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Philosophical transactions. Series A, Mathematical, physical, and engineering sciences logoLink to Philosophical transactions. Series A, Mathematical, physical, and engineering sciences
. 2016 Jun 13;374(2069):20150163. doi: 10.1098/rsta.2015.0163

Loschmidt echo in many-spin systems: contrasting time scales of local and global measurements

Pablo R Zangara 1, Denise Bendersky 1, Patricia R Levstein 1, Horacio M Pastawski 1,
PMCID: PMC4855402  PMID: 27140970

Abstract

A local excitation in a quantum many-spin system evolves deterministically. A time-reversal procedure, involving the inversion of the signs of every energy and interaction, should produce the excitation revival. This idea, experimentally coined in nuclear magnetic resonance, embodies the concept of the Loschmidt echo (LE). While such an implementation involves a single spin autocorrelation M1,1, i.e. a local LE, theoretical efforts have focused on the study of the recovery probability of a complete many-body state, referred to here as global or many-body LE MMB. Here, we analyse the relation between these magnitudes, with regard to their characteristic time scales and their dependence on the number of spins N. We show that the global LE can be understood, to some extent, as the simultaneous occurrence of N independent local LEs, i.e. MMB∼(M1,1)N/4. This extensive hypothesis is exact for very short times and confirmed numerically beyond such a regime. Furthermore, we discuss a general picture of the decay of M1,1 as a consequence of the interplay between the time scale that characterizes the reversible interactions (T2) and that of the perturbation (τΣ). Our analysis suggests that the short-time decay, characterized by the time scale τΣ, is greatly enhanced by the complex processes that occur beyond T2. This would ultimately lead to the experimentally observed T3, which was found to be roughly independent of τΣ but closely tied to T2.

Keywords: Loschmidt echo, irreversibility, decoherence, non-equilibrium quantum many-body dynamics

1. Introduction

If an ink drop falls into a pond, the stain diffuses away until no trace of it remains whatsoever. One may naturally say that such a process is in fact irreversible. In the microscopic world, similar phenomena are also ubiquitous. For instance, let us consider a many-spin quantum system in thermal equilibrium where a local polarization excess is injected. Then, this excitation would spread all over as a consequence of spin–spin interactions. Such an apparently irreversible process is known as spin diffusion [1,2] and it can lead the system back to equilibrium. However, this naive picture has its limitations. On the one hand, spreading is not always the rule, as there are physical situations where the initial excitation does not vanish. This is the case of Anderson localization [3,4] or when the excitation remains topologically protected [5]. On the other hand, even in cases where the system seems to have reached an equilibrium state, the unitarity of quantum dynamics ensures a precise memory of the non-equilibrium initial condition. Then, if some experimental protocol could reverse the many-body dynamics, it would drive the system back to the initial non-equilibrium state [6]. Such a general idea defines the Loschmidt echo (LE), which embodies the various time-reversal procedures implemented in nuclear magnetic resonance (NMR) [79].

The first NMR time-reversal experiment was performed by Hahn in the 1950s [10]. The procedure, known as spin echo, reverses the precession dynamics of each independent spin around its local magnetic field by inverting the sign of the Zeeman energy. However, the sign of the energy associated with the spin–spin interactions is not inverted and, accordingly, the echo signal is degraded. Such a decay occurs within the time scale T2 that characterizes the spin–spin interactions. Indeed, these interactions determine the survival of a spin excitation at short times as ∼ 1−(t/T2)2 and its later complex dynamics generating a diffusive spreading. By the early 1970s, Kessemeier, Rhim, Pines and Waugh implemented the reversal of the dynamics induced by the spin–spin dipolar interaction [11,12]. This results in the ‘magic echo’, which indicates the recovery of a global polarization state. Two decades later, Ernst and co-workers introduced the ‘polarization echo’ [13]. There, a local excitation injected in a many-spin system is allowed to evolve, then time-reversed and finally detected locally at the initial spot. While the success of these time-reversal echoes unambiguously evidenced the deterministic nature of spin dynamics in NMR, it is clear that the reversal is unavoidably degraded by uncontrolled internal or environmental degrees of freedom or by imperfections in the pulse sequences. Furthermore, the degradation seems to occur in a time scale, say T3, much shorter than a naive estimation of the characteristic scale of these perturbations, say τΣ. Then, the question that arises is whether the complexity inherent to a large number of correlated spins would enhance the fragility of the procedure under perturbations.

The next generation of experiments in organic crystals [1416] seemed to confirm that the experimental T3 never exceeds a few times T2. In other words, T3 remains tied to the time scale that characterizes the reversible many-body interaction. This led to the postulate that, in an infinite many-spin system, the complex dynamics could favour the action of any small non-inverted interaction that perturbs the reversal procedure. Thus, reversible interactions become determinant for the irreversibility rate. This constitutes our central hypothesis of irreversibility. Such wisdom is further reinforced by the natural association of many-body complexity with a form of chaos [17,18] and the confirmation that quantum dynamics of classically chaotic systems should manifest a dynamical instability [19] which leads to an environment-independent decoherence rate [20,21].

During the last decade, solid-state NMR has kept on providing a versatile testing bench to study time reversal in large spin arrays [2226]. In fact, a standard experiment involves a crystalline sample with an infinitely large number of spins. By contrast, the numerical test of many-spin dynamics has to be restricted to strictly finite systems [27,28]. While this appears to be a major limitation, it allows the analysis of a situation that the experiments cannot achieve: moving progressively from small systems to larger ones with a fully controlled perturbation. The expectation is that a sort of finite size scaling may allow one to identify an emergent mechanism that rules reversibility in the thermodynamic limit [29]. As in the experiments, the witness for such a transition should be the LE as measured by a single spin autocorrelation function M1,1, i.e. a local polarization. For short, we call M1,1 the local LE. It is not difficult to prove that Π1,1≡(M1,1+1)/2 is the probability that a given spin, say the first, remains up after the whole procedure. Besides, in a case of a spin excitation in a one-dimensional chain with XY interactions [3032], M1,1 precisely coincides [27] with the global overlap of two one-body wave functions as defined for semi-classical systems [20,33,34]. The square of the overlap between the initial and final many-body wave functions, MMB, defines a global or many-body LE. It is important to note that MMB has not been addressed experimentally, but nevertheless it is a natural magnitude in theory [3537]. Thus, we are left without a precise relation between the object of theoretical studies and experimental ones, i.e. MMB and M1,1, respectively. This missing link is the central question we address in this paper.

Here, we consider a system of N spins whose initial state is given by a local excitation injected in a high-temperature state. First, we discuss the formal relation between MMB and M1,1, which is derived exactly at least for very short times. In particular, we assess how the N dependence or extensivity of MMB is evidenced in the time scales involved. This leads us to hint that the revival of a many-spin state results from the recovery of each individual spin configuration, much as if they were statistically independent events. Because in the initial high-temperature state there are N/2 spins up, their rough statistical independence would lead to a behaviour of the sort MMB∼(Π1,1)N/2∼(M1,1)N/4. This is confirmed by the numerical evaluation of the LE in a specific spin model.

Furthermore, we discuss a general picture beyond the short-time regime, where the decay of M1,1 results from the interplay between the time scale that characterizes the reversible interactions (T2) and that of the perturbation (τΣ). This would ultimately lead to the experimentally observed T3. In such a sense, our analysis provides a conceptual link between the theoretical and the experimental realms.

The paper is organized as follows. In §??sec2, we introduce the LE framework: the initial state and the time-reversal procedure. Here, we define both the local and global LEs. In §??sec3, we compute the short-time expansions for the local LE and its non-local contributions (in particular, the many-body LE). This allows us to discuss a general picture of the LE decay in terms of the times scales that characterize MMB and M1,1. The dependence on N is discussed in terms of the extensivity of MMB and statistical independence of the local autocorrelations. In §??sec4, we assess our expectations by a numerical evaluation of the LE in a spin system. Section ??sec5 summarizes our main conclusions and some of the important open questions in the field.

2. The Loschmidt echo in spin systems

Let us first specify the initial condition of a ‘local excitation in a many-spin system’. We consider N spins Inline graphic in an infinite-temperature state, i.e. completely depolarized mixture, plus a locally injected polarization,

2. 2.1

Here, the spin 1 is polarized while the others are not, i.e. Inline graphic. Such an initial state can be experimentally implemented not only in NMR [38] but also in cold atoms [39].

As in the early LE experiments [1416], our numerical evaluation focuses on an imperfect time-reversed evolution of the excitation, followed by a local measurement. The procedure is depicted in figure 1. A many-spin Hamiltonian Inline graphic rules the forward evolution of the system up to a certain time tR. At that moment, an inversion of the sign of Inline graphic is performed, leading to a symmetric backwardevolution. Nevertheless, there are unavoidable perturbations, denoted by Inline graphic, that could arise from the incomplete control of the Hamiltonian, acting on both periods. Thus, evolution operators for these tR periods are Inline graphic and Inline graphic respectively. It is quite practicable to define the LE operator as

2. 2.2

which produces an imperfect refocusing at time 2tR. A local measurement of the polarization, performed at site 1, defines the local LE:

2. 2.3

Here, we choose as free variable t=2tR, the total elapsed time in the presence of the perturbation. The time dependence of Inline graphic in the Schrödinger picture is

2. 2.4

Figure 1.

Figure 1.

The scheme of the local LE, M1,1(t). (a) The initial state is given by a local excitation in a high-temperature spin system, as stated in equation (2.1). The system is allowed to evolve under the Hamiltonian Inline graphic and the excitation diffuses all over until a time t=tR (b). At that time, a time reversal is performed, leading to a backward evolution ruled by Inline graphic. At time t=2tR (c), a local measurement is performed at the initial spot. (Online version in colour.)

Using equation (2.1), and after some algebraic manipulation, the LE can be explicitly written as a correlation function:

2. 2.5

Here, the time dependence is written according to the Heisenberg picture,

2. 2.6

Note that equation (2.5) is an explicit correlation function at the same site but different times, i.e. an autocorrelation. This kind of correlation has been recently employed to address localization phenomena in spin systems [4,40,41], and it generalizes the standard one employed to assess spin diffusion [42]. In terms of the Hilbert–Schmidt inner product between the initial and the time-evolved density matrices, i.e. equations (2.1) and (2.4) respectively, the LE can be written as [15,43,44]

2. 2.7

which, in the present case, progressively decays from 1 to 0, as occurs with the statistical overlap between two wave packets in the standard LE definition [20].

Equivalent expressions for the LE can be derived by decomposing the statistical state into a simpler basis. In order to proceed with the pure state decomposition of Inline graphic, we consider the computational Ising basis {|βi〉}, also known as the Sz-decoupled basis. Additionally, we define the set Inline graphic of indices j that label basis states which have the first spin pointing up, i.e. Inline graphic. It is straightforward to verify that Inline graphic. Then, as introduced in [30],

2. 2.8

Here, Π1,1(t) denotes the probability that the first spin keeps pointing up after a time t. After some manipulation,

2. 2.9

Here, Inline graphic stands for the complement of Inline graphic, i.e. Inline graphic Inline graphic. One can naturally identify and define the two terms that contribute to the local polarization M1,1(t). The first sum in equation (2.9) stands for the average probability of revival of the many-body states, denoted by MMB(t),

2. 2.10

The second sum in equation (2.9) represents the average probability of changing the configuration of any spin except the first. The third sum stands for the average probability that the first spin has actually flipped, i.e. of all those processes that do not contribute to M1,1(t). Then, the processes that contribute to M1,1(t) but not to MMB(t) are denoted as

2. 2.11

This balance of probabilities leads to the appropriate asymptotic behaviour of M1,1(t) according to the symmetries that constrain the evolution. The identification

2. 2.12

is a crucial step for the following discussions.

If we use the identity Inline graphic in equation (2.5), the invariance of the trace under cyclic permutations ensures that Inline graphic. As Inline graphic, then

2. 2.13

which is indeed an explicit way to rewrite equation (2.3) in the form of an ensemble average. Remarkably, as Inline graphic is a local (one-body) operator, its evaluation in equation (2.13) can be replaced by the expectation value in a single superposition state [45],

2. 2.14

where

2. 2.15

Here, φi is a random phase uniformly distributed in [0,2π). In fact, the state defined in equation (2.15) is a random superposition that can successfully mimic the dynamics of ensemble calculations and provides a quadratic speed-up of computational efforts [4547].

3. The Loschmidt echo dynamics

(a). Short-time expansions and beyond

In order to analyse the N dependence of the LE and its time scales, we compute here the short-time expansion of the magnitudes M1,1(t), MMB(t) and MX(t). Up to second order in time,

(a). 3.1

Similarly, the leading contributions to MMB(t) and MX(t) are

(a). 3.2

and

(a). 3.3

Let us consider a generic secular(i.e. polarization-conserving) perturbation Inline graphic given by a Hamiltonian with an arbitrary anisotropy α,

(a). 3.4

This is still quite general, as even a double quantum perturbation (Inline graphic, which does not conserve polarization) can be reduced to a secular one by the truncating effects of radiofrequency fields [29]. In addition, we do not consider here the case Inline graphic (e.g. pure Ising or on-site diagonal disorder), as in such a condition the first non-trivial order in time is the fourth (see Appendix). Then, the following identities hold:

(a). 3.5
(a). 3.6
(a). 3.7

Here, σ2 stands for the average local second moment of Inline graphic,

(a). 3.8

Being a perturbation, we note that σ2 is much smaller than the average local second moment Inline graphic of the unperturbed Hamiltonian Inline graphic. In terms of time scales,

(a). 3.9

The identities in equations (3.5)–(3.7) lead to

(a). 3.10
(a). 3.11
(a). 3.12

These expansions hold for t<(τΣ/N). Beyond such a very short-time regime, a general term in the expansion of M1,1(t) will be of the form

(a). 3.13

with k≥2 and the coefficient c(N,n) described by combinatorial numbers of increasing size that depend on the topology of the interactions (e.g. see [25,48]). As the experimental set-up corresponds to the limit described by equation (3.9), this expansion will be dominated by terms with the lowest possible order in the weak interaction, i.e. k=2:

(a). 3.14

Equation (3.14) indicates that, beyond the very short-time expansion, i.e. (τΣ/N)<t<τΣ, the dependence on τΣ becomes superseded by the diverging terms in the scale T2. This could lead to the new time scale T3, which was seen experimentally to be tied to T2 as

(a). 3.15

In that sense, T3 becomes characteristic of the complexity or ‘chaos’ of the many-spin system that amplifies the small effect of the perturbation. In addition, it is important to stress that, being an experimental fact, equation (3.15) corresponds to a system composed by infinitely many interacting spins. In other words, equation (3.15) stands for the relations of time scales in the thermodynamic limit. Quite on the contrary, any numerical simulation involves a finite, very small indeed, number of spins where the irreversibility rate T3 would be essentially given by τΣ. Then, the LE decay rate evaluated in a finite system would ultimately be perturbation-dependent [28]. Thus, our central hypothesis of irreversibility would mean that equation (3.15) is an emergent property. It should rely on the thermodynamic limit, which implies taking the limit Inline graphic first, and then Inline graphic. The non-uniformity of these limits plays a crucial role to yield quantum phase transitions, as discussed in the context of Anderson localization [4951].

The physical picture described above is schematically represented in figure 2. There, we show the expected interplay between MMB(t) and MX(t) leading to M1,1(t). Indeed, as stated in equations (3.11) and (3.12), the very short-time dependence of both contributions is extensive in N: MMB(t) decreases as 1−2t2/4 and MX(t) increases as (N−4)σ2t2/4. Such a precise balance provides for the short-time decay of M1,1(t) given by equation (3.10), i.e. 1−σ2t2. Note that there is no reason to assume that the decay of MMB(t) would remain ruled by τΣ. Beyond the very short times, we expect that the time scale T3 should also show up as T3/Nν with ν∼1 in the decay of MMB(t) (see below). Furthermore, while MMB(t) goes monotonically to zero, MX(t) displays a highly non-trivial behaviour. Indeed, MX(t) first increases by feeding from the decay of MMB(t) until it reaches a maximum. This growth indicates a progressive divergence of long-range correlations. Thereafter, MX(t) should decay, accounting for the fact that the state remains properly normalized. This is precisely what M1,1(t) measures: a conserved polarization that ultimately distributes uniformly within the spin system. In an isolated finite system this implies the asymptotic plateau Inline graphic. As pointed out above, the decay of both M1,1(t) and MX(t) occurs in a time scale T3, which, according to equation (3.14), is somewhat longer than but close to the ‘diffusion’ time T2. This is the regime captured experimentally.

Figure 2.

Figure 2.

A pictorialscheme of the time dependence of M1,1(t) (black dotted line) and its contributions, as indicated by the labels, MMB(t) (blue solid line) and MX(t) (green solid line). Their short-time expansions, as stated in equations (3.10)–(3.12), are indicated with arrows. In particular, the expansion corresponding to the short-time behaviour of M1,1 (t) is plotted with a black dashed line. (Online version in colour.)

(b). The extensive decay hypothesis

The previous short-time expansions provide a hint on the scaling relation between the local LE, M1,1(t), and the global one as embodied by MMB(t). In particular, let us first compare the probability of refocusing the configuration (up or down) of a single spin, i.e. Π1,1(t), and the probability of refocusing a complete many-spin state MMB(t). If the refocusing of each individual spin could be treated as an independent event, then the scaling between Π1,1 and MMB would be extensive in N,

(b). 3.16

Here, the factor Inline graphic in the exponent comes from equation (2.1), i.e. the initial high-temperature state, where basically half of the spins point up, and half of them point down. Then, one can resort to the picture of a lattice gas where N/2 particles jump among N lattice sites. As in the well-known Jordan–Wigner transformation [52], a fermion is associated with a spin pointing up and a vacancy corresponds to a spin pointing down. Thus, the microstate of the gas is completely described by the position of N/2 particles.

Strictly speaking, the notion of extensiveness corresponds to standard thermodynamic quantities such as the entropy of the system. In addition, as discussed in [16], Inline graphic is precisely a measure of the entropy. Then, the validity of equation (3.16) implies an extensivity relation between the entropy per spin and the total entropy of the system.

According to equations (2.8) and (3.10),

(b). 3.17

which, in turn, up to second order in time, implies Π1,1(t)≃(M1,1(t))1/2. Thus, equation (3.16) yields

(b). 3.18

This is precisely the relation verified between equations (3.10) and (3.11).

One might expect that, beyond the very short-time decay, individual spin autocorrelations deviate from statistical independence. However, this deviation will still have a local nature and, therefore, the N-extensivity would remain valid. Indeed, we propose

(b). 3.19

where the exponent η would be some appropriate function η=η(N,t). Our ‘extensive decay hypothesis’ implies that η factorizes,

(b). 3.20

where f(t) stands for a function that encloses information of the correlations originated by the system dynamics. Additionally,

(b). 3.21

is required in order to recover equation (3.18), i.e. statistical independence.

4. A one-dimensional model

The physical picture described above is discussed here in the light of a specific model. In particular, we assess the validity of equations (3.18) and (3.20). We consider a one-dimensional spin chain with an anisotropic interaction described by

4. 4.1

with periodic boundary conditions, i.e. a ring configuration. Here, J0 stands for the natural units of the spin–spin interaction energy. As a perturbation Inline graphic, we choose a next-nearest-neighbour interaction described by

4. 4.2

Such a perturbation appears naturally when one attempts to build an effective one-body dynamics from linear crystals with dipolar interactions [53]. This is also the case in a regular crystal, when the natural non-secular dipole–dipole terms are truncated by the Zeeman energy of the radiofrequency irradiation, which ultimately leads to effective secular two-body next-nearest-neighbour interactions [29].

The local second moments σ2 and Inline graphic of Inline graphic and Inline graphic, respectively, can be evaluated as in equation (3.8) as

4. 4.3

and

4. 4.4

and constitute the main energy scales of our problem.

In figure 3, we plot M1,1(t), MMB(t) and MX(t) for the particular choice JΣ=0.1J0. The short-time expansions given in equations (3.10)–(3.12) are evaluated according to equation (4.3). It is observed that MMB(t) vanishes for long times. Actually, a close observation shows that Inline graphic (data not shown). In addition, note that Inline graphic. Such an asymptotic contribution provides for the equidistribution of the spin polarization Inline graphic. This long-time saturation corresponds to the equilibration of a finite system.

Figure 3.

Figure 3.

The localLE and its non-local contributions. M1,1(t), MMB(t) and MX(t) correspond to the black, blue and green solid lines, as indicated by the labels; N=14, JΣ=0.1 J0. The short-time expansions given in equations (3.10)–(3.12) are shown as black, blue and green dashed lines, respectively. (Online version in colour.)

In contrast with our schematic plot in figure 2, here MX(t) does not get too close to 1 and MMB(t) does not decay much faster than M1,1(t). As MX(t) provides for the whole M1,1(t) once MMB(t) has fully decayed, the contribution of MX(t) is considerable only at long times. These effects are a consequence of the relatively small size of the system considered. Indeed, the case in figure 3 corresponds to N=14 spins, and thus the exponent that relates M1,1(t) and MMB(t) is quite small, (N/4)=3.5. The need for larger systems indicates that revealing the dominant orders in equation (3.14) is a major numerical challenge that may go beyond the state-of-the-art techniques [54].

In order to assess the accuracy of the ‘extensive decay hypothesis’, in figure 4, we address the scaling relation between M1,1(t) and MMB(t) discussed in §??sec3b. In particular, we try out the factorization stated in equation (3.20). By plotting Inline graphic as a function of time, we observe a unique function which does not depend on N or JΣ, but it has a weak dependence on time. Such a unique curve is indeed f(t) as defined in equation (3.20). This means that the extensivity relation between M1,1(t) and MMB(t) is confirmed. The statistical independence, in turn, fails progressively once f(t) departs from the Inline graphic factor of the ideal relation in equations (3.18) and (3.21). As beyond the short-time regime f(t) decreases with time, we conclude that the recovery of a single spin is tied to the recovery of its neighbours. Thus, the spins are positively correlated and the revival probability of the complete N-spin state is enhanced. This argument is particularly relevant in one-dimensional systems.

Figure 4.

Figure 4.

Therelation Inline graphic as a function of time. For JΣ=0.1 J0, the sizes plotted are: N=10 (circles), N=12 (squares), N=14 (diamonds) and N=16 (stars). For JΣ=0.2 J0, the sizes plotted are: N=10 (solid line), N=12 (dashed line), N=14 (dash-dotted line) and N=16 (dotted line). For JΣ=0.3 J0, the sizes plotted are: N=10 (up triangles), N=12 (down triangles), N=14 (plus signs) and N=16 (right triangles). (Online version in colour.)

After the onset of the saturation regime, where M1,1∼1/N and Inline graphic, the universal scaling naturally becomes noisy and the curves for different N and JΣ separate from each other. As the decay is faster for larger perturbations, the appearance of such a spurious behaviour is observed to occur first for the largest value of JΣ considered (JΣ=0.3J0, plus signs and triangles).

5. Conclusion

We presented a detailed analysis of the LE in interacting spin systems. As in the NMR experiments, a local version of the LE, M1,1, is defined as a single spin autocorrelation function. Simultaneously, we define a global LE, MMB, as the average of the square of the overlap between many-body wave functions that evolved under perturbed Hamiltonians. While the former constitutes a specific experimental observable, the latter has only been assessed theoretically. Here, we showed the formal relation between both magnitudes, as far as their characteristic time scales and N dependence are concerned.

By analysing a short-time expansion of M1,1 and MMB, we derived a precise relation between their time scales. In this regime, the decay of M1,1 is given by the average local second moment of the perturbation Inline graphic, and the decay of MMB by N times the local scale (Inline graphic). This relation hints at a scaling law MMB∼(M1,1)N/4 that accounts for the extensivity of MMB. In such a case, the recovery of a many-spin state results from the recovery of each individual spin, much as if they were independent events. The numerical evaluation in a specific spin model shows that the exponent slightly diminishes with time, starting from the initial N/4. This means that the recovery of a single spin is positively correlated with the probability of recovery of its neighbours, and thus it improves the probability of the revival of the complete N-spin state. A precise control of these correlations may hint at experimental access to the global autocorrelation, i.e. MMB, just by measuring a single spin (local) autocorrelation M1,1. This would require an experimental protocol capable to encode a local excitation into a correlated many-spin state.

In addition, we discussed a general dynamical picture beyond the very short-time regime. There, the decay of M1,1 results from the interplay between the time scale that characterizes the reversible interactions (T2) and that of the perturbation (τΣ). This would ultimately lead to the experimentally observed T3, which was found to be roughly independent of τΣ but closely related to T2. The theoretical quest for the emergent T3 time scale remains open and it may be beyond the reach of current numerical approaches. Assessing a fair estimate analytically would require a detailed account of the higher-order processes that dress the quadratic term in the perturbative expansion.

Note that our discussion led us to identify T3, and hence the spin–spin interaction time T2, as the time scales characterizing the complexity or many-spin chaos. As such, they show up not only in the decay of M1,1 and MMB, but also in the growth of MX=M1,1MMB. Indeed, in the field of anti-de Sitter/conformal field theory (AdS/CFT) correspondence there is an increasing interest in characterizing the role of chaos in quantum dynamics [5558]. There, chaos manifests in the growth of four-body correlation functions, following an early suggestion by Larkin & Ovchinnikov [59]. They employed semiclassical arguments to address disordered superconductors and probed that the square dispersion of momentum should grow exponentially in a time scale determined by the collisions with impurities, i.e. with the unperturbed Hamiltonian (in our physical picture, T2). Similarly, our average multi-spin correlation MX would ultimately diverge within a time scale T3/N, i.e. independent of the perturbation. This is indeed a measure of the decoherence, and hence of irreversibility, induced by many-spin chaos. Of course, we do not have a precise characterization of this time scale or the specific mathematical dependence on time. Thus, this is a puzzling issue to explore in the field of many-body chaos. Besides the obvious relevance for statistical mechanics and experimental physics, this might also contribute to a possible pathway between quantum mechanics and gravity.

Acknowledgements

This work benefited from discussions with A.D. Dente and F. Pastawski. H.M.P. greatly acknowledges hospitality of A. Kitaev at Caltech, P.A. Lee at MIT and V. Oganesyan at CUNY, where the issues discussed in this paper acquired certain maturity. P.R.Z. acknowledges M.C. Bañuls and J.I. Cirac for their kind hospitality at MPQ in Garching.

Appendix A

It is worth mentioning that the very short-time expansions in equations (3.10)–(3.12) do not depend on the anisotropy α of the perturbation. In general, it can be proved that if Inline graphic then

graphic file with name rsta20150163-e41.jpg A 1

This is precisely the case of a perturbation Inline graphic enclosing Anderson disorder and Ising interactions [40] or interactions with a fluctuating field [60].

Data accessibility

Numerical data plotted in figures 3 and 4 can be made available upon request to the corresponding author.

Competing interests

We declare we have no competing interests.

Authors' contributions

The authors contributed equally to the research reported in this paper.

Funding

We acknowledge financial support from CONICET, ANPCyT, SeCyT-UNC and MinCyT-Cor. This work used computational resources from CCAD—Universidad Nacional de Córdoba (http://ccad.unc.edu.ar/), in particular the Mendieta Cluster, which is also part of SNCAD—MinCyT, República Argentina.

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Associated Data

This section collects any data citations, data availability statements, or supplementary materials included in this article.

Data Availability Statement

Numerical data plotted in figures 3 and 4 can be made available upon request to the corresponding author.


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