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Proceedings. Mathematical, Physical, and Engineering Sciences logoLink to Proceedings. Mathematical, Physical, and Engineering Sciences
. 2018 Feb 21;474(2210):20170566. doi: 10.1098/rspa.2017.0566

Nematic director fields and topographies of solid shells of revolution

Mark Warner 1,, Cyrus Mostajeran 2
PMCID: PMC5832830  PMID: 29507509

Abstract

We solve the forward and inverse problems associated with the transformation of flat sheets with circularly symmetric director fields to surfaces of revolution with non-trivial topography, including Gaussian curvature, without a stretch elastic cost. We deal with systems slender enough to have a small bend energy cost. Shape change is induced by light or heat causing contraction along a non-uniform director field in the plane of an initially flat nematic sheet. The forward problem is, given a director distribution, what shape is induced? Along the way, we determine the Gaussian curvature and the evolution with induced mechanical deformation of the director field and of material curves in the surface (proto-radii) that will become radii in the final surface. The inverse problem is, given a target shape, what director field does one need to specify? Analytic examples of director fields are fully calculated that will, for specific deformations, yield catenoids and paraboloids of revolution. The general prescription is given in terms of an integral equation and yields a method that is generally applicable to surfaces of revolution.

Keywords: nematic, elastomers, glasses, curvature, shape

1. Introduction

We explore the creation of intrinsically curved shells from flat sheets, completing the connection between the specification of planar mechanical response to the final shapes obtaining. Mechanical response due to heat, light or solvent uptake that spatially varies in-plane means that the metric, specifying intrinsic lengths in a sheet, also varies. Such metric variation means that lengths in neighbouring elements in a plane that become inconsistent with each other can only be resolved by a topography change to that of a Gaussian-curved state. The simplest example is discussed in [1,2], in the context of circular symmetry that interests us here, that is of length changes along and perpendicular to a nematic director, n of a liquid crystalline solid, but where n forms concentric circles: Contraction along the preferred (circumferential) direction and (radial) elongation perpendicular leads to the ratio of circumference and radius deviating from 2π, necessitating the formation of cones (with localized Gaussian curvature (GC) at their tips) in order to avoid in-plane stretches.

The connection between metric change and GC is straightforward in principle, though perhaps in practice arduous to calculate, see [35] for examples, in nematic solids. In particular, see eqns (2.2) and (3.6) of [5] for the prescription in the current context for connecting this metric variation with GC. However, connecting GC with the topography of a final state without stretch (but with, cheaper, bend) is not always possible, is not necessarily 1:1, and is generally very difficult. The final topography is the most interesting aspect of local length changes, and we give an explicit connection for the important case of circularly symmetric distributions of GC leading to cylindrically symmetric topographies. We also thereby show the inverse—of how to connect a given topography of a surface of revolution back to its GC and thence to a particular form of metric variation, and hence ultimately to the director distribution required to create the desired Gaussian-curved shape. This connection, forwards and backwards, is also addressed for cylindrical symmetry in some generality by Aharoni et al. [3] in the case of director patterns that are symmetric under translations along specific planar directions and who, as in [4,5], gave examples of constant curvature surfaces. We give a straightforward method for director fields that are instead symmetric under planar rotations about a central point in the reference state and illustrate it with some examples beyond constant curvature. An interesting contrast between our method and the work in [3] is that our approach yields surfaces of revolution that intersect the axis of revolution, whereas the approach in [3] results in surfaces of revolution that do not. This is due to the utilization of circularly symmetric director fields in our method, which offers the added benefit of enabling the construction of anchorable topographical surfaces with fixed circular perimeters [5,6].

If the extent of solvent absorption is modulated in-plane, even where the swelling is isotropic, GC can arise [7,8]. But when the length changes at each point can differ as well in each direction, the topographical response can be much richer. Such examples arise, irreversibly, in the growth of some plant leaves where the anisotropy of growth direction can vary spatially to give wrinkling [9]. We mentioned simple circular patterns above giving cones. Logarithmic spirals (where the director has a fixed direction to a radius) also give cones, and have been experimentally investigated by Broer et al. and by White et al [10,11]. Other suitable spirals also give surfaces of constant, but now non-zero curvature (spheres and spherical spindles) [3,4], and these too are found experimentally [5,6]. Such systems have also been explored numerically by Selinger et al. [12] for liquid crystal elastomers where a range of curvatures from complex director distributions lead to shells with curvature.

The imposed deformation of conventional flat sheets to intrinsically curved surfaces without tearing or wrinkling is impossible; it is the map-maker’s problem. These non-isometric problems, including ones arising in applications to origami, are intriguing in their own right and are reviewed in this context [13], and have recently indeed been termed ‘non-isometric origamis’ [14]. There is a more practical interest: Impeding the evolution of such non-isometric topographies gives effective stretches and compressions away from induced equilibrium values, leading to strong forces (as opposed to those arising when impeding bend), and thus highly effective actuation. An example is the resting of a load on an array of would-be cones or square pyramids. To avoid in-plane stretches, the load must be lifted on the tips of the shapes evolving below it [15], such a lifter being able to lift loads greatly exceeding (×100 or more) its own weight. Although these structures are slender, and are acting in a pushing mode, they are not susceptible to Euler buckling instabilities due to their pushing through their intrinsic curvature. Thus actuations large compared with the material thickness are possible, in distinction to more conventional pushers that need to be stout. Equally, a deforming shell anchored at its boundary (see [5] for a scheme for achieving fixed boundaries, and below for induced paraboloids) will raise a fluid underneath it by suction—a pump—or strongly block a channel on deforming into it—the first valve working by push has been developed by Sánchez et al. [16], albeit of the stout type. In general, we envisage action in these curvature-changing systems to be uniquely functional at the micro-level since there the concept of ‘The Material Is the Machine’ [17] is very powerful.

2. Connecting director patterns to topography

We consider nematic solids, elastomers or glasses, with an anisotropy direction n along which there may be elongation or contraction by a factor of λ>1 or λ<1, respectively. The deformation gradient may be 1/4<λ<4 for elastomers and 0.9<λ<1.1 for glasses, can be induced by heat or light, and is reversible [18,19]. The two directions perpendicular to n suffer λν where ν is the thermal or optical equivalent of the Poisson ratio, that is, it gives the sympathetic transverse mechanical response to a λ induced along n; it takes the value ν=1/2 for elastomers and ν0.8⇠⇢2.0 for glasses. The thermo-optical deformation gradient tensor is accordingly

F=(λλν)nn+λνId3, 2.1

where Id3 denotes the identity operator on R3, and where F gives the heated or irradiated relaxed state without stresses. We either (i) take an in-plane pattern for n(r) to obtain a GC and topography, or (ii) address the inverse problem of a target topography and inquire as to what imprinted in-plane variation of n(r) is needed to generate it.

The two-dimensional metric tensor of the deformed sheet upon stimulation is a=FTF, i.e.

a=(λ2λ2ν)nn+λ2νId2. 2.2

With respect to local coordinates (xi)i=1,2, the metric tensor can be symbolically represented by the squared length element ds2=aijdxidxj, where the metric components take the form

aij=(λ2λ2ν)ninj+λ2νδij. 2.3

It describes a new system, if it is thin enough to relax stretches in preference to much cheaper bends. The variation of a gives the connections Γijk. The variation of the connections, and their products with themselves, give K(r), the GC; see [5] for these results in this context.

Dealing with circular symmetry, we resort to circular coordinates (r,θ). The angle α between the director and the radius is only a function of r, that is α(r). In circular coordinates and with this symmetry, the metric tensor’s components are shown in [5] to be

arr=λ2+(λ2νλ2) sin2(α),arθ=aθr=r2(λ2νλ2) sin(2α)andaθθ=r2[λ2ν(λ2νλ2) sin2(α)].} 2.4

The Gaussian curvature is

K(r)=λ2λ2ν2[(α+3rα) sin(2α)+2α2cos(2α)], 2.5

where α′ is dα(r)/dr.

Consider as an illustration a reference state director field n(r) allowing largely analytic illustrations in what follows: α(r)=α0+α1ln(r/r0). From a differential triangle, the inset box of figure 1, of a director element dn and its elements in the radial and θ directions, one sees the director integral curve r=rn(θ) must obey rdθ/dr=tanα(r). In this illustration, dα/dr=α1/r and hence:

dθdr=1rtanα1α1ddr ln(cosα(r))θ(r)=1α1 ln(cosα(r))r=rn(θ)=r0 exp [1α1cos1(eα1θ)α0α1]. 2.6

The origin of θ is where α=0, at a radius rin=r0 exp (α0/α1). The maximal α in this band of the director field is π/2 (and thus an azimuthal n) and occurs at r=r0 exp ((π/2α0)/α1)rin exp (π/2α1) (figure 1). The pattern then repeats in radial bands. For further examples of similar periodic spiral director fields, along with their stream functions, see [4,5].

Figure 1.

Figure 1.

Centre: An integral curve, rn(θ), of the director field n(r) in the initial, flat space, for α(r)=α0+α1 ln(r/r0). The inner and outer (Γ1) solid circles are where the director angle to the radius is α=0 and απ/2, respectively. The pattern repeats in circular bands of exponentially varying width. A section (Γ2) of the proto-radius’ initial state integral curve r(θ) starts on the inner, full circle where α=0 and ends on the outer. The dotted circle, r=r0, is where α=α0. The image Γ2′ of Γ2 is the distorted (three dimensional) state’s new radius (the in-material distances represented here on the same diagram). It ends on the deflated circle Γ1′, the image of Γ1 at new intrinsic length u from the centre, and starts a little inside the inner circle. (For α0=0.2, α1=0.85, λ=0.7, ν=2.) Right: Director integral curves corresponding to α(r). Solid circle r=r0. Inset square: Geometry to construct director integral curve. (Online version in colour.)

We now construct a parametrization of the final, curved surface by curves that are related back to their original trajectories in the initial flat space.

(a). Construction of in-material circles and radii in the deformed state

Consider two curves Γ1 and Γ2 in the plane that, after F acts, will remain circles and become radii, respectively. We will need these elements to describe the final topography, and the transformation method between the Γ curves and the final descriptors will be repeatedly used (figure 1).

Take a parametrization (by t) of the Γ curves as (r(t),θ(t)), for convenience taken to be unit speed and thus with a unit tangent vector t=(r˙,θ˙) (with ˙d/dt), that is r˙2+(rθ˙)2=1. It transforms to F(r˙,θ˙). By symmetry, the circle Γ1 with r˙1=0 must transform into an, in general, de/inflated circle, Γ1′. Demanding that the transformed tangent vectors are orthogonal (so Γ2 generates a radius curve Γ2′ in the sense that it meets the circle Γ1′ perpendicularly) yields

((r˙2,θ˙2)FT)(F(r˙1,θ˙1))(r˙2,θ˙2)a(r˙1,θ˙1)=0,r˙2arθ+θ˙2aθθ=0dr2dθ2=aθθarθ 2.7

on using FTF=a in polar coordinates, and r˙1=0, θ˙1=1 to parametrize circles centred at the origin. The final result specifies the proto-radius Γ2, that is r2(θ2), which is defined as the curve in the reference state that evolves to become a geodesic radial curve in the final state. The identification of proto-radii is central to our length specification method which determines the principal curvatures and hence topography, as developed in subsection b. With our illustrative choice of α(r) entering the elements of the metric, equations (2.4), we obtain explicitly:

dθdr=12r(λ2νλ2) sin2αλ2ν(λ2νλ2) sin2α=12α1ddr ln(λ2ν(λ2νλ2) sin2α)e2α1θ=1(1λ2(1+ν)) sin2α, 2.8

with θ=0 where α=0. Inverting equation (2.8) for α(θ) and using α(r)=α0+α1 ln(r/r0) in the form of r(α), the proto-radius’ integral curve is thus:

r(θ)=r0 exp [1α1 sin11e2α1θ1λ2(1+ν)α0α1] 2.9

and is depicted in figure 1. This would-be radius starts and ends perpendicular to circles where it is respectively along or perpendicular to the director. It remains so during deformation since at these points there is no rotational effect: The proto-radius’s tangent vector at these points is along the principal directions of the deformation. Between these points there is an inflectional point of maximal angle to the radial direction. When α=const., one has a log spiral for n and the proto-radii can trivially be shown also to be (different) log spirals [20].

The lengths of the intrinsic circles and radii in the transformed state are not necessarily in the ratio 2π and hence there is enclosed GC that we will now calculate by ascertaining the lengths of the transformed curves Γ1′ and Γ2′. One can further see from figure 1 that transformation gives material rotation, since Γ2Γ2 by an amount that depends on radial position r. The transformation of Γ1 by F gives a new circle Γ1′ with a new element of length:

(dt)2[(0,θ˙1)a(0,θ˙1)](dt)2dt=aθθr2rdθ1andl1=2πraθθr2,} 2.10

where l1 is the de/inflated circumference. Questions of new geodesics and the effect of rotations are explored more generally in [20]. In particular, it is there demonstrated how proto-radii are rotated locally whereas circles naturally remain circles.

(b). Circularly symmetric director fields and surfaces of revolution

We employ a standard calculation of the GC, K(r), in terms of the specification of points on a surface of revolution using projected radii and height functions γ1(u),γ2(u) (figure 2), where the parameter u is the intrinsic, radial length from the pole of the surface. Comparing the K(r) obtained from γ1 and γ2 with that obtained from the metric tensor variation, we obtain expressions for the functions γi. The azimuthal angle will be ϕ.

Figure 2.

Figure 2.

A point w (heavy dot) in the cylindrically symmetric surface is specified by the radius γ1(u) and the height function γ2(u), both functions of the in-surface radial length u from the apex. The usual azimuthal angle in such cylindrical coordinates is ϕ. (Online version in colour.)

With c and s shorthand for cosϕ and  sinϕ, respectively, the variation of the surface point w=(γ1(u)c,γ1(u)s,γ2) in the u and ϕ directions yields the respective unit tangents. Radially, one obtains tu=∂w/∂u=(γ1c,γ1s,γ2′)/(γ′21+γ′22)1/2, where γ′≡dγ/du, differentiation with respect to its argument u. Since the unit speed representation is differentiable, then γ′21+γ′22=1. The azimuthal, unit tangent is tϕw/ϕ(s,c,0). These orthogonal, unit tangents generate the unit normal to the surface N=tutϕ=(γ2c,γ2s,−γ1′)/(γ′21+γ′22)1/2.

The rate of change of N with γ1ϕ in the ϕ direction determines the associated curvature 1/Rϕ:

1Rϕ=|1γ1Nϕ|=|γ2γ1(s,c,0)|=γ2γ1. 2.11

The other principal curvature, 1/Ru, derives from the normal’s in-material variation with u, that is ∂N/∂u. One can easily show, from the orthogonality of tu and tϕ, that 1/Ru depends only on the variation of tu, and is 1/Rϕ=|∂tu/∂u|. After a little algebra, one can show that 1/Ru=(γ1′′γ2′−γ1γ2′′)/(γ′21+γ′22). In deriving these results, we can set γ′21+γ′22=1 at the end, and along the way use this constraint in its differentiated form: γ1γ1′′+γ2γ2′′=0.

Recognizing that K=1/(RuRϕ), we arrive at:

K(u)=γ1γ1. 2.12

The form of K is only deceptively simple since we have the connections between γ1′ and γ2′, and the constraints 0<|γ′|<1 which considerably restrict solutions. Indeed we will find regions where we contravene this essential condition because the surfaces are not those of revolution, as we have assumed, and one has moved away from the underpinning assumptions made. Note also that K(u) is a function of the in-material radius u rather than of the original parametrization radius r that our other, metric-derived expression (2.5) for K depends. Therefore, except for the case of constant GC (addressed for actual examples of surfaces in [35]), we need to connect r and u in order to solve equation (2.12) with a K(r) from the metric to obtain γ1 and γ2, and thus the surface.

The proto-radius Γ2 tangent vector (r˙2,θ˙2) transforms under F to give a new element of length du along Γ2′ of du=|F(r˙2,θ˙2)|dt, whence the new curve’s length is:

u=dt(r˙2,θ˙2)FTF(r˙2,θ˙2)=0r2dr2[arr+2arθθ˙2r˙2+aθθ(θ˙2r˙2)2]1/2, 2.13

on taking out dr2/dt and using FTF=a. Further, the last part of equation (2.7) which defines the proto-radius Γ2 in flat space, dr2/dθ2r˙2/θ˙2=aθθ/arθ, means u simplifies to:

u=0r2dr2Det(a)aθθ=λ1ν0r2dr2r2aθθ(r2)=λ1ν0r2dr2λ2ν(λ2νλ2) sin2(α(r2)). 2.14

since Det(a)=r2λ2(1−ν). A trivial example is a log spiral with α=const., independent of r2′. One then directly obtains u=λ1νr2/λ2ν(λ2νλ2) sin2(α), with ur2, which is indeed characteristic of a cone [1] with K=0 everywhere except for a concentration of GC at its tip.

We transform variables from u to r (in effect r2) by taking g1(r)≡γ1(u(r)) and g2(r)≡γ2(u(r)), say, whence dγ1/du=(dr/du)(dg1/dr), where the coefficient of dg1/dr can be expressed as a function of r:

drdu(r)=1du/dr=λ2ν(λ2νλ2) sin2(α(r))λ1ν. 2.15

The second derivative needed for equation (2.12) also follows: d2γ1/du2=(dr/du)2d2g1/dr2+(d2r/du2)dg1/dr, with

d2rdu2(r)=α(λ2νλ2) sin(2α(r))/(2λ2(1ν)), 2.16

where α′≡dα/dr. The functions (dr/du)(r) and (d2r/du2)(r) enter the differential equation (2.12) for the surface in terms of its original coordinate r:

(d2rdu2)g1+(drdu(r))2g1=g1K(r). 2.17

The curvature on the right-hand side is that derived from the metric variation, equation (2.5), and depends on α(r), α′(r) and α′′(r), as do the coefficients of g1′ and g1′′, the derivatives with respect to their argument, r, that is here ′≡d/dr. It is this equation we now solve to illustrate a range of shells resulting from an imprinted director distribution steering the mechanical response.

As the original perimeter 2πr deforms to an l1=2πraθθ/r2, see equation (2.10), and that from figure 2 clearly l1=2πγ1, then

g1(r)γ1(u(r))=raθθr2=r(λ2ν(λ2νλ2) sin2α(r))1/2. 2.18

One can confirm that this g1(r) is indeed the1 solution of equation (2.12). Having thus solved for g1, one simply needs to solve for the height function through dγ2/du=1(dγ1/du)2 where dγ1/du=(dg1/dr).(dr/du). Thus, rather in terms of r, we have for g2:

dg2dr=(dudr(r))2(dg1dr)2. 2.19

The elements of the right-hand side of equation (2.19) are all known functions of r, once α(r) is given, and the surface is specified by the solution of this first-order ODE in r for g2(r) and g1(r) above.

For most director variations α(r) there can be an eventual r where circular symmetry is lost: In the expression above equation (2.19) for dγ1/du, solutions are retained for (dγ1/du)2<1. In dγ1/du=(dγ1/dr)(dr/du), we use γ1=aθθ and, from equation (2.14), du/dr=λ1νraθθ. The resulting condition becomes daθθ/dr<2λ1−νr which is identical to eqn (21) of [20]. That source offers a geometric discussion of this condition for circular symmetry.

(c). Examples of topographies generated by spiral director patterns

Topography develops because of a spatially varying deformation gradient, itself arising from a varying director field. For the forward problem, from director field to topography, the above machinery makes it straightforward to select α(r) fields and then find the resultant topographies, which we now illustrate by three example functions for α(r), with sample values of material parameters and geometry specifiers.

Surfaces must have (dγ1/du)2≡((dr/du)(dg1/dr))2≤1. Using equation (2.15) for dr/du and equation (2.18) for g1(r), we can express this condition as:

1λ(1+ν)(1(1λ2(1+ν)) sin2α)12rλ(1+ν)(1λ2(1+ν))ddr sin2α1. 2.20

The upper bound turns out to be important, and constrains the choice of α(r) at r=0 and at a higher, and thus limiting value of r. At r0 one requires:

 sin2(α(0)min)=1(1+λ1+ν) 2.21

which is a constraint recurrent in the examples below. Clearly, α(0)>π/4, with equality at λ=1.

If the offset at the origin of α(r=0) is greater than α(0)min=arcsin(1+λ1+ν)1/2, then the resulting shells have a finite point at r=0, that is dγ1/du<1. Otherwise if α(r=0)=α(0) they are flat, with dγ1/du=1.

(i). Linear director angle variation

Consider α(r)=α0+r with geometric and material parameters α0=1.01, λ=0.85 and ν=2. The Gaussian curvature and the shell topography arising from this linear variation of α with r are shown in figure 3.

Figure 3.

Figure 3.

Calculated Gaussian curvature (a) and shell shape (b) arising from a deformation λ=0.85, ν=2, in a spatially varying director field α(r)=α0+r, with α0=1.01. The GC is plotted against the radial coordinate r of the initially flat, undistorted reference state. The shell is plotted parametrically with r specifying the radial coordinate g1(r) and the height function g2(r). Both plots correspond to the same region r∈[0,1] of the reference state. (Online version in colour.)

(ii). Quadratic director angle variation

Consider α(r)=α0+r2 with geometric and material parameters α0=1.25, λ=0.51 and ν=1.5. The Gaussian curvature and the shell arising from this quadratic variation of angle α with r are shown in figure 4. The integral curves of the director field with this α(r) will be shown in figure 7.

Figure 4.

Figure 4.

Calculated Gaussian curvature (a) and shell shape (b) arising from a deformation λ=0.51, ν=1.5, in a spatially varying director field α(r)=α0+r2, with α0=1.25. Coordinates and range of plots are as in figure 3. (Online version in colour.)

Figure 7.

Figure 7.

(a) The director field α(ar) required to yield a paraboloid of revolution γ2=12aγ12 when the deformation is λ=0.8, with ν=2. (b) For comparison the integral curves for α(r)=α0+r2 with α0=1.25 as employed in the forward problem shown in §c(ii); see figure 4.

(iii). Exponential director angle variation

For an exponential director angle variation α(r)=α0+α1(1−er), with geometric and material parameters α0=0.956, α1=1.245, λ=0.76 and ν=1.5, one has the Gaussian curvature and shell topography shown in figure 5.

Figure 5.

Figure 5.

Calculated Gaussian curvature (a) and shell shape (b) arising from a deformation λ=0.76, ν=1.5, in a spatially varying director field α(r)=α0+α1(1− er), with α0=0.956 and α1=1.245. Coordinates of the plots are as in figure 3, but the radial range in the reference state is r∈[0,4]. (Online version in colour.)

3. The inverse problem; connecting topography to directors

The inverse challenge is to determine what director distribution α(r) is required to be able to generate a given circularly symmetric shell. We have seen in the forward direction one has to at most solve a first-order ODE, equation (2.19), but the inverse problem throws up mathematical challenges that vary enormously in complexity depending on the specified shell. We give examples of where a simple, nonlinear first-order ODE is encountered, and solved, but in general, highly nonlinear integro-differential equations result.

Consider the two key defining equations for the resulting shell and its connection with the flat-space director field:

γ1=aθθ(r)=λνr(1β sin2α(r))1/2, 3.1
u(r)=λ1ν0rdr/aθθ(r)/r2λ0rdr(1β sin2α(r))1/2 3.2
du(r)dr=λ1ν/aθθ(r)/r2λ1νr/γ1. 3.3

where (3.1) is a compressed form of equation (2.18), and (3.2) is equally of equation (2.14), using β=1−λ2(1+ν). The difficulty exposed by equation (3.1) is that the surface (γ1(u),γ2(u)) can be expressed parametrically in the intrinsic radial distance u, but the curvature is in terms of the flat, reference space coordinate r. Equation (3.2) shows α is buried in an integral leading, in general, to integral equations. Equation (3.3) is sometimes a route to avoiding this complexity. We first illustrate some principles arising by reconsidering the simplest example:

(a). Spherical caps and spindles

The spherical cap (and spherical spindles) solved in [5] is a simple example of the inverse problem—given a constant curvature K, what is the α(r) that generates it? In that case one does not have to wrestle with the connection between u in the target space and r in the reference state since K is constant. Taking the expression (2.5) with constant K as an ODE for the director field yields:

α(r)=12arccos(12C(K)r2+c) 3.4

(eqn (3.17) of [5]) where C=K/(λ−2λ2ν) and c is a constant of integration. It is shown that c≤−(1−λ1+ν)/(1+λ1+ν), with equality in the case of spherical caps and inequality for spherical spindles. Considering the argument of arccos in equation (3.4) must be ≥−1, then clearly −1≤c. Also, the maximal radius rm is given by:

rm2=4λ(1ν)(1λ1+ν)/KorrmR=2λ(1ν)(1λ1+ν).} 3.5

We have inserted the value of C, used K=1/R2 where R is the radius of curvature, and we have taken c appropriate to a spherical cap. There is a maximum r because, in deforming a flat disc to a cap, lines of longitude have to extend, and lines of latitude have to shrink, relative to the radii and circumferences in the flat state from which they evolve. Roughly speaking, in the extreme limit radii extend by λν and circles contract by λ when α has advanced to π/2. This ratio of distortions must be sufficient to accommodate the geometric changes in trying to smooth a flat sheet around a sphere. Eventually, the changes are just too great: for instance as one approaches the South pole, geometry requires the former to approach πR, and the latter to approach 0, for which the λ factors are inadequate and the cap that can be formed is limited in extent. We meet the limitation also below for catenoids and paraboloids. This limitation can be partly obviated by adapting ‘petals’ [21], or conversely when flattening a spherical shell by partially cutting into sectors as can be left behind in an elaborately peeled orange.

What fraction of a spherical shell can be achieved for a given λ and be directly determined: It is also shown in [5] that the in-surface radius of the cap, u as defined above generally in equation (2.14), is related to the radial distance r in the reference state as:

u(r)=λ1νμ2 arctan (μ2rμ1μ2r2) 3.6
tan2(ϕm/2)=1λ1+νλ1+ν. 3.7

Here μ1=12[λ2ν+λ2+c(λ2νλ2)], μ2=14λ2(1ν)K. To arrive at equation (3.7), we have taken K=1/R2, as well as using C and c for a cap, and the above expression (3.5) for the corresponding rm. Here ϕ=u/R and is the semi opening angle for the cap. It gives a universal expression for the shape limitation explained above. For instance, λ0 would be required to make a sphere, ϕm=π. For a hemisphere, ϕm=π/2, one would require λhs=(2/3)1/(1+ν)λhs=0.85 for the value ν=1.5 considered in the examples above.

(b). The director field required for spatially varying shell curvature

To best illustrate the method of director field determination given a shell shape, we explore cases that admit of a complete, analytical solution. We thereby explore the limits of an α field specifying surfaces of revolution and the geometric constraints of radii and perimeters changing in very different ways.

Surfaces of revolution, where the in-material radius u and the radius γ1 are related as below, can be simply analysed:

u=f(γ1) 3.8
λ0rdr(1β sin2α(r))1/2=f(rλν1β sin2α(r)). 3.9

Again β=1−λ2(1+ν). In general, forms other than equation (3.8) lead to nonlinear integral equations for  sin2α. In f, the argument γ1 from equation (3.1) has been re-written as raθθ(r)/r2 to make the argument of the surd only depend on r through the dependent variable α. The integral equation nature of equation (3.9) can be eliminated by differentiation with respect to r which, after a little re-arrangement, yields a trivial, first-order ODE which we can re-write as:

dvdwvf(v)=λ1+νw. 3.10

Here w=λνr is the scaled, reference state radial length and vγ1=w1β sin2α(w). Quadrature gives the relation

h(v)vf(v)0vf(v)dv=12λ1+νw2. 3.11

We take v=0 at w=0 quite naturally since they involve intrinsic and extrinsic radii, but below in an example generalize to where this is not satisfied, that is with a more general constant of integration allowable when shells have a central disc excised.

It is generally easier to consider w2 as a function of v:

w2=2λ1+νh(v)2λ1+ν(vf(v)0vf(v)dv). 3.12

The director field required to generate a shell with a given γ1(u) (and γ2 from γ2=1γ12) is then specified by inverting the definition of v to yield  sin2α and employing equation (3.12) for w2(v) in that inversion:

α(v)=sin1[1β(1(v/w)2)]1/2=sin1[1β(1λ1+νv22h(v))]1/2 3.13

and

w(v)=2λ1+νh(v). 3.14

 Conditions on the director field.From the first part of equation (3.13), we see that

(v/w)21β=λ2(1+ν) 3.15

in order that  sin2α1. One also requires (v/w)2≤1 for  sin2α0. This condition is most seriously tested at w0 where one can expand in the right-hand side of equation (3.12) if f does not specify a surface with a singular tip:

ww02(f0λ1+ν)v2(vw)w02f0λ1+ν, 3.16

where f0df/dv|v0 is the derivative at the shell centre. From equation (3.13), we extract the required α behaviour around what will become the tip as:

 sin2α0=1β(1λ1+νf0)1λ1+ν/f01λ1+ν11+λ1+ν. 3.17

The character of the apex of the shell determines the expansion of f:

u=f(γ1)=f0+f0γ1+ 3.18

and hence the initial α. Clearly f0=0 (no in-plane radial length when γ1=0).

Shells flat at their apex have f0′=1, that is uγ1 as u,γ10. We then see from equation (3.17) the familiar result  sin2α0=1/(1+λ1+ν), that is equation (2.21).

Peaked shells have f0′>1. Simple geometry of the cone fitted to the very tip of the shell shows that u=γ1/ sinϕ and thus f0=1/ sinϕ, where ϕ is the fitting cone’s opening angle. Equation (3.17), with f0′>1, clearly now requires a larger α0 than that leading to centrally flat shells, for the same λ.

The maximum α0 is π/2, whereupon from equation (3.17) one has f0′=1/λ1+ν, or otherwise expressed  sinϕ=λ1+ν, which is the familiar result for a cone deriving from a circular director field where α=π/2, independently of r .

(c). The director field required for a catenary of revolution

An example of the general method above is that of a catenary of revolution (revolved about its symmetry axis). It can be specified by γ1,γ2 such that f(v)=sinh(v), that is

u=sinh(γ1) 3.19

and γ2=cosh(γ1). Now solution as above gives the relation

h(v)v sinh(v)cosh(v)+c=12λ1+νw2 3.20

with c a constant of integration, the size of which is critical to the character of the solutions v(w) and hence to the angle α that the director makes with the radial direction in the reference state. Following the procedure leading to equations (3.13) and (3.14), we show α(w), parametrically in v, in figure 6a.

Figure 6.

Figure 6.

(a) Calculated director angle α(w) with respect to a radius in the reference state in order to generate a target state catenary of revolution. Radii in the reference state, r, are scaled by the characteristic length of the catenary, and further as w=λνr. This illustration takes a deformation λ=0.7 with ν=1.5. The curves are labelled by the value taken for the constant c of integration in equation (3.20). (b) The in-material radial length u in a (inverted) catenoid becomes exponentially longer than the embedded radius γ1, a difference that eventually cannot be accommodated by a change in their ratio of λ1+ν induced by heat or light on even a director field with α=π/2 (which must be the director angle at the outer limit of solutions). (Online version in colour.)

The left-hand side of equation (3.20), that is h(v), is monotonic and, for small v, is:

h(v0)1+c+12v2+18v4+ 3.21

See figure 6a for the three qualitatively different solutions for α: For c<1, there is a region of small v for which f(v)<0 and there are clearly no solutions for equation (3.20). For c>1, there is a tip region of small w where the right-hand side, 12λ1+νw2, is less than the finite limiting value f(v∼0)=c−1 of the left-hand side, and again there are no solutions around the tip of the catenoid. These failures are indicative of the α(w) stemming from the choice of c failing to generate a surface of revolution. See below where we show the choice c=1 avoids this failure.

For any c, at large v we have f(v)12vev and eventually this exponential increase in f(v) again renders solutions unattainable, but for the different geometrical reason we saw in the limitation on spherical caps: figure 6b shows the in-material radius of length u corresponding to the embedded radius γ1. In the reference state, this circumference was originally 2πr and is now 2πγ1. For large enough r, for a catenoid the length u is exponentially larger than γ1 and hence exponentially larger than the original circumference to which it relates. The ratio of the two has changed by λ/λν=λ1+ν and, for large r, this transformation ratio is not large enough to accommodate the geometry of a catenoid—solutions are no longer possible (figure 6a). However, the more λ deviates below λ=1, the larger the range of radii leading to surfaces of revolution, as seen above for the spherical cap.

The case of c=1 is most interesting since then solutions obtain down to w=0 (but still fail at large w for the reasons given above): Around v∼0, equation (3.20) reduces to

12v2+12w2(1β sin2α(w))+=12λ1+νw2, 3.22

concentrating on v2 terms and using the definition v2=w2(1β sin2α(w)). Then as w0, one has the limiting (minimal) α(0) given before at equation (2.21), α(0)min=sin1(1/1+λ1+ν).

Away from w=0, the angle α grows to its maximum, π/2, which it attains on the outer boundary of the reference state domain that can support formation of catenoids by contraction along a director field. It is such an azimuthal n that gives the maximal circumferential contraction, beyond which the disparity of intrinsic and embedded radii can no longer be supported.

(d). The director field required for a paraboloid

We turn now to an important class of surfaces, paraboloids, that are susceptible to a variation of the general method stemming from u=f(γ1). Further, we emphasize an important general point about the inverse problem, that the director distribution, once chosen for a particular λ=Λ, say, produces different surfaces for all other λΛ. One is able to make general observations about the λ-surfaces arising from the Λ distribution of director, αΛ(r) say. We also show that it is possible to anchor paraboloids in their reference state support.

For the paraboloid formed from rotating γ2=12aγ12 about γ1=0, one has:

du=dγ11+(dγ2dγ1)2=dγ11+a2γ12. 3.23

Differentiating w.r.t. r, using equation (3.3) for du/dr, and replacing w=λνr and now v=1, one obtains

a2λ1+νw=v1+v2dvdw12a2λ1+νw2=13(1+v2)3/213 3.24

where the constant of integration, 13, ensures w=0,v=0. Rearrangement, and restoring v2=a2w2(1β sin2α) yields an equation for  sinα:

 sin2αλ(w)=1βλ(11a2w2[(1+32λ1+νa2w2)2/31]), 3.25

where the subscript λ on the α(w) and the β reminds us that this α(w) only yields a paraboloid for this particular λ. Expansion of equation (3.25) for w0 yields  sin2αλ(w0)=1/(1+λ1+ν)+O(w2), holding, as we have argued above, for all shells flat at their apex. We show the pattern in figure 7 for λ=0.8, ν=2, for the range α(0) (=54° for these λ and ν values) to the limit of surfaces of revolution, α=π/2.

For increasing w, the director angle increases until  sin2αλ=1, at which w we cease to be able to generate a shell of revolution. With this value of  sin2αλ, equation (3.25) yields the condition for the maximal radius:

1+λ2a2r2=(1+32λ1νa2r2)2/3, 3.26

where we return to r=ν. This expression clearly shows that the natural reduced length in the reference space is ar. The reasons for the failure to realize a shell of revolution are precisely those discussed below equation (3.5) for spherical caps, and above equation (3.22) for catenoids.

For a given αΛ pattern designed to produce a paraboloid when λ=Λ<1, we inquire of the sequence of shapes generated as λ=1λ=Λ (and possibly λ<Λ). We thus have to return to solving the forward problem, since α(r) is now given, where:

g1(r)=rλν(1βλ sin2αΛ(r))1/2. 3.27

For clarity, βλ=1−λ2(1+ν) has its λ dependence flagged, and the α field relates to Λ. To determine the shell parametrically in r, we need in addition to the embedded radius g1(r) the height function g2(r) given from the differential equation (2.19) where one needs care with du/dr=λ/1βλ sin2αΛ(r) which depends on λ and has a memory of Λ through αΛ from equation (3.25) with λ=Λ. The differential equation for g2 does not appear to admit of analytic solution, but is straightforward to solve numerically.

We can however analytically determine that for Λ<λ<1 a sequence of peaked shells is explored, terminating in a paraboloid: The derivative (dγ1/du)(r), considered as a function of the reference space r, must be bounded as −1≤dγ1/du≤1. Take (dγ1/du)(r)=(dr/du)(dg1/dr)=(1/λ)1βλ sin2αΛ(r)(dg1/dr), and take equation (3.27) to evaluate the last derivative. One then obtains for the condition that shells of revolution exist: 1λ(1+ν)(1βλ sin2αΛ(r))1 around r=0. We have used the next term in the expansion of equation (3.25), which is O(w2), to determine that (d/dr) sin2αΛ(r)|r0=0, and we further employ  sin2αΛ(0)=1/(1+Λ1+ν). After some rearrangement we obtain the condition 0≤(Λ/λ)1+ν+λ1+ν≤1+Λ1+ν which is clearly satisfied2 for Λ<λ<1. This sequence of shells exists and all have, until λ=Λ, that dγ1/du<1. They accordingly have a finite slope at r=0, that is they are pointed until λ=Λ.

(i). Fixed boundaries for mounting the paraboloid

Invariant radii are important for anchoring for applications; see the discussion in [5]. From equation (3.1), the condition γ1(r)=r for the reference space radius r to be identical to the target space embedded radius γ1 is:

λν(1βλ sin2αΛ(w))=1. 3.28

This condition determines the scaled radius w where the non-paraboloid shells at λ>Λ have natural anchoring, that is, their outer perimeter is unchanged from its value in the reference state and so it can be joined without mismatch to an inert outer region. The condition is quite simple when λ=Λ where we have the actual parabola:

1+(aw)2Λ2ν=(1+32(aw)2Λ1+ν)2/3. 3.29

Apart from the trivial solution at w=0, there is another solution at finite aw if ν>1. (One sees this from expanding around (aw)2∼0 to see that the right-hand side dominates, whereas the left-hand side is dominant at large (aw)2.) One can check whether anchoring occurs within attainable values of  sin2α by rewriting γ1(r)=r as awλν=v, squaring and substituting for v2=(aw)2(1β sin2α) whereupon  sin2α=(1λ2ν)/(1λ2(1+ν))<1 as required at the point of anchoring.

A reasonable estimate of the anchoring radius can be achieved by assuming it occurs such that 32λ1+νa2w21 so that on both sides. of equation (3.26) the 1 terms can be neglected, whereupon (aw)2(32)2Λ2(12ν). Post hoc justification of the neglect of the 1 terms, at for instance Λ=0.8 and ν=1/2, can be directly tested and holds well. Thus anchoring is possible with an outer radius of w=1a32Λ12ν.

4. Discussion

We have given explicit routes via which one can find (i) the shape of revolution resulting from the action of light or heat on a given circularly symmetric director field in an initially flat plate, and (ii) the circularly symmetric director field needed in an initially flat reference state in order to generate a specified shape of revolution. In both cases, the domain of the reference state that will generate a shape of revolution is limited by an important geometric factor that comes into conflict with the limits on how much a solid can differentially deform parallel and perpendicular to its director. It should be noted that the focus on surfaces of revolution is justified by the observation that they are often (but not always) energetically favourable isometric embeddings of a given metric based on theoretical as well as experimental findings [36]. It is also noteworthy that although the inverse problem for a given surface of revolution may not have a solution in some cases, the method developed in this paper will yield the solution if it exists. These insights should inform future programmes of the limitations for developing topography for non-isometric applications such as strong actuation, micro-mechanical components and machines (gates, valves, pumps and lifters). It also suggests future strategies for obviating these limitations, for instance, excision of regions of the reference state, and using piecewise continuous director distributions rather than simple functions as employed here. Practical examples for anchoring perimeters are given as illustrations of a general strategy for anchoring that will be needed for practical applications; we return to difficulties and advantages within this framework.

Acknowledgements

Mark Warner is grateful to Dr JS Biggins for advice and for help with numerics.

Footnotes

1

One can see that, although equation (2.12) is linear in g1, one cannot take multiples of any solution for g1 to obtain another since doing so upsets the geometric foundations (radii and circumferences) on which the solution was based.

2

As it is equivalent to (λ1+νΛ1+ν)2(1Λ1+ν)2.

Data accessibility

No additional data are associated with this work.

Authors' contributions

Both authors contributed equally to this work.

Competing interests

We have no competing interests.

Funding

C.M. is supported by the Engineering and Physical Sciences Research Council (EPSRC) of the United Kingdom.

References

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Data Availability Statement

No additional data are associated with this work.


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