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Scientific Reports logoLink to Scientific Reports
. 2026 Jul 23;16:23094. doi: 10.1038/s41598-026-62846-z

Numerical investigation of liquid-Cooled battery thermal management system configurations for a lithium-ion battery pack with experimental validation

Abdelrahman O Ali 1, Osama Abdelrehim 1, Mahmoud M Saafan 2,, Mohamed R Elmarghany 1, Ahmed M Hamed 1
PMCID: PMC13396402  PMID: 42493524

Abstract

Efficient thermal management is crucial for lithium-ion battery safety and longevity in Electric Vehicles (EVs). This study presents a numerical investigation and experimental validation of liquid cooling strategies for NMC lithium-ion battery modules, comparing serpentine (Configuration 1), parallel (Configuration 2), and parallel/counter-flow hybrid (Configuration 3) layouts. A custom-built 4-cell test rig validated against CFD simulations showed close agreement, with relative deviations below 0.6%, confirming model reliability. Under regulated flow conditions, clear differences in thermal and hydraulic behavior were observed. Configuration 1 exhibited the highest thermal stress, with peak temperatures reaching 75.7 Inline graphic (cell 7) and 74.1Inline graphic (cell 18) due to downstream heat accumulation and limited contact area, alongside the largest temperature difference (ΔT = 11.0 K) and highest pressure drop (27.3 Pa). Configuration 2 reduced peak pack temperature to 70.6 Inline graphic at cell 18 (6.7% lower vs. Configuration 1) and 64.7 Inline graphic at cell 7 (14.8% lower), achieving the best intra-cell uniformity (σ = 0.47 K, CV = 5.6%) and lowest pressure drop (9.1 Pa). Configuration 3 offered the most balanced cooling, lowering maximum cell temperature by 7.6% compared to Configuration 1 and 0.9% compared to Configuration 2, while the maximum temperature of cell 18 decreased by 11.8%. It achieved the narrowest inter-cell ΔT (4.1 K), a 62.5% and 11% reduction versus Configurations 1 and 2, respectively, with the lowest σ = 1.0 K (CV = 0.32%). Overall, serpentine cooling is simple but thermally inefficient, parallel flow is the most energy-efficient, and the hybrid parallel/counter-flow design delivers the best overall thermal balance while lowering the required pumping power by about 89%, making it the most suitable layout for safe and reliable EV battery operation.

Keywords: Battery Thermal Management System (BTMS), Liquid Cooling, Lithium-Ion Battery, Conjugate Heat Transfer, Sony VTC6

Subject terms: Energy science and technology, Engineering

Introduction

Rapid electrification in the automotive sector and consumer electronics has increased the demand for high-performance lithium-ion (Li-ion) batteries. Thermal stability is crucial for safety, efficiency, and lifespan1. High C-rates, ambient temperature fluctuations, and prolonged cycling impose high thermal loads2, where the C-rate denotes the charge or discharge current relative to the battery’s nominal capacity. Inadequate thermal management causes non-uniform temperature distribution, which accelerates aging, degrades performance, and can trigger thermal runaway3. High temperatures accelerate electrolyte decomposition and electrode degradation4. Low temperatures reduce ion mobility and depress power output5. Because these electrical, thermal, and aging mechanisms are strongly coupled, recent work stresses joint electro-thermal–aging state estimation to capture their interaction in operating packs6, while exergy-based analyses that explicitly account for lithium plating quantify the efficiency and safety penalties incurred when cells operate outside this window7. Thus, effective thermal management ensures that batteries operate within an optimal temperature range, typically between 15 Inline graphic and 40 Inline graphic8,9.

Battery thermal management strategies fall into passive and active cooling techniques. Passive methods include Phase Change Materials (PCMs) and natural convection, offering simplicity but provide limited thermal performance10. Active cooling, including air and liquid systems, provides higher heat dissipation and better temperature uniformity, though it requires auxiliary power and added controls11,12. Figure 1 compares different cooling strategies on cooling effectiveness, design complexity, cost, thermal uniformity, weight impact, noise, high loads performance, and manufacturer adoption. Liquid cooling stands out for stable performance under high-load and fast-charging conditions and for compatibility with compact battery pack designs. It balances performance and scalability, making it adopted by many modern Electric Vehicle (EV) platforms. This comparison helps select thermal solutions tailored to specific EV design and operational requirements. Comprehensive reviews of energy-efficient liquid cooling for high-energy-density Li-ion batteries reinforce this direction, consolidating both heat-extraction and thermal-runaway-suppression strategies across cell formats13. At the vehicle level, system-level modelling further situates the thermal subsystem within the broader energy architecture, including emerging dual-energy-storage powertrains14.

Fig. 1.

Fig. 1

Battery Cooling Strategies in EVs Comparison19.

Liquid cooling, which is classified into direct and indirect cooling techniques, delivers high thermal performance due to the high heat capacity and density of different used coolants. Direct cooling, such as immersion cooling submerges cells in a dielectric (non-conductive) fluid, enabling direct contact convection and low thermal interface resistance15. It reduces temperature gradients, suppress hotspots, and can improve performance and lifespan16. A Channeled Dielectric Fluid Immersion Cooling (C-DFIC) system for high-energy Lithium Titanate Oxide (LTO) cells is presented in17, reduced maximum temperature by 17.8% and improved temperature uniformity by 33.3% versus a conventional design. With HFE-6120 at 0.5 L/min, aged cell temperature stayed below 26.1Inline graphic (299.2 Inline graphic) after 3972 US06 drive cycle repeats. However, immersion cooling also presents several challenges, such as system complexity, leak-tight enclosure, added fluid weight, and fluid-material compatibility. High fluid cost and maintenance still limit adoption in EVs18.

Indirect liquid cooling, using cold plates with serpentine channels, is widely used in Li-ion EV packs because it balances cooling performance, design flexibility, and safety. Coolant circulates through channels adjacent to cells, removing heat without electrical contact20. Key advantages include high heat removal, compatibility with modular packs, and tighter temperature uniformity than air or PCM cooling21. However, it adds system complexity, weight, cost, and seal maintenance. Despite these trade-offs, EV manufacturers favor it for reliability, scalability, and robust control under high load and fast charge conditions22. Recent numerical channel-design studies continue to refine coolant distribution and temperature uniformity in cold plates; a diamond-shaped flow-channel architecture, for instance, has been proposed to homogenize flow and lower cell temperature gradients23. Complementing geometry-focused work, coupled loss and finite-element thermal models of production fast-charging modules resolve heat generation and temperature fields under aggressive charging, linking cell-level losses to module-scale thermal response24. Beyond physics-based Computational Fluid Dynamics (CFD) and Finite Element Analysis (FEA), data-driven and digital methods are increasingly deployed for real-time thermal awareness: optimized random-forest models estimate cell surface temperature for closed-loop BTMS control25, and digital-twin frameworks fuse sensing with simulation to track battery-system states across their life26.

Indirect liquid cooling employs several architectures including cooling tubes, jackets, helical coils, serpentine channels, and hybrid designs. Table 1 summarizes recent studies on channel design for cylindrical Li-ion cells, covering Configurations, techniques, and thermal performance from experiments and simulations274041. Vertical tube layouts (e.g., for Li-ion iron phosphate) improve temperature uniformity and thermal stability versus horizontal arrangements but raise mechanical complexity and packing constraints. Cooling jackets deliver strong uniformity with multi-directional flow35. Serial/parallel arrangements also affect performance. Parallel Configurations lower thermal resistance and suppress hotspots31. Innovative designs such as bionic hexagonal channels, double helical coils, and external PCM composites further reduce temperature gradients40. Serpentine channels deliver cooling performance comparable to U-shaped layouts but with lower pressure drop, improving thermal-hydraulic tradeoffs in EV modules28,33. Counterflow routing, where adjacent paths carry coolant in opposite directions, further reduces through module temperature gradients. Hybrid designs that combine parallel and counter-flow remain understudied in 6s4p-type packs, representing a gap this study addresses.

Table 1.

Indirect liquid cooling designs and Configurations.

S.N. Cooling System Type Type of Battery Cooling Technique Used Design of BTMS (Cooling Plate/Channel Geometry) Type of Study Significant Remarks Refs.
1 Indirect Liquid Cooling 18,650 Cylindrical Li-ion Single-phase forced convection (Water/Glycol) Stepped-channel liquid-cooled BTMS. Investigated channel width, cell-to-cell lateral spacing, contact height, and angle. Numerical Simulation Optimized design significantly reduced weight (54.08%) while maintaining acceptable temperature control (Tmax increase by only 2.52 Inline graphic). Channel width was identified as the most critical parameter. 27
2 Indirect Liquid Cooling 18,650 Cylindrical Li-ion Single-phase forced convection (Water/Glycol) Converging-diverging liquid cooling channel with wave-shaped structure (based on serpentine/U-shaped). Four geometrical Configurations analyzed. Numerical Simulation Optimized design reduced peak internal temperature by 20.6% compared to other designs. Identified importance of Reynolds number, arc depth, and cell spacing. Optimal for 2 C discharge. 28
3 Indirect Liquid Cooling 18,650 Cylindrical Li-ion Single-phase forced convection (Water, Nanofluids) Mini-channel fins heat sink units are integrated into cooling channels. Four models with different fin Configurations (e.g., Model II with lowest max temp). Numerical Analysis & Experimental Testing Demonstrated significant thermal cooling enhancement. For Model II, Tmax was 30.10Inline graphic and temperature gradient was 1.48Inline graphic, exploring various heat transfer enhancement approaches. 34
4 Indirect Liquid Cooling 18,650 Cylindrical Li-ion Single-phase forced convection Gradient contact surface angle in cooling jacket for 18,650 cells. Numerical Simulation Achieved good cooling performance with a temperature gradient of 2.58 Inline graphic at 2 C discharge for a 15° contact surface angle. 35
5 Indirect Liquid Cooling 18,650 Cylindrical Li-ion Single-phase forced convection Liquid-cooled cold plate with Gradually Varied Circular Notched Fins (GV-CNF). Numerical Simulation (CFD) GV-CNF design showed 41.1% improvement in comprehensive performance (temperature uniformity, max temp, pressure drop) over traditional circular fins. Optimal channel height identified. 36
6 Indirect Liquid Cooling 18,650 Cylindrical Li-ion Single-phase forced convection Optimizing two inlets/outputs, channel widths, and flow orientations in a liquid cooling BTMS. Numerical Simulation This type of study focuses on flow distribution and channel Configurations to improve overall cooling, particularly for 18,650 packs. Results show improved temperature uniformity and reduce maximum temperatures by adjusting these parameters. 37
7 Indirect Liquid Cooling 18,650 Cylindrical Li-ion Single-phase forced convection Serpentine channel with redesigned baffles on the inner surface. Numerical Simulation Significant improvement in temperature uniformity and heat transfer between cells and coolant due to enhanced mixing flow in the channel. 38
8 Indirect Liquid Cooling 18,650 Cylindrical Li-ion Single-phase forced convection Wavy cooling channel liquid-cooled system. Numerical Simulation At 5 C discharge, this design reduced the highest temperature by 12.80 Inline graphic and temperature gradient by 5.30 Inline graphic. 39
9 Indirect Liquid Cooling 18,650 Cylindrical Li-ion Single-phase forced convection Helical vs. Linear channel designs in a cold plate. Numerical Simulation (CFD) Linear Channel Design (LCD) proved superior in both maximum temperature reduction and thermal uniformity (1.796 Inline graphic lower Tmax, 8.740 Inline graphic lower ΔT) compared to Helical Channel Design (HCD). 40
10 Indirect Liquid Cooling 18,650 Cylindrical Li-ion Single-phase forced convection Liquid-cooled plate with variable density topology optimization for channel design. Numerical Simulation Reduced maximum battery module temperature by 2.4% (from 27.88Inline graphic to 27.21 Inline graphic) and temperature difference by 13.2% (from 5.7 Inline graphic to 4.95 Inline graphic), meeting performance requirements. 30
11 Indirect Liquid Cooling 18,650 Cylindrical Li-ion Single-phase forced convection (Water) Microchannel-embedded cylinder cooling system. Numerical Simulation Optimized design kept the maximum temperature at 27.80 Inline graphic with a temperature gradient of 0.80 Inline graphic for discharge rates of 1 C, 1.5 C, and 2 C. 41
12 Direct Liquid Cooling (Immersion) 18,650 Cylindrical Li-ion Dielectric fluid immersion No complex channels; cells directly immersed in SF33-based liquid. Numerical Simulation & Experimental Validation Effectively mitigates heat accumulation and provides notable advantages in temperature control and equalization, with greatly reduced cooling energy consumption compared to forced air cooling. 29
13 Liquid 18,650 cylindrical Serial & parallel tubing Serial-parallel channels Simulation + Experimental Parallel system outperforms serial; glycol solution better than water 31
14 Liquid 18,650-type cylindrical Wavy multi-channel tubes Multi-channel embedded pipes Simulation + Experimental Wavy design increases heat exchange even at high discharge 32
15 Liquid 18,650-type cylindrical Serpentine/U-shaped channels Flow optimization channels Simulation U-shaped channels reduce pressure loss; same thermal effect as serpentine 33 33
16 Indirect Liquid Cooling 18,650 (Sony VTC6), 6s4p pack Single-phase forced convection (water) Serpentine vs. parallel vs. hybrid parallel–counter-flow, normalized flow Numerical Simulation & Experimental Validation Hybrid gives narrowest ΔT (4.1 K); 62.5%/11% lower than serpentine/parallel; validated at 3 C Present study

Despite these advances, the studies summarized in Table 1 share three limitations that constrain their relevance to real EV modules: (i) they predominantly examine simplified cell arrays or single-layer modules rather than electrically realistic series–parallel packs; (ii) most validate cooling only up to moderate discharge rates (≤ 2 C), leaving high-load behavior unverified; and (iii) they typically optimize a single channel geometry rather than benchmarking competing topologies under an identical flow budget. Hybrid layouts combining parallel and counter-flow routing, in particular, remain largely unexplored for compact, high-power Configurations such as 6s4p cylindrical packs.

The present work addresses these gaps by experimentally validating a CFD model against a custom 4-cell rig (steady-state error within ± 1.6 K, relative deviation below 0.6%) and then benchmarking three topologies — single serpentine (Config. 1), three parallel channels (Config. 2), and a hybrid two-parallel/one-counter-flow design (Config. 3) — in a realistic 6s4p Sony VTC6 pack under a normalized total flow rate and discharge rates up to 5 C. The main contributions are: (1) a like-for-like, flow-normalized comparison of serpentine, parallel, and hybrid counter-flow cooling at module level, in which maximum cell temperature, inter- and intra-cell uniformity, and channel pressure drop are all reported; (2) experimental validation of both the numerical model and the serpentine-manufactured cooling channel, confirming that the fabricated geometry reproduces the idealized design intent; (3) quantitative evaluation of the hybrid design’s thermal and hydraulic advantage under high load (up to 5 C), where it attains the narrowest inter-cell temperature difference (ΔT = 4.1 K — 62.5% and 11% lower than the serpentine and parallel layouts), while the parallel and hybrid layouts cut pumping power by ~ 89% at matched flow, giving a thermal-hydraulic efficiency nearly an order of magnitude higher; and (4) a practical design recommendation showing that the parallel layout already captures most of the benefit at lower complexity, with diminishing returns beyond moderate flow rates.

Fig. 2.

Fig. 2

Schematic illustration of three liquid cooling channel Configurations for cylindrical Li-ion battery packs (a) Configuration 1, (b) Configuration 2, (c) Configuration 3.

Fig. 3.

Fig. 3

Dimensions of the cylindrical Li-ion battery pack.

The remainder of the paper is as follows: Sect. 2 describes the system design and simulation setup; Sect. 3 outlines the governing equations and modeling approach; Sect. 4 details the simulation tools and experimental validation procedures; Sect. 5 discusses the simulation results; Sect. 6 concludes the paper with key findings and future research directions.

Battery thermal management design

The system models three battery thermal management Configurations (serpentine, parallel, and a hybrid counter-flow) within a realistic 6s4p battery pack. Figure 2 illustrates the liquid cooling channel layout. In Configuration 1 (Fig. 2a), a single serpentine tube traverses the entire battery pack, directing coolant sequentially across all 24 cells. The serpentine tube layout follows the approach described in42, originally used in Tesla battery systems43. Configuration 2 (Fig. 2b) employs three parallel tubes placed between cell rows; the flow splits and runs simultaneously in each branch. Configuration 3 (Fig. 2c) employs two parallel tubes with one counter-flow tube to create bidirectional routing. All cooling channels are made of aluminum with 0.5 Inline graphic wall thickness and an internal cross section of 50 Inline graphic × 4 Inline graphic as shown in Fig. 3. This compact geometry maintains stiffness and limits system weight while providing adequate coolant flow area. A 1.5 Inline graphic Thermal Interface Material (TIM) layer is placed between each cooling tube and the cylindrical cell surfaces to enhance the contact and reduce interfacial resistance.

This modular aluminum-tube-based approach ensures scalable integration into EV packs with minimal added weight and high structural compatibility with existing 18,650 cylindrical cell arrays. Its low-profile height and selective thickness ensure efficient space usage, a critical consideration for EV architecture. The design’s feasibility is further supported by Computational Fluid Dynamics (CFD) simulations validating its performance across multiple flow and heat generation scenarios.

The thermal management system used a 6s4p Li-ion pack built from Sony VTC6 cells which are widely used in high-performance applications due to their high capacity and good discharge characteristics. The Sony VTC6 is a high-drain 18,650 cell employing a nickel–manganese–cobalt oxide (NMC) cathode, a graphite anode, and a lithium-salt (LiPF₆) organic carbonate electrolyte. The complete cell- and pack-level technical specifications are summarized in Table 2. The 24 cells are assembled in a 6-series × 4-parallel (6s4p) configuration, providing a nominal pack voltage of 21.6 V and a capacity of 12 Ah.

Table 2.

Technical specifications of the Sony VTC6 18,650 cell and the assembled 6s4p pack.

Parameter Specification
Cell chemistry
Cathode material Nickel–manganese–cobalt oxide (NMC)
Anode material Graphite
Electrolyte LiPF₆-based organic carbonate
Cell electrical ratings
Nominal voltage 3.6 V
Rated capacity 3000 mAh
Max. continuous discharge current 15 A
Nominal energy ≈ 10.8 Wh
Cell physical properties
Diameter 18.4 mm
Length 65 mm
Mass 46.6 g
Pack-level ratings (6s4p, 24 cells)
Configuration 6 series × 4 parallel
Nominal voltage 21.6 V
Capacity 12 Ah

Material properties

In the thermal simulation of the battery cooling system, each material plays a critical role in determining heat transfer efficiency and overall thermal stability. The Sony VTC6 Li-ion cell is modeled as a low thermal conductivity solid, emphasizing the importance of effective heat extraction. TIM, placed between the battery surface and cooling components, reduces contact resistance, and improves heat spreading between cells and the cooling channels. The channels are made of aluminum — chosen for its high conductivity, low density, and manufacturability — providing a rapid path from TIM to the coolant. Water serves as the coolant because of its high specific heat capacity, which allows it to absorb significant amounts of heat with minimal temperature rise. Together, these materials create a continuous thermal pathway from the cell core to the heat sink. Table 3 summarizes the thermal properties, thermal conductivity, specific heat, and density, of each material used in the model.

Table 3.

Thermal properties of materials used in the battery cooling system.

Material Thermal Conductivity Inline graphic Specific Heat Inline graphic Density Inline graphic
Sony VTC6 Battery Cell44[,45 3.0 880 2871.8
Thermal Interface Material (TIM)46 2.0 1000 2500
Aluminum (Cooling Channel)47 202.4 871 2719
Water (Coolant)47 0.6 4182 998.2

Governing equations and thermal modeling approach

The governing equations and thermal modeling approach presented in this section provide a foundational framework for simulating heat generation, transfer, and dissipation within the battery pack, enabling accurate prediction of thermal behavior under various operating conditions.

Fluid flow equations

The coolant flow inside the tubes was assumed laminar, given the low Reynolds numbers calculated for the flow rates considered. Thus, the steady, incompressible continuity and momentum equations govern the flow47,48:

Continuity equation:

graphic file with name d33e1524.gif 1

Momentum conservation:

graphic file with name d33e1530.gif 2

Where: Inline graphic, Inline graphic, Inline graphic, and Inline graphic are the pressure (Inline graphic), dynamic viscosity (Inline graphic), velocity vector (m/s), and density (kg/m3).

Energy conservation

The thermal behavior of the battery pack was modeled using the energy conservation equation, accounting for internal heat generation within the battery cells and heat conduction through solid materials and through the cooling water47,49:

graphic file with name d33e1574.gif 3

Where Inline graphic, Inline graphic, Inline graphic, and Inline graphic are the specific heat (Inline graphic), temperature (Inline graphic), thermal conductivity (W/m.K), and volumetric heat generation rate (Inline graphic).

Heat generation in battery cells

The internal heat generation rate inside each cell Inline graphic was calculated using a simplified Bernardi equation50:

graphic file with name d33e1621.gif 4

Where V, I, Inline graphic, and Inline graphic are the cell volume (Inline graphic), discharge current (Inline graphic), internal resistance (Inline graphic, and entropic heat coefficient (Inline graphic). For the battery used here (Sony VTC6), a typical value of Inline graphic is Inline graphic51. Internal resistance values were assumed based on manufacturer data and experimental measurements of the battery, with an average value of Inline graphic.

Thermal uniformity metrics

Battery thermal analysis distinguishes between inter-cell thermal uniformity and intra-cell thermal uniformity. Inter-cell thermal uniformity assesses the temperature consistency among all cells in the pack and is quantified using statistical metrics such as the standard deviation and coefficient of variation of the average cell temperatures. This metric is crucial for evaluating pack-level balance, preventing uneven aging, and supporting State-of-Charge (SOC) and State-of-Health (SOH) equalization strategies in BMS. If Inline graphic is the temperature of the Inline graphic cell at a given time, then the mean temperature Inline graphic, standard deviation Inline graphic, and coefficient of variation (CV) can be calculated as shown in Eqs. 5752. Note that a lower Inline graphic indicates better uniformity.

graphic file with name d33e1701.gif 5
graphic file with name d33e1705.gif 6
graphic file with name d33e1709.gif 7

On the other hand, intra-cell thermal uniformity evaluates the temperature gradient within each individual cell, typically expressed as:

graphic file with name d33e1715.gif 8

where Inline graphic and Inline graphic are the maximum and minimum temperatures observed on cell Inline graphic. This metric reflects internal thermal stress that drives material degradation, electrochemical imbalances, and thermal runaway risk. Ensuring high intra-cell uniformity is especially important for safe operation and long-term cell integrity. Both types of uniformity must be analyzed together for a comprehensive evaluation of thermal performance in battery packs, especially under high C-rate or fast-charging conditions.

Simulation tools and boundary conditions

All simulations used ANSYS Fluent 2023 R1, a commercial CFD solver. The solver was used to solve the conjugate heat transfer by coupling the solid and fluid energy equations. This setup is appropriate for battery thermal modeling.

Solver settings

ANSYS Fluent settings were selected to capture the pack’s thermal and flow behavior. A pressure-based solver was employed due to the incompressible nature of the coolant. The simulation is conducted in a steady state mode. The flow regime was characterized using the Reynolds number based on the channel hydraulic diameter, Inline graphic, with Inline graphic. For the Inline graphic mm cross-section, Inline graphic. Using water properties Inline graphic), the Reynolds number ranges from Inline graphic at Inline graphic to Inline graphic 370 at Inline graphic (Inline graphic at the Inline graphic reference). These values are well below the laminar-turbulent transition (Inline graphic), confirming that the laminar flow model adopted in the simulations is appropriate across the entire operating range. The Second-Order Upwind scheme was used for spatial discretization to enhance accuracy in capturing thermal and velocity gradients. Pressure-velocity coupling was handled using the SIMPLE algorithm. A convergence criterion of 10⁻¹⁰ was set for residuals to ensure solution stability and numerical reliability throughout the simulation.

Boundary conditions

To accurately assess the thermal behavior of the battery pack under various operating conditions, the simulation incorporated realistic boundary conditions as outlined in Tables 4 and 5. The ambient temperature and coolant inlet temperature were both set at 25Inline graphic. Uniform inlet velocities varied between 0.001 Inline graphic and 0.05 Inline graphic, corresponding to flow rates ranging from 0.009 to 0.45 Inline graphic for Configurations 2 and 3. To maintain the same total mass flow rate in Configuration 1, the inlet velocity was set three times higher (i.e., 0.003–0.05 Inline graphic or 0.027–0.45 Inline graphic). The cell heat generation rates were determined using the simplified Bernardi model50, incorporating both electrochemical and resistive components, and varied with discharge rates from 1 C to 5 C. A convective heat transfer coefficient of 5 Inline graphic was used for natural heat loss to ambient air. These values ensure realistic simulation conditions that reflect typical EV battery operation under various C-rates and thermal loads. The solid and fluid domains were thermally coupled through conjugate heat transfer, allowing heat conduction in solids and convective heat transfer in fluids to be modeled simultaneously. Boundary conditions at the solid-fluid interface ensured continuity of temperature and heat flux:

graphic file with name d33e1834.gif 9

Table 4.

Heat generation at different discharge rates based on the Bernardi model.

Discharge Rate (C-rate) 1 2 3 4 5
Battery Current (A) 3 6 9 12 15
Heat Generation Rate Q. Inline graphic 12,082 46,381 103,547 183,579 286,477

Table 5.

Boundary conditions used in thermal simulation.

Parameter Value
Ambient Temperature Inline graphic Inline graphic
Inlet Coolant Temperature Inline graphic Inline graphic
Inlet Velocity (Configurations 2 & 3) Inline graphic
Inlet Velocity (Configuration 1) Inline graphic
Convective Heat Transfer Coefficient of Air Inline graphic Inline graphic

Where subscripts Inline graphic and Inline graphic denote solid and fluid properties, respectively, and Inline graphic represents the normal direction to the interface.

Mesh generation and independence test

The mesh was generated in ANSYS Meshing using a combination of structured hexahedral and unstructured tetrahedral elements. A global element size of 1 Inline graphic was applied, with local refinement around the serpentine cooling channel to capture fluid–solid interactions and accurately resolve the thermal and velocity boundary layers. Cylindrical cells were discretized with a predominantly structured hexahedral mesh to improve accuracy and reduce skewness, while the curved cooling channel and complex contact regions were meshed with unstructured tetrahedral elements for flexibility as shown in Fig. 4. The inflation-layer growth rate was 1.2. Each Configuration contained approximately 1.5 million elements. To verify mesh quality and balance computational efficiency, a mesh independence study was performed for Battery 1 in Configuration 1 under a 5 C discharge rate and a flow velocity of 0.024 Inline graphic. As illustrated in Fig. 5, increasing the element count from 200,000 to 1,464,174 resulted in a consistent decline in the maximum battery temperature. For meshes above 1,000,000 elements, the change in cell temperature was less than 1%, with a final relative error of approximately 0.03%. Therefore, the mesh containing 1,464,174 elements with an average size of 1 mm was selected for all subsequent simulations to ensure both accuracy and computational feasibility.

Fig. 4.

Fig. 4

Mesh of the 6s4p cylindrical Li-ion battery module with integrated serpentine liquid-cooling channel, generated in ANSYS Meshing using structured hexahedral elements for the cells and unstructured tetrahedral elements with inflation layers near the fluid–solid interfaces.

Fig. 5.

Fig. 5

Variation of maximum battery temperature and error with different mesh element counts.

Model validation

The experimental system, shown in Figs. 6, 7 and 8, was designed to simulate liquid cooling of Li-ion batteries using a serpentine flow channel. Instead of actual battery cells, four miniature ceramic thermal heaters (rated 10 Inline graphic each) were used to emulate the heat generation of 18,650-type cylindrical cells under operation; the supplied power was set so that the emulated volumetric heat load matched the 3 C cell heat-generation rate of 103,547 Inline graphic used in the simulations. Each heater is individually instrumented with a Negative Temperature Coefficient (NTC) thermistor ([10 Inline graphic, B = 3950 Inline graphic, ± 0.2 Inline graphic]) placed at its geometric center to measure the surface temperature. A transparent water tank (6000 Inline graphic) serves as the coolant reservoir. Water is circulated from the tank through the serpentine tube using a small DC pump (6 Inline graphic, up to 2 Inline graphic). The serpentine tube, made of aluminum with a 50 × 4 Inline graphic internal cross-section and 0.5 Inline graphic wall thickness, clamped between two rigid plates (Fig. 7), ensures a controlled flow path for effective heat exchange, with a 1.5 mm TIM layer at the heater–tube interface. The coolant exits the serpentine channel and returns to the water tank, establishing a closed-loop flow. A photograph of the fully assembled rig is shown in Fig. 8, providing a direct physical counterpart to the schematic in Fig. 7. An ESP32 microcontroller (ESP32-WROOM-32, 12-bit ADC) was used for system control and data acquisition as shown in Fig. 8. It regulates the coolant flow rate via a flow sensor (YF-S402, range 0.1–3.0 Inline graphic, accuracy ± 5%) and the pump’s control signal, maintaining the target 0.27 L/min, while also recording temperature measurements from the four NTC sensors. The power supply unit provides the necessary voltage and current for both thermal heaters and the control electronics.

Fig. 6.

Fig. 6

Experimental system Configuration for power delivery and control.

Fig. 7.

Fig. 7

Schematic layout of key components in the experimental system.

Fig. 8.

Fig. 8

The actual experimental setup for simulating liquid cooling of Li-ion batteries using a serpentine tube (Configuration 2).

The schematic in Fig. 6 illustrates the system Configuration, divided into three functional blocks:

  • Power & Control – comprising the power supply and ESP32 microcontroller.

  • Thermal Simulation – consisting of the small pump, four thermal heaters, four NTC temperature sensors, and the serpentine tube heat exchanger.

  • Instrumentation – including the water tank, flow regulation components, and a PC/laptop for real-time data logging.

This setup enables controlled investigation of coolant flow rate, temperature distribution, and heat dissipation performance in a serpentine cooling channel, providing a safe and repeatable method for evaluating liquid cooling strategies for Li-ion battery packs.

Under 3 C discharge conditions (I = 9 Inline graphic), the thermal response of the battery pack subsection (four-cell module) was experimentally evaluated with and without serpentine liquid cooling at a flow rate of 0.27 Inline graphic. In the absence of active cooling, as shown in Fig. 9, the maximum cell temperature reached 355.44 Inline graphic (82.3 Inline graphic) with an average of 352.5 Inline graphic (79.3 Inline graphic) across all sensors, clearly exceeding the safe operating threshold of 333.15 Inline graphic (60 Inline graphic). By contrast, in Fig. 10, serpentine cooling limited the maximum temperature to 312.46 Inline graphic (39.3 Inline graphic) and the average to 310.9 Inline graphic (37.7 Inline graphic), corresponding to a reduction of approximately 42.98 Inline graphic (42.98 Inline graphic, 52.2%) at the peak cell and 41.6 Inline graphic (41.6 Inline graphic, 52.5%) in the average temperature. Furthermore, thermal non-uniformity across the cells was reduced from a 4.2 Inline graphic (4.2 Inline graphic) spread in the uncooled case to 3.6 Inline graphic (3.6 Inline graphic) with cooling, reflecting a 14% improvement in temperature homogeneity. Transient analysis within a 10-minute window (13:00–13:10) revealed that the heating rate decreased from 1.87 Inline graphic (1.87 Inline graphic) without cooling to 0.85 Inline graphic (0.85 Inline graphic) with cooling, representing a 55% reduction in thermal accumulation. These findings demonstrate that serpentine cooling not only prevents excessive temperature rise but also enhances spatial uniformity and mitigates thermal stress, thereby supporting safer operation and improved cycle life of Li-ion cells under high discharge rates.

Fig. 9.

Fig. 9

Temperature maximum distribution for experimental setup (Configuration 2) at no cooling case.

Fig. 10.

Fig. 10

Temperature maximum distribution for experimental setup (Configuration 2) at flow = 0.27 Inline graphic.

The ANSYS thermal model was validated against a 4-cell experimental rig using the same serpentine cooling geometry. The CFD model was validated against experimental measurements obtained under a 3 C discharge rate (I = 9 Inline graphic), with heat generation and coolant conditions set identical to the simulation case (Q. = 103547 Inline graphic, velocity = 0.03 Inline graphic, flow rate = 0.27 Inline graphic). Temperature evolution was recorded at four sensor positions (T1–T4) over 35 time steps, and the steady-state temperature was defined as the average of the final five readings for each sensor.

Steady-state temperatures (average of the last five experimental readings) agree well with the CFD predictions: the absolute errors range from − 1.57 Inline graphic (− 1.57 Inline graphic) to + 1.54 Inline graphic (+ 1.54 Inline graphic), corresponding to relative errors of −0.51% to + 0.50%. These differences are small and lie within accepted thermal-validation tolerances (≤ 5% and ≤ 2–5 Inline graphic or ≤ 2–5 Inline graphic for battery thermal studies). Residuals are attributed primarily to minor flow maldistribution and local contact-resistance differences; after accounting for these effects, the CFD model reliably predicts local cell temperatures for the studied geometry and operating point.

The 4-cell sub-module was selected as the validation unit because it isolates the governing physics common to the full 6s4p pack while remaining experimentally manageable. The repeating thermal-hydraulic unit of the pack — coolant flow through the serpentine channel, conjugate heat transfer across the channel wall, boundary-layer development, and the contact resistance introduced by TIM — is fully represented at the 4-cell scale. Capturing these localized fluid–solid interactions accurately is the prerequisite for trustworthy pack-level prediction, since pack behavior is an aggregation of these same unit-cell phenomena rather than a fundamentally different regime. A further purpose of the rig was to validate the serpentine-manufactured channel against the idealized CFD geometry: machining and assembly tolerances in the serpentine tube and clamping plates can introduce flow maldistribution and contact-resistance variations not present in the CAD model, and agreement between measured and predicted temperatures confirms that the manufactured channel reproduces the intended thermal-hydraulic behavior. The close steady-state agreement (relative errors of − 0.51% to + 0.50%) therefore confirms both the fidelity of the numerical model and the manufacturing quality of the cooling channel. Therefore, the subsection CFD model is validated and can be used with confidence for local thermal performance assessment.

Table 6 provides a numerical comparison of these experimental steady-state values with the ANSYS-predicted maximum cell temperatures, showing accepted agreement confirming the reliability of the local temperature predictions. Additional full time-series goodness-of-fit analysis yielded RMSE values of [4.89, 4.17, 3.58, 3.61] K ([4.89, 4.17, 3.58, 3.61] Inline graphic) and MAE values of [3.83, 2.78, 2.01, 2.22] K ([3.83, 2.78, 2.01, 2.22] Inline graphic) for T1–T4, respectively. The larger RMSE/MAE values result from transient discrepancies during the warm-up phase, since ANSYS provides a single steady-state maximum value while the experimental data captures instantaneous temperature fluctuations. Overall, the close steady-state match demonstrates that the CFD framework can accurately reproduce the thermal response of the battery module under realistic operating conditions.

Table 6.

Numerical experimental comparison (steady-state).

Sensor Numerical Tmax (K) Exp steady mean (average of the last five experimental readings) (K) Relative error (%)
T1 310.38 308.81 0.51%
T2 310.25 309.50 0.24%
T3 309.84 310.69 0.27%
T4 310.27 311.82 0.50%

Following the root-sum-square method of Moffat, the measurement uncertainties were quantified by combining systematic and random components as Inline graphic. The NTC thermistors have a systematic accuracy of Inline graphic, and the random scatter of the steady-state readings contributed below Inline graphic, giving a combined temperature-measurement uncertainty of approximately Inline graphic per sensor. The YF-S402 flow sensor is accurate to Inline graphic of reading (Inline graphic at 0.27 Inline graphic), while the 12-bit data-acquisition resolution (Inline graphic) is negligible. Since the maximum numerical-experimental deviation (Inline graphic) exceeds this measurement uncertainty, it is attributed to minor flow maldistribution and contact-resistance effects rather than sensor error, confirming that the CFD model reliably reproduces the measured thermal response.

The present validation was conducted at a single representative operating point (3 C, 0.27 L/min). As the validated physics are governed by the unit-cell interactions described above rather than by pack size, the model is considered reliable for scaling to the 24-cell domain; nevertheless, full-scale 24-cell experimental validation under a range of flow rates and discharge conditions is identified as a valuable extension and is planned for future work.

Results and discussion

This section compares the thermal performance across the three cooling Configurations: serpentine, parallel and counter-flow. In EV applications, Li-ion packs face a wide C-rate range from daily driving (Inline graphic 0.2–0.5 C) to short high-power transients during rapid acceleration or regenerative braking, which impose high C-rates that can reach 5 C. Although these events last only seconds, so pack average temperature rises slowly, local heating can be severe and can govern BTMS design. In the simulation, discharge rates from 1 C to 5 C are tested. Although 5 C exceeds typical sustained operation, it probes performance limits and robustness under worst-case thermal loading. These conditions reveal thermal gradients, hotspot formation, and the effects of surface contact and flow distribution. The 5 C cases validate the cooling capacity and structural resilience and inform optimization, supporting safer, longer-lasting EV packs.

Temperature distribution

Temperature contours were analyzed for each Configuration. The cell numbering across the three Configurations follows a consistent top-down, left to right order: row 1, cells 1 to 6; row 2, cells 7 to 12; row 3, cells 13 to 18; row 4, cells 19 to 24. Figure 11 illustrates this scheme, where Fig. 11a shows Configuration 1, and Fig. 11b applies the same numbering to Configurations 2 and 3 to maintain consistency.

Fig. 11.

Fig. 11

(a) Cell numbering scheme for Configuration 1& (b) Cell numbering layout for Configurations 2 and 3,.

Single serpentine tube

The serpentine design shows pronounced temperature gradients along the flow direction. Cells near the inlet remain cooler, whereas outlet-side cells run hotter as heat accumulates downstream. Figure 12 reports the temperatures of 24 Li-ion cells at 0.024 Inline graphic for Configuration 1, which routes a single serpentine tube through the pack across 1 C to 5 C. It is clear from the figure that cell temperature rises with C-rate, and this is due to the increased internal heat generation. Above 3 C the temperature rise becomes steep. Cells later in the path reach higher maximum temperature because of the cumulative heating and declining local heat transfer. This highlights a core limitation of serpentine routing: upstream cells receive colder coolant and cool more effectively than downstream cells as the coolant warms. It is also worth noting that contact interfaces, especially the TIM and the battery-aluminum channel contact are vital for reducing thermal resistance. To study this effect, uneven contact was deliberately modeled at selected cells (e.g., cells 7 and 8). These findings show that both the cooling Configuration and battery contact quality strongly affect pack-level temperature.

Fig. 12.

Fig. 12

Battery maximum temperatures for Configuration 1 (serpentine flow) at 0.024 m/s under different C-rates.

The serpentine-cooled pack exhibited a strong dependence of cell temperature on discharge rate. At 1 C (3 Inline graphic), the hottest cell (7) reached 27.2 Inline graphic, while the coolest inlet-side cell (6) was at 25.8 Inline graphic, giving a gradient of about 1.4 Inline graphic. At 2 C (6 A), the maximum rose to 33.4 Inline graphic, representing a 6.2 Inline graphic increase over 1 C, while the inlet-side cell (6) rose to 28.5 Inline graphic, an increment of 2.7 Inline graphic. At 3 C (9 Inline graphic), the peak temperature jumped to 43.6 Inline graphic, which is 10.2 Inline graphic higher than 2 C, while inlet cells increased to 32.7 Inline graphic, a rise of 4.2 Inline graphic. At 4 C (12 Inline graphic), the maximum reached 57.7 Inline graphic, showing a further 14.1Inline graphic rise compared to 3 C, while inlet cells reached 38.7 Inline graphic, an additional 6.0 Inline graphic increase. At 5 C (15 Inline graphic), the downstream cell temperature spiked to 75.7 Inline graphic, marking a total rise of nearly 48.5 Inline graphic relative to 1 C, while the inlet-side cells increased more moderately to 46.3 Inline graphic, or 20.5 Inline graphic above 1 C. These results indicate that temperature gradients across the pack widen sharply with increasing C-rate, from about 1.4 Inline graphic at 1 C to nearly 30 Inline graphic at 5 C, with downstream cells such as 7 and 18 consistently hotter due to accumulated heating, and local imperfections in thermal contact further confirming that both cooling Configuration and interface quality critically affect pack-level thermal performance.

The results validate Configuration 1 as a baseline but expose thermal limits under high loads and uneven contacts. Configuration 1 shows acceptable performance up to 3 C, but at higher C-rates it suffers from excessive temperatures. These findings motivate improved designs for EV applications where safety and uniform temperature are critical.

Figure 13 shows the temperature contours of the battery packs for Configuration 1 across the 24 cells at 0.024 m/s over discharge rates from 1 C to 5 C. Raising the C-rate increases internal heat generation, elevating Tmax and broadening pack-wide thermal gradients. At 1 C, temperatures remain relatively uniform, with all cells below 27 Inline graphic. At 3 C, localized heating emerges, especially in mid and end path cells (7 and 18) attributed to insufficient contact area. At 5 C, a clear inlet to outlet gradient appears: Tmax exceeds 75 Inline graphic, driven by the warming unidirectional flow and the limited contact area of some cells. For instance, cell 7 reaches 75.7 Inline graphic and cell 18 exceeds 74.1 Inline graphic, confirming a nonuniform profile. These results show that, despite adequate bulk velocity, serpentine routing imposes sequential cooling and thermal stacking, motivating parallel or counter-flow layouts in later sections.

Fig. 13.

Fig. 13

Temperature contour plots for Configuration 1 (serpentine channel) at a constant coolant velocity of 0.024 m/s under increasing discharge rates from 1 C to 5 C.

Three parallel tubes

The parallel design yields better temperature uniformity by cooling multiple cells simultaneously. In Configuration 2, illustrated in Fig. 2b and visualized in Fig. 14, three parallel cooling tubes are inserted between the battery rows, each receiving an inlet velocity of 0.008 Inline graphic, giving the same total flow rate (0.024 Inline graphic) as the single serpentine channel. Despite the reduced velocity per channel, the parallel distribution limits cumulative heat absorption along any one path and extracts heat simultaneously from each row, thereby reducing fluid-side resistance and preventing the inlet-to-outlet buildup observed in Configuration 1. This is evident in Fig. 14; the maximum cell temperature drops across all C-rates compared to Configuration 1 at the total flow rate. Quantitative results confirm this advantage: at 1 C, both systems show similar peak temperatures (~ 27 Inline graphic), but the parallel layout narrows the gradient from 1.4 Inline graphic to 0.6 Inline graphic. At 2 C, Tmax falls from 33.4 Inline graphic (serpentine) to 32.6 Inline graphic (parallel) while ΔT drops from 4.9 Inline graphic to 2.1 Inline graphic. At 3 C, parallel cooling reduces Tmax by 1.9 Inline graphic and halves the gradient (10.9 Inline graphic → 4.5 Inline graphic). At 4 C, the difference becomes more pronounced, with Tmax reduced from 57.7 Inline graphic to 54.4 Inline graphic and ΔT cut from 19.0 Inline graphic to 8.0 Inline graphic. Finally, at 5 C, the serpentine pack overheats to 75.7 Inline graphic with a 29.4 Inline graphic gradient, while the parallel pack remains at 70.6 Inline graphic with only a 12.4 Inline graphic gradient. Former hotspots (cells 7, 12, 18, and 24) now fall within a much narrower range, confirming that parallel cooling not only lowers absolute temperatures but also significantly enhances thermal uniformity across the pack. Expressed as a reduction, the parallel layout narrows the inter-cell gradient by 57%, 57%, 59%, and 58% at 2 C, 3 C, 4 C, and 5 C respectively relative to the serpentine design, while lowering peak temperature by up to 5.1 Inline graphic at 5 C.

Fig. 14.

Fig. 14

Temperature maximum distribution for Configuration 2 (parallel flow) at 0.008 m/s per channel.

Surface contact between the cells and cooling plates remains critical. Cells with optimized contact and uniform TIM application, such as in cells 2–5, 8–11,13–17 and 20–23, show better thermal performance. In contrast, degraded contacts, for example, cells 6,7, 21, and 24 produce localized temperature spikes, even in the improved Configuration. Thus, increasing the contact area is as important as channel-level design for effective BTMS.

Figure 15 illustrates the temperature contours for Configuration 2 under discharge rates ranging from 1 C to 5 C at a coolant velocity of 0.008 m/s per channel. In this setup, the coolant enters three separate inlets, each serving a row of six cells, which shortens the flow path and enables simultaneous heat extraction. As a result, the overall cell temperatures are markedly reduced compared to Configuration 1. For example, at 1 C the pack operated between 26.4 Inline graphic (cell 22) and 27.0 Inline graphic (cell 18), giving a narrow spread of only 0.6 Inline graphic. At 2 C, temperatures rose to 30.5–32.6 Inline graphic, with a spread of 2.1 Inline graphic, nearly half the 4.9 Inline graphic variation observed in Configuration 1. At 3 C, the hottest cell reached 41.7 Inline graphic (cell 18) while the coolest remained at 37.2 Inline graphic (cell 22), giving a ΔT of 4.5 Inline graphic—less than half the 10.9 Inline graphic gradient in serpentine cooling. At higher loads, the benefit becomes even more apparent: at 4 C the parallel design limited Tmax to 54.4 Inline graphic, compared to 57.7 Inline graphic. Finally, at 5 C the pack peaked at 70.6 Inline graphic (cell 18) while the lowest was 58.2 Inline graphic (cell 22). Despite these improvements, local variations remain evident: corner or edge cells such as 6, 7, and 24 recorded 3–6 Inline graphic higher than the coolest regions, underscoring the influence of thermal interface quality and channel proximity. Overall, Configuration 2 delivers superior heat mitigation, with temperature spreads consistently narrowed by 40–60% across all C-rates relative to Configuration 1, confirming the effectiveness of parallel flow distribution in BTMS.

Fig. 15.

Fig. 15

Temperature contour plots of Configuration 2 (three parallel cooling channels) under 1 C to 5 C discharge rates at a constant coolant velocity of 0.008 m/s per channel.

Counter-flow tube

The counter-flow design achieved the best thermal performance, minimizing temperature rise and improving uniformity. In Configuration 3, depicted in Fig. 2c and quantitatively represented in Fig. 16, two parallel channels and one counter-flow tube operate at a flow velocity of 0.008 m/s, as in Configuration 2. This maintains the same total inlet flow rate as Configuration 1, enabling direct comparison at matched flowrate.

Fig. 16.

Fig. 16

Temperature maximum distribution for Configuration 3 (parallel + counter-flow) at 0.008 m/s.

The counter-flow feature reverses coolant direction over part of the pack, balancing inlet-outlet gradients and mitigating downstream heat accumulation typical of unidirectional layouts. Compared to Configuration 1, Configuration 3 shows lower Tmax and tighter pack-level uniformity through divided and redirected flow. Compared to Configuration 2, the difference in peak temperature and thermal uniformity over each cell is relatively minor, primarily because the number of cells per row is limited, reducing the total heat accumulation in each stream. However, Configuration 3 offers marginally better pack-level thermal uniformity which will be analyzed in more detail in Sect. 5.3.

At 1 C (3 A), Configuration 3 maintained a maximum temperature of 27.0 Inline graphic. At 3 C (9 Inline graphic), the maximum temperature rose to 41.5 Inline graphic; this corresponds to about 4.8% lower Tmax than Configuration 1 (≈ 43.6 Inline graphic). Under the most severe condition of 5 C (15 Inline graphic), the pack reached a maximum of 70.0 Inline graphic, which is 5.7 Inline graphic cooler than Configuration 1 (≈ 75.7 Inline graphic) and 0.6 Inline graphic cooler than Configuration 2 (≈ 70.6 Inline graphic). These results confirm that the counter-flow arrangement distributes heat extraction more evenly across the pack, limiting hotspot formation in downstream cells. The improvements over Configuration 2 are modest, primarily because the limited cells per row reduce heat accumulation per stream; nevertheless, Configuration 3 consistently provides the lowest Tmax and ΔT across all C-rates and offers marginally better pack-level thermal uniformity which will be analyzed in more detail in Sect. 5.3.

Figure 16 shows a narrower spread of maximum temperature and more even gradients than other two Configurations. Critical cells such as 6, 12, 18, and 24 now lie closer to the pack mean, indicating effective temperature smoothing. Surface contact and TIM still govern local behavior; where contact is suboptimal, small anomalies persist, confirming the influence of interface resistance.

Figure 17 shows the temperature contours for Configuration 3, which employs two parallel channels and one counter-flow channel, under discharge rates ranging from 1 C to 5 C at a fixed coolant velocity of 0.008 Inline graphic per channel. As expected, higher C-rates increase the thermal load, raising cell temperatures across the pack. At 1 C, the pack temperature remained tightly clustered between 25.5 Inline graphic and 27.0 Inline graphic (ΔT = 1.5 Inline graphic). At 3 C, Configuration 3 limited the maximum temperature to 41.5 Inline graphic, around 2.1 Inline graphic cooler than Configuration 1 (≈ 43.6 Inline graphic) and 0.3 Inline graphic cooler than Configuration 2 (≈ 41.7 Inline graphic). At severe conditions of 5 C, Configuration 3 peaked at 70.0 Inline graphic, which is 5.7 Inline graphic lower than Configuration 1 (≈ 75.7 Inline graphic) and 0.6 Inline graphic lower than Configuration 2 (≈ 70.6 Inline graphic). These results confirm that the counter-flow design effectively redistributes coolant, reducing hotspot formation and balancing inlet-outlet gradients. While the differences from Configuration 2 are modest in uniformity, Configuration 3 consistently achieves the lowest maximum temperatures and most symmetric distribution, particularly in mid-path and outlet-side cells, making it the most effective layout for pack-level thermal control.

Fig. 17.

Fig. 17

Temperature contour distribution of Configuration 3 (two parallel + one counter-flow channel) at 0.008 m/s coolant velocity per channel under discharge rates from 1 C to 5 C.

Maximum cell temperature differs across Configurations, especially between Configuration 1 and the parallel/counter-flow layouts, highlighting distinct thermal behaviors and cooling effectiveness. In Configuration 1, the maximum temperature at 5 C occurred at cell 7 (75.7 Inline graphic), with cell 18 at 74.1 Inline graphic, illustrating sequential flow and downstream heat buildup. In Configuration 2, the pack maximum dropped to 70.6 Inline graphic at cell 18, a 6.7% reduction compared to Configuration 1. Notably, cell 7 cooled more strongly to 64.7 °C, corresponding to a 14.8% reduction, while cell 6 stabilized at 67.3 Inline graphic. In Configuration 3, under the most severe condition of 5 C (15 Inline graphic), the pack reached a maximum of 70.0 Inline graphic which is 5.7 Inline graphic cooler than Configuration 1 (≈ 75.7 Inline graphic) and 0.6 Inline graphic cooler than Configuration 2 (≈ 70.6 Inline graphic). Overall, both Configurations 2 and 3 significantly reduce peak temperatures compared to Configuration 1, with Configuration 2 yielding the coolest local hotspot at cell 7, but Configuration 3 achieving the lowest overall pack maximum and the most balanced temperature distribution. The persistent elevation at cell 6, attributed to degraded thermal contact, underscores the importance of applying TIM across the pack to ensure uniform heat dissipation.

Figures 18, 19 and 20 present the minimum cell temperatures for Configurations 1–3 under discharge rates of 1 C to 5 C at a coolant velocity of 0.008 Inline graphic per channel. In Configuration 1, the minimum temperature increases from 25.1 Inline graphic at 1 C to 38.9 Inline graphic at 5 C, with cell 6 recording 31.3 Inline graphic as the lowest value at 5 C. In Configuration 2, the minimum rises from 25.5 Inline graphic at 1 C to 38.8 Inline graphic at 5 C, with cell 4 registering 36.4 Inline graphic at the highest load, representing a 5.1 Inline graphic increase compared to Configuration 1. In Configuration 3, Tmin starts at 25.5 Inline graphic at 1 C and reaches 39.6 Inline graphic at 5 C, with cell 4 showing 36.3 Inline graphic at 5 C, very close to Configuration 2 but still slightly higher than Configuration 1. These results show that while all Configurations follow the expected rising trend of Tmin with increasing C-rate, Configurations 2 and 3 maintain higher baseline minimum values compared to Configuration 1.

Fig. 18.

Fig. 18

Battery minimum temperatures for Configuration 1 (serpentine flow) at 0.024 m/s under different C-rates.

Fig. 19.

Fig. 19

Temperature minimum distribution for Configuration 2 (parallel) at 0.008 m/s.

Fig. 20.

Fig. 20

Temperature minimum distribution for Configuration 3 (parallel + counter-flow) at 0.008 m/s.

Degraded contacts cause deviations especially at boundary cells such as 6 and 18 highlighting the need for effective TIM layer. Configuration 3, which is presented in Fig. 20, shows the most balanced minimum temperature profile across the 24 cells. The reverse path dissipates heat and equalizes thermal exposure.

Effect of coolant flow rate

Across all Configurations, maximum cell temperature decreases as coolant velocity increases, reflecting stronger convective cooling. However, this cooling enhancement diminishes beyond 0.008 Inline graphic most evident in Configuration 2 and Configuration 3. In Configuration 1, cell 7 temperature drops by 1.8% (5.81 Inline graphic) and cell 18 temperature drops by 1.63% (5.22 Inline graphicwhen velocity rises from 0.003 to 0.05 Inline graphic. In Configuration 2, cell 7 temperature drops by 1% (3.18 Inline graphic and cell 18 temperature drops by 1.61% (5.11 Inline graphic when velocity increases from 0.008 to 0.05 m/s. In Configuration 3, the temperatures of cells 7 and 18 decrease by 1.57% (4.97 Inline graphic) and by 3.32 Inline graphic, respectively when coolant velocity increases from 0.008 to 0.05 Inline graphic, respectively. While all designs benefit from higher velocity, improvement slows markedly after 0.008 Inline graphic in Configuration 2 and 3, indicating a cooling saturation region where further velocity increases yield only marginal reductions in Tmax. Figures 21, 22 and 23 compare the maximum temperature distribution of the 24-cell pack under 3 C discharge for Configurations 1–3, showing the effect of varying coolant velocity from 0.001 to 0.05 Inline graphic; as the flow rate increases, all Configurations exhibit a reduction in Tmax, with Configuration 3 maintaining the lowest values, followed by Configuration 2, while Configuration 1 consistently records the highest peak temperatures.

Fig. 21.

Fig. 21

Maximum temperature distribution across all 24 cells at various coolant flow velocities (0.003–0.05 m/s) for Configuration 1 under 3 C-rate discharge.

Fig. 22.

Fig. 22

Maximum temperature distribution at different coolant flow velocities (0.001–0.05 m/s) for Configuration 2 under 3 C-rate discharge.

Fig. 23.

Fig. 23

Maximum temperature variation with increasing coolant velocity (0.001–0.05 m/s) for Configuration 3 at 3 C-rate discharge.

Cell uniformity

In battery thermal analysis, it is essential to distinguish between inter-cell thermal uniformity (often referred to as Thermal Uniformity over the Entire Pack) and intra-cell thermal uniformity (also called Thermal Uniformity over Each Cell), as they address different thermal challenges and serve distinct engineering purposes.

Inter-cell thermal uniformity (thermal uniformity over the entire pack)

Inter-cell thermal uniformity evaluates the temperature consistency among all cells in the pack. Minimizing deviations is crucial for safe, efficient operation because large temperature differences accelerate aging, cause uneven capacity fade, and degrade performance. The average temperature of each of the 24 cells was analyzed at 3 C for three cooling Configurations. The metrics used to assess uniformity included the mean temperature, standard deviation, CV, and maximum temperature difference (ΔTinter).

Table 7 reports the calculated values for these parameters. Configuration 1, characterized by a high coolant velocity (0.024 Inline graphic), exhibited the poorest inter-cell uniformity with a standard deviation of 2.406 Inline graphic and ΔTinter of 11.04 Inline graphic. This large spread is attributed to the sharp temperature rise in certain cells (e.g., Cell 7) despite the moderate average pack temperature. In contrast, Configurations 2 and 3, which utilized parallel and counter cooling, showed improved uniformity. Configuration 3 achieved the best performance with a coefficient of variation of 0.32% and a ΔTinter of only 4.14 Inline graphic. Relative to Configuration 1 (CV = 0.78%, σ = 2.41 Inline graphic), Configuration 3 reduced the coefficient of variation by 59% (to 0.32%) and the standard deviation by 58% (to 1.0 Inline graphic) and cut ΔTinter by 62.5% (11.04 Inline graphic to 4.14 Inline graphic); Configuration 2 achieved comparable gains (CV 0.36%, σ = 1.11 Inline graphic). This suggests that parallel flow designs, even at lower flow rates, can more effectively equalize cell temperatures than single-loop serpentine designs at higher velocities. These findings highlight the importance of not only coolant speed but also flow distribution and Configuration geometry in maintaining thermal balance across the pack.

Table 7.

Inter-cell thermal uniformity metrics for three cooling Configurations at 3 C discharge rate.

Metric Configuration 1 Configuration 2 Configuration 3
Mean Cell Temperature (Inline graphic) 308.51 309.35 309.36
Standard Deviation (Inline graphic) 2.41 1.11 1.00
Coefficient of Variation (%) 0.78 0.36 0.32
Max Cell Temp Difference ΔTinter (Inline graphic) 11.04 4.65 4.14

Intra-cell thermal uniformity (thermal uniformity over each cell)

Intra-cell thermal uniformity refers to the temperature difference within each individual cell, typically represented by the difference between the maximum and minimum temperatures across the cell’s surface. This metric is critical because internal temperature gradients can induce mechanical stress, localized aging, electrode degradation, and thermal runaway risk, especially under high C-rate operations. The intra-cell thermal non-uniformity for each of the 24 cylindrical cells was computed under three different cooling Configurations at a 3 C discharge rate. The temperature difference (ΔTₖ) for each cell was derived from simulation outputs. Table 8 compares the intra-cell thermal uniformity across the three cooling Configurations. Configuration 1 contains the single cell with the smallest internal gradient (ΔTₖ = 5.48 K), but simultaneously the widest range (4.66 K) and the highest standard deviation (1.09 K), indicating that this low minimum is an outlier rather than evidence of uniform heat dissipation. Configuration 2 delivered the best uniformity, with the lowest standard deviation, 0.47 Inline graphic, and coefficient of variation 5.6%, this represents a 57% reduction in intra-cell standard deviation (1.09 K to 0.47 K) and a 60% reduction in coefficient of variation (13.9% → 5.6%) relative to Configuration 1, showing that distributing flow across separate paths enhances cell heat extraction. Configuration 3 showed slightly higher variability, likely from flow alignment differences. These results confirm that the flow distribution and channel Configuration, not flow rate alone, govern intra-cell uniformity.

Table 8.

Intra-cell thermal uniformity comparison across three cooling Configurations (ΔT = Tmax – Tmin per cell).

Metric Config 1 (0.024 m/s) Config 2 (0.008 m/s) Config 3 (0.008 m/s)
Mean Temp Difference (K) 7.85 8.37 8.34
Max Temp Diff (K) 10.14 9.50 9.68
Min Temp Diff (K) 5.48 7.73 7.69
Range ΔT (K) 4.66 1.77 1.99
Standard Deviation (K) 1.09 0.47 0.54
Coefficient of Variation % 13.9% 5.6% 6.5%

Figures 24, 25, 26, 27, 28, 29 visualize intra-cell thermal uniformity, expressed as the temperature difference (ΔT) within each of the 24 cells across the three studied Configurations under fixed and varying discharge conditions. In Fig. 24 (Configuration 1), serpentine cooling led to significant variation in ΔT among the cells. Some cells, cells 1 and 18, exhibited ΔT values exceeding 10 K, while others, cells 6 and 19, showed much lower values (~ 5.5 K). This reflects serial flow in which upstream cells are colder and downstream cells are warmer, creating uneven heat removal and a high standard deviation. Configuration 2 (Fig. 25) shows tighter clustering around the mean. Parallel distribution supplies each row simultaneously, reducing the coefficient of variation to 5.6%. Configuration 3 (Fig. 26) performs slightly worse compared to Configuration 2 but better than Configuration 1. Counter-flow reduces through-pack gradients but lacks the full symmetry and pressure balance of parallel channels. Cells near the flow reversal region remain mildly higher ΔT.

Fig. 24.

Fig. 24

Temperature difference (ΔT) distribution over each cell in Configuration 1 (serpentine cooling) under a 3 C discharge.

Fig. 25.

Fig. 25

Thermal uniformity over each cell in Configuration 2 (Parallel cooling) under a 3 C discharge.

Fig. 26.

Fig. 26

Thermal uniformity over each cell in Configuration 3 (Counter cooling) under a 3 C discharge.

Fig. 27.

Fig. 27

Temperature difference (ΔT) distribution over each cell in Configuration 1 (serpentine cooling at 0.024 m/s) under different discharge rates.

Fig. 28.

Fig. 28

Temperature difference (ΔT) distribution over each cell in Configuration 1 (serpentine cooling at 0.024 m/s) under different discharge rates.

Fig. 29.

Fig. 29

Thermal uniformity over each cell in Configuration 3 (Counter cooling at 0.008 m/s) under different discharge rates.

Pressure drop analysis

To evaluate the hydrodynamic performance of the three cooling Configurations, pressure drop (∆P) was evaluated across a range of coolant flow velocities (0.001 to 0.05 Inline graphic) under a fixed 3 C discharge condition. The total pressure loss in each Configuration reflects the pumping power demand, which directly impacts the energy efficiency and operational cost of the BTMS.

In Configuration 1, the coolant travels sequentially through all 24 cells, resulting in a longer flow path and higher hydraulic resistance. As shown in Fig. 30, the pressure drop increased nonlinearly with velocity, reaching a maximum of 27.34 Inline graphic at 0.05 Inline graphic. Even at moderate velocities, such as 0.024 Inline graphic, the pressure drop was 12.34 Inline graphic, indicating significant resistance due to the serpentine geometry. This Configuration requires higher pumping power, especially at elevated flow rates, making it less energy-efficient, despite its simplicity.

Fig. 30.

Fig. 30

Pressure drop across the single serpentine cooling channel (Configuration 1) under a 3 C discharge rate.

In Configuration 2 (three parallel channels), the coolant divides among three shorter parallel paths, significantly reducing the flow length and frictional losses per channel. At 0.05 Inline graphic, the average pressure drop across the three channels was approximately 9.07 Inline graphic, which is 33% lower than Configuration 1 at the same normalized flow rate. At 0.01 Inline graphic, pressure drop remained below 1.65 Inline graphic, offering energy-efficient performance at typical EV cooling conditions. This demonstrates that parallelization helps achieve better cooling with less hydraulic penalty. Configuration 3 behaves similarly to Configuration 2, as all flow paths are nearly identical in geometry. The maximum pressure drop at 0.05 Inline graphic was around 9.07 Inline graphic (Fig. 31).

Fig. 31.

Fig. 31

Pressure drop comparison for Configuration 2 (three parallel channels) and Configuration 3 (two parallel + one counter-flow channel) under a 3 C discharge rate.

Pumping power and thermal-hydraulic efficiency

Pressure drop alone does not capture the energy penalty of a cooling layout; the relevant quantity is the pumping power, Inline graphic. Because the parallel and serpentine layouts distribute flow differently, pumping power was evaluated at a matched total volumetric flow rate, so that differences reflect channel topology rather than the supplied flow. Table 9 reports Inline graphic, and Inline graphic for the three Configurations across matched operating points.

Table 9.

Pumping power and thermal-hydraulic performance of the three Configurations at matched total volumetric flow rates.

Inline graphic) Config. 1 Config. 2 & 3 Pumping Power Reduction
Velocity, Inline graphic (m/s) Pressure Drop, Inline graphic Pumping Power, Inline graphic Velocity, Inline graphic (m/s) Pressure Drop, Inline graphic Pumping Power, Inline graphic
Inline graphic 0.003 1.3 0.78 0.001 0.2 0.12 Inline graphic
Inline graphic 0.009 4.3 7.74 0.003 0.5 0.90 Inline graphic
Inline graphic 0.015 7.4 22.2 0.005 0.8 2.40 Inline graphic
Inline graphic (design point) 0.024 12.34 59.2 0.008 1.3 6.24 Inline graphic
Inline graphic 0.030 15.6 93.6 0.010 1.65 9.9 Inline graphic

At the Inline graphic reference flow, Configuration 1 demands Inline graphic of pumping power, whereas Configurations 2 and 3 require only Inline graphic - an Inline graphic reduction because splitting the flow into three short parallel branches lowers per-channel frictional loss. Crucially, this reduction is achieved while Configurations 2 and 3 simultaneously lower the peak pack temperature, so the parallel layouts outperform the serpentine layout on both cooling performance and energy cost. Defining a thermal-hydraulic efficiency Inline graphic (heat removed per unit pumping power), Configurations 2 and 3 are therefore nearly an order of magnitude more efficient at equal total flow. The absolute pumping powers are small owing to the low velocities and compact cross-section, but the Inline graphic relative difference scales directly with pack count and fleet size, where parasitic pumping load erodes vehicle range.

Table 10 consolidates the key performance indices for the three Configurations at 3 C. Relative to the serpentine baseline (Configuration 1), both parallel-based layouts lower peak temperature by ~ 2 Inline graphic, more than halve the inter-cell gradient (11.04 Inline graphic → 4.65 and 4.14 Inline graphic), and cut the coefficient of variation from 0.78% to 0.36% and 0.32%. Configuration 3 attains the lowest Tmax (41.5Inline graphic), narrowest inter-cell ΔT (4.14 Inline graphic, a 62.5% reduction), and best inter-cell uniformity (CV = 0.32%), while Configuration 2 shows marginally better intra-cell uniformity (σ = 0.47 vs. 0.54 Inline graphic). Both achieved these gains at 6.24 Inline graphic—an 89% pumping-power reduction versus Configuration 1 (59.2 Inline graphic), giving a nearly order-of-magnitude higher thermal-hydraulic efficiency (~ 9×). Overall, flow distribution and channel topology, not coolant velocity alone, govern both thermal and energy performance: Configuration 3 offers the most balanced result, while Configuration 2 captures most of the benefit at lower complexity.

Table 10.

The key performance indices for the three Configurations at 3 C discharge.

Index (at 3 C) Config 1 Config 2 Config 3
Tmax (°C) 43.6 41.7 41.5
Inter-cell ΔT (K) 11.04 4.65 4.14
Inter-cell CV (%) 0.78 0.36 0.32
Intra-cell σ (K) 1.09 0.47 0.54
Pumping power (µW) 59.2 6.24 6.24
η_th-h (relative) 1.0× ~ 9× ~ 9×

Conclusion

A combined numerical and experimental study compared three liquid-cooling layouts for an NMC Li-ion module: serpentine (Configuration 1), parallel (Configuration 2), and hybrid parallel/counter-flow (Configuration 3). A four-cell test rig validated the CFD model to within ± 1.6 Inline graphic (relative deviation below 0.6%). Key findings are summarized as follows:

  • Peak temperature: Configuration 1 was the hottest (75.7 Inline graphic at cell 7 and 74.1 Inline graphic at cell 18). Configuration 2 lowered the peak to 70.6 Inline graphic (− 6.7% versus Configuration 1), and Configuration 3 gave the lowest peak (− 7.6% versus Configuration 1), reducing cell 18 by 11.8%.

  • Inter-cell uniformity: Configuration 3 was best, with σ = 1.00 Inline graphic, CV = 0.32% and the narrowest spread (ΔT = 4.14 Inline graphic) – a 62.5% reduction versus serpentine (11.04 Inline graphic) and 11% versus parallel (4.65 Inline graphic).

  • Intra-cell uniformity: Configuration 2 was best (σ = 0.47 Inline graphic, CV = 5.6%).

  • Hydraulic cost: Configuration 1 incurred the highest pressure drop (27.34 Inline graphic) and pumping power (59.2 Inline graphic); Configurations 2 and 3 cut pumping power to ≈ 6.24 Inline graphic (− 89% at matched flow), giving a nearly ten-fold higher thermal–hydraulic efficiency.

  • Beyond cooling layout, the study demonstrated that surface contact quality and the use of TIMs are equally decisive in preventing localized hotspots, particularly in boundary and mid-path cells. Flow rate analysis further revealed diminishing returns beyond moderate velocities (≈ 0.008–0.024 Inline graphic), identifying a saturation region where higher pumping effort yields marginal improvements.

Overall, while Configuration 1, although simple, suffered from excessive thermal gradients and pressure loss. Configuration 2 excelled in intra-cell uniformity and hydrodynamic efficiency as it provides a balanced solution for efficient heat transfer and minimal pumping losses. Configuration 3 demonstrated the best thermal balance as slightly improves thermal uniformity but at the cost of added complexity, Future designs should incorporate advanced flow layouts, TIM optimization, and system-level control for improved battery safety and longevity under realistic operating conditions.

List of symbols

Cp

Specific heat capacity(Inline graphic)

CV

Coefficient of variation(Inline graphic)

t

Time(Inline graphic)

T

Temperature(Inline graphic)

Inline graphic

Temperature of cell Inline graphic(Inline graphic)

Inline graphic

Temperature difference (Tmax - Tmin)(Inline graphic)

Inline graphic

Intra-cell temperature difference(Inline graphic)

Inline graphic

Mean cell temperature(Inline graphic)

U0

Open-circuit voltage(Inline graphic)

V

Coolant velocity vector(Inline graphic)

V

Cell volume(Inline graphic)

Inline graphic

Thermal conductivity(Inline graphic)

Inline graphic

Volumetric heat generation rate(Inline graphic)

Inline graphic

Pressure(Pa)

Inline graphic

Cell volume(Inline graphic)

I

Discharge current(A)

Inline graphic

Internal resistance(Inline graphic)

Greek symbols

µ

Dynamic viscosity(Inline graphic)

ρ

Density(Inline graphic)

σ

Standard deviation of cell temperature(Inline graphic)

Subscripts

cell

Quantity evaluated over an individual cell

f

Fluid (coolant) domain

i

Cell index / internal

max

Maximum value

min

Minimum value

p

At constant pressure (specific heat)

s

Solid domain

t

Temperature-based statistical quantity

Superscripts and accents

Overbar – time-mean (average) value, e.g. T̄

Overdot – time rate of change, e.g. q̇

Abbreviations

BMS

Battery Management System

BTMS

Battery Thermal Management System

CAD

Computer-Aided Design

C-DFIC

Channeled Dielectric Fluid Immersion Cooling

CFD

Computational Fluid Dynamics

CV

Coefficient of Variation

EV

Electric Vehicle

FEA

Finite Element Analysis

GV-CNF

Gradually Varied Circular Notched Fins

Li-ion

Lithium-Ion

LTO

Lithium Titanate Oxide

MAE

Mean Absolute Error

NMC

Nickel Manganese Cobalt (oxide)

PCM

Phase Change Material

RMSE

Root Mean Square Error

SIMPLE

Semi-Implicit Method for Pressure-Linked Equations

SOC

State of Charge

SOH

State of Health

TIM

Thermal Interface Material

US06

US06 Aggressive (high-speed) Drive Cycle

Author contributions

Abdelrahman O. Ali contributed to conceptualization, methodology, and manuscript drafting. Osama Abdelrehim participated in the Project administration, methodology, Resources, and critical review of the manuscript, and supervised the technical aspects of the research. Mahmoud M. Saafan provided expertise in Investigation, Resources, methodology, manuscript revisions, and supervised the technical aspects of the research. Mohamed R. Elmarghany contributed to data interpretation, methodology, manuscript revisions, and supervised the technical aspects of the research. Ahmed M. Hamed was involved in project administration, methodology, Supervision, and final approval of the version to be published. All authors have read and approved the final manuscript and agree to be accountable for all aspects of the work.

Funding

Open access funding provided by The Science, Technology & Innovation Funding Authority (STDF) in cooperation with The Egyptian Knowledge Bank (EKB). The authors received no specific funding for this study.

Data availability

Not applicable. This manuscript does not report data generation or analysis.

Declarations

Competing interests

The authors declare no competing interests.

Ethical approval

There are no ethical conflicts.

Declaration of competing interest

There are no conflicts of interest. I would like to confirm that there were no known conflicts of interest associated with this publication and that there was no significant financial support for this work that could affect its outcome.

Footnotes

Publisher’s note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

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Associated Data

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Data Availability Statement

Not applicable. This manuscript does not report data generation or analysis.


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