage cost below 35 USD per ton of CO2 stored. Assuming 35 USD2023 per ton of CO2 stored, the total cost to store 2,446 GtCO2 is 86 trillion USD2023 and to store 471 GtCO2 is 16 trillion USD2023.
Total cost
The capture and compression/liquefaction of CO2 are expected to be the dominant costs involved in DACCS, followed by transport costs39. With OTEC powering DACCS directly above tropical depleted to semi-depleted oil and gas fields, the cost associated with the transport of the liquified CO2 would be eliminated. We can also assume, due to the presence of pre-existing technology, that the cost of CO2 injection into marine sites is similar to that of DACCS on land and so use estimates from existing enhanced oil recovery operations. Taken together, we estimate the total cost for 33,000 90 MW OTEC plants that sequester 2,446 Gt (ODHMit) of CO2 over a 70-year period (Figs. 1b and 2a) using existing enhanced oil recovery technology ranges from 407 trillion to 973 trillion USD2023 (equivalent to between 166 and 398 USD2023 per ton of CO2 sequestered). The total cost for 30,700 98 MW OTEC plants that sequester 417 GtCO2 (ODLMit) over a 70-year period ranges from 90 trillion to 238 trillion USD2023. This is equivalent to between 215 and 570 USD2023 per ton of CO2 sequestered. Expected costs could be lower than these estimates as we took the conservative approach of not fully including cost savings associated with energy production from OTEC.
Technological feasibility
The current experimental efficiencies of OTEC systems are relatively low compared to theoretical estimates likely due to the latter not accounting for the efficiencies of external components such the generator, mechanical transmission, and inverter40. Efforts are currently underway to improve system efficiency, primarily through turbine design which is the most influential component40. Non-seawater working fluids are known to increase efficiency, especially in the case of refrigerant grade R717 ammonia which is considered to be the most effective working fluid, producing up to a six-times greater power output compared to alternatives40. Additionally, the use of solar energy to enhance the heating of the working fluid could increase net power generated by 20–25%41,42.
Onshore, offshore, and floating OTEC facilities offer distinct infrastructure options for implementation. Floating facilities have the potential to be relocated depending on the available ocean vertical temperature gradient. OTEC plants could also repurpose decommissioned marine oil and gas platforms43,44. This oil and gas industry infrastructure has undergone decades of improvement and is known to be durable under harsh marine conditions. The use of such existing infrastructure might allow for an acceleration of the implementation of OTEC while creating a transitional pathway from the reliance on fossil fuels44.
Environmental feasibility
Exploring the potential environmental consequences of widespread marine OTEC implementation is the subject of several recent studies. Modelling efforts have found ocean surface cooling in regions of OTEC implementation9,26,45, ocean surface warming at high latitudes9,26,45, and heating in the ocean interior26,45 due to OTEC-induced vertical mixing. Enhanced OTEC-induced vertical mixing also leads to an increased meridional gradient of depth-integrated steric height along the western boundary of the North Atlantic46, thereby reinforcing or even increasing the strength of the Atlantic Meridional Overturning Circulation (AMOC; 9, 26, 45). This might be viewed as a positive environmental effect of OTEC deployment as it counteracts AMOC weakening associated with increased atmospheric greenhouse gas loading. On the other hand, the optimal location for OTEC deployment is within the warm pool of the western equatorial Pacific. Net surface cooling in this area would almost certainly affect El Niño and monsoonal systems which future research might explore.
Near-surface discharge associated with OTEC also transports large volumes of deep-nutrient rich seawater into the photic zone45,47,48. Artificial upwelling in nutrient depleted waters has been found to alter the assemblage of phytoplankton communities, resulting in a greater percentage of micro-phytoplankton compared to pico-phytoplankton, while primary production rates remained low49. Nevertheless, a mitigative solution could involve increasing the density of the discharge plume so that neutrally buoyant settling of nutrient rich waters occurs well below the photic zone thereby preventing interference with natural primary productivity levels or shifts in the composition of phytoplankton communities44,48,49.
Other potential biological effects associated with OTEC implementation include entrainment or impingement of marine organisms in water intake pipes47,48, disruption of seabed communities47, and changes to marine organism foraging patterns as offshore and floating OTEC infrastructure might act as fish aggregating devices that attract marine fauna potentially creating artificial reef communities47,48,50,51. Deep ocean organisms are highly susceptible to temperature, pH, and salinity changes47. Therefore, it is important to conduct field assessments at potential OTEC facility sites to establish baselines for comparison with induced changes and improve spatial planning of cumulative environmental effects47,48.
Concluding remarks
As identified in ref.1, the goal of the Paris Accord to limit global warming to well below 2 °C above pre-industrial levels while pursuing efforts to limit the temperature increase to 1.5 °C ultimately requires the introduction and scale-up of negative emission technology. Earth has already warmed by ~ 1.1–1.2 °C since preindustrial times and if worldwide fossil fuel combustion was immediately eliminated, the direct and indirect net cooling effect of atmospheric aerosol loading would rapidly dissipate through gravitational settling and precipitation scavenging of these aerosols. As such, the source of the ~ 0.5 °C aerosol cooling realized since the preindustrial era would be eliminated, thereby taking the Earth rapidly to ~ 1.6–1.7 °C warming. The Earth would warm further as we equilibrate to the present 523 ppm CO2e52 greenhouse gas loading in the atmosphere (only 417 ppm of which is associated with CO2), and that is not including the committed warming from the permafrost carbon feedback that would add another 0.1 to 0.2 °C this century53,54.
The need to reach global net zero CO2 emissions this century to keep warming to below 2 °C above preindustrial times has long been recognized. For example ref.55, concluded that “…if a 2.0°C warming is to be avoided, direct CO2 capture from the air, together with subsequent sequestration, would eventually have to be introduced in addition to sustained 90% global carbon emissions reductions by 2050.” The recognition that future warming responds linearly to cumulative carbon dioxide emissions has also allowed for the calculation of probabilistic estimates of the remaining allowable carbon budget before exceeding either the 1.5–2 °C threshold1,56–58. Given socioeconomic inertia in the built environment, and the previous discussion, the 1.5 °C threshold will almost certainly be passed within the next few decades and even the 2 °C threshold cannot be avoided without an immediate decarbonization of energy systems and widespread deployment of negative emissions technology.
Finally, despite uncertainties in the size of the geological reservoirs available for deep ocean CO2 storage, our results are encouraging. The combination of OTEC and DACCS could serve as an important component of any global climate change mitigation strategy. While nature-based solutions have received a lot of attention of late (forestry, land management, blue carbon etc.), such solutions are incapable of recapturing the fossil carbon that took tens of millions of years to be created (and only a few decades to combust). Cumulative anthropogenic fossil carbon dioxide emissions from 1750 to 2021 have been 1738 GtCO2, while deforestation and land use changes have contributed another 744 GtCO259. Nature-based solutions are certainly capable of addressing historical cumulative land-use carbon dioxide emissions, but they are insufficient to respond to the growing atmospheric loading of fossil carbon60. Given the urgency of implementing negative emission solutions, if we wish to keep global warming to a reasonable level, it may be time to consider the installation of a pilot OTEC/DACCS system in the western equatorial Indian or Atlantic Oceans. Regardless of whether OTEC/DACCS emerges as a viable global mitigation strategy, the scale of the geological sequestration required to mitigate past and future emissions suggests we are a very long way from reaching mid-century net zero emissions.
Author contributions
A.W., S.O, A.N, L.M., M.E. worked collaboratively on all aspects of this manuscript from experimental design, through data analysis to writing and reviewing the manuscript.
Data availability
The datasets used and/or analysed during the current study are available from the corresponding author upon request.
Declarations
Competing interests
The authors declare no competing interests.
Footnotes
Publisher’s note
Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
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Associated Data
This section collects any data citations, data availability statements, or supplementary materials included in this article.
Data Availability Statement
The datasets used and/or analysed during the current study are available from the corresponding author upon request.