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. 2018 May 29;8:8204. doi: 10.1038/s41598-018-26650-8

Quantum entanglement of a harmonic oscillator with an electromagnetic field

Dmitry N Makarov 1,
PMCID: PMC5974296  PMID: 29844533

Abstract

At present, there are many methods for obtaining quantum entanglement of particles with an electromagnetic field. Most methods have a low probability of quantum entanglement and not an exact theoretical apparatus based on an approximate solution of the Schrodinger equation. There is a need for new methods for obtaining quantum-entangled particles and mathematically accurate studies of such methods. In this paper, a quantum harmonic oscillator (for example, an electron in a magnetic field) interacting with a quantized electromagnetic field is considered. Based on the exact solution of the Schrodinger equation for this system, it is shown that for certain parameters there can be a large quantum entanglement between the electron and the electromagnetic field. Quantum entanglement is analyzed on the basis of a mathematically exact expression for the Schmidt modes and the Von Neumann entropy.

Introduction

It is known that quantum entanglement arises when the wave function of a particle system cannot be represented as a product of the wave functions of each particle. There are many such systems from which to choose. The basic method of quantum entanglement of particles is spontaneous parametric down-conversion (SPDC)13. In this process, when a nonlinear birefringent crystal is irradiated by a laser pump field the pump photons decay with a low probability into two quantum-entangled photons of lower frequencies. Despite the low probability of the decay of the pump photon, SPDC has been widely studied and has many practical applications in quantum computer science. This is due to the fact that this method is the simplest for obtaining quantum-entangled photons. While other more sophisticated methods of generating entangling particles have been proposed48 none of them result in a greater probability of entanglement of the particles under consideration than SPDC9,10. There is also a difficulty with the theoretical study of the various methods, which is that basically, quantum entanglement is a complex process for the mathematical research. For the systems under consideration, it is impossible to solve exactly the nonstationary Schrodinger equation and calculate the entanglement parameter (for example, the Von Neumann entropy in the case of a two-component system). Solutions are mainly sought using higher orders of perturbation theory and on the basis of these solutions conclusions are drawn about quantum entanglement. It is known that perturbation theory is applicable if there is a weak interaction of particles in the system, and therefore use of this theory is based on the assumption that quantum entanglement is not a large quantity. In order to study a system with large quantum entanglement, the exact solution of the Schrodinger equation must be used - a task that is very difficult to achieve mathematically. Nonetheless, when studying quantum entanglement, such a solution would be of fundamental interest. In quantum physics, it is known that exact solutions of the Schrodinger equation do present any great difficulty. In studying quantum entanglement, one can include a two-level model of Jaynes-Cummings11 in order to achieve sufficiently accurate solutions. In this model are studied the physical characteristics of a two-level atom in an electromagnetic field. It should also be noted that the Jaynes-Cummings model describes the system of a two-level atom interacting with a quantized electromagnetic field, which greatly limits its application to many physical systems (the results presented in this work go beyond this limitation). Also some model problems and particular cases for the stationary Schrodinger equation12,13. Quantum Dynamics of quantum-entangled systems is being studied actively at the present time1417. For example, on the basis of the exact solution of the nonstationary Schrodinger equation for an atom in a strong two-mode electromagnetic field, it has been shown17,18 that there is a strong quantum entanglement between photons. However, as this solution is based upon the assumption that the external electromagnetic field is many times stronger than the Coulomb field of attraction of an electron in an atom, it does not promote an understanding of the influence of the Coulomb field on quantum entanglement. Therefore, the problem of finding a system whose quantum entanglement is large, and also in which it would be possible to mathematically study quantum entanglement on the basis of an exact solution of the Schrodinger equation, is topical. In addition to this relevance, the problem of practical application is important, i.e. the proposed method should be simple enough for practical implementation.

It should be added that quantum entanglement is widely used in quantum computer science. That is why at present a great interest is attracted to this problem. In particular, using entangled states, it is possible to explain quantum communication protocols19, such as quantum cryptography20, quantum coding21, quantum key distribution22, quantum secure direct communication23, quantum machine learning24,25, entanglement swapping26,27, quantum computing algorithms28 and quantum state teleportation29. There are quite a lot of practical problems in quantum informatics, one of which is the weak generation of quantum-entangled particles. The method of generation of quanta-entangled particles proposed in this work gives a large amount of quantum entanglement.

In this paper we study the generation method of quantum entanglement of a harmonic oscillator with an external electromagnetic field. A harmonic oscillator can be an electron in a uniform magnetic field with induction B, see Fig. 1. It is known30 that in such a field the electron behaves like a harmonic oscillator with frequency ωc=Bemec, where c is the speed of light, me and −e are, the mass and charge of an electron, respectively. The wave function of such a system can be found on the basis of the exact solution of the Schrodinger equation of the specific system being studied. The quantum entanglement of the system can be studied using the analytical form of the Schmidt mode31,32 and the von Neumann entropy33,34. It is shown that for certain parameters of the system under consideration, a large quantum entanglement is possible.

Figure 1.

Figure 1

Interaction of an electromagnetic field with an electron in a magnetic field.

Exact solution of the Schrodinger equation

Let us consider, at a time t > 0, a quantized electromagnetic field acting on a system consisting of a quantum harmonic oscillator. The interaction of a harmonic oscillator of mass m occurs via an electric charge e. The Schrodinger equation for this system will be

iΨt={12m(ir+ecAˆ)2+Hˆf+mωc2(x2+δ(y2+z2))2}Ψ. 1

In the expression: (1) δ = 0 corresponds to one type of interaction, and δ = 1 to another type; i is the imaginary unit; ωc is the frequency of the oscillator; Hˆf=k,uω(aˆk,u+aˆk,u+12) is the Hamiltonian of the electromagnetic field, where aˆk,u+ and aˆk,u are the creation and annihilation operators, respectively, for photons with the wave vector k and the polarization u; and the vector potential of the electromagnetic field Aˆ has the form

Aˆ=k,u2πc2ωVf(uexp(i(ωtkr))aˆk,u+uexp(i(ωtkr))aˆk,u+). 2

The summation for Hˆf and expression (2) include all possible values of the wave vector k and the polarization u. Next we consider a single-mode field, in which k,u has one summand with the wave vector k with polarization u. Further, for convenience we apply a system of units similar to atomic ħ = 1, m = 1, e = 1. It should be added that any suitable physical system can be an oscillator. In such a system, the charge e and the mass m depends on the problem under consideration. Therefore, everywhere below, under the oscillator interacting with the electromagnetic field, we mean any suitable physical system, the Schrodinger equation of which is described by the expression (1). Now consider expression (1) in the dipole approximation in which the vector potential, expressed in terms of field variables, is equal to Aˆ=auq, where a=4πc2ωV, ω is the frequency of the mode under consideration, V is the quantization volume, and q is the field variable of the mode. Since we are considering a single-mode electromagnetic field, it is convenient to orient the polarization vector along the x axis i.e. u = i, where i is the unit vector directed along the x axis (the same assumption applies throughout the paper).

For example, expression (1) for δ = 0 corresponds to the case of an electron in a magnetic field interacting with an external quantized electromagnetic field if the polarization of the electromagnetic field u is in the plane perpendicular to the magnetic induction vector B. This is easily obtained by using the Landau gauge30 for the magnetic field AL = Bxj, where j is the unit vector directed along the y axis.

As a result, the dynamics of the system, and electronic transitions are not determined by the stationary Schrodinger equation with the Hamiltonian

Hˆ=12(ix+βq)2+ω2(q22q2)+ωc2x22, 3

where β=4πωV. It should be clarified that expression (3) corresponds to the Hamiltonian without the variables y, z, since the wave function corresponding to the solution of equation (1) Ψ(x, y, z, q, t) = Ψ(y, z, t)Ψ(x, q, t), and this means that Ψ(y, z, t) is not a perturbed wave function and therefore does not affect the electronic transitions of the system under the action of an external electromagnetic field. Extending the argument, we replace xωcx, and the Hamiltonian (3) becomes

Hˆ=ω2(q22q2)+ωc2(x22x2)+β22q2iβωcqx. 4

We consider the nonstationary Schrodinger equation with the Hamiltonian (4). We represent the differential equation in question in the form

HˆΨ=iΨt, 5

where Hˆ=SˆHˆSˆ1 and Ψ=SˆΨ, with Sˆ being a unitary operator and Sˆ1 being the inverse operator of Sˆ (i.e. Sˆ1Sˆ=1). Finding the solution of the Schrodinger equation (5), we obtain the required wave function using the inverse transformation Ψ=Sˆ1Ψ. We seek a solution for Ψ in the form, where the operator

Sˆ=exp(iγxq)exp(iαqx). 6

It should be noted that the choice of the operator Sˆ in expression (6) is determined as a result of a careful analysis of the stationary Schrodinger equation with the Hamiltonian (4) for the possibility of its diagonalization. In expression (6), the constant values γ, α are unknown: our task now is to find values of γ, α so that the Hamiltonian Hˆ in (5) becomes diagonal.

Knowing the form of the operator Sˆ in expression (6) and using known properties of the operators (eAˆHˆeAˆ=Hˆ+[Aˆ,Hˆ]+1/2[Aˆ,[Aˆ,Hˆ]]+) it is not difficult to obtain the diagonal Hamiltonian Hˆ; all that is required is to find the appropriate parameters γ, α. As a result, we get

α=ωcω(εε2+1),γ=±12ωωc1ε2+1,ε=ω2ωc2+β2ω2βωωc. 7

When β → 0, the system must go to the initial state, for this it is necessary to use the upper sign in expression (7) (and elsewhere below) for ε > 0, and the lower sign when ε < 0. The case with ε = 0 will be considered below. As a result, the expression for Hˆ takes the form

Hˆ=ω2(Λq2σ2q2)+ωc2(1σx2κ2x2), 8
Λ=1+α2ωcω2βαωcω+β2ω,σ=11+α2ωωc,κ=σ+2βεγ2ω2βγωc(1+αγ). 9

It is not difficult to solve the Schrodinger equation with the Hamiltonian (8), since all the variables are separated. The solution for the nonstationary equation will be sought in the form Ψ(x,q,t)=n,mAn,meiEn,mtΨn,m(x,q), where HˆΨn,m(x,q)=En,mΨn,m(x,q), n,m=0,1,2, are quantum numbers, An,m are coefficients that depend on the initial conditions, and En,m are the eigenvalues of the energy. First, we write the eigenvalue of the energy of the Hamiltonian (8)

En,m=ωc(n+12)G+ω(m+12)S, 10

where

G=1βω2ωcσε2+1,S=1βωcω3/2(εε2+1)+β2ω. 11

Next, we write out the wave function of the Hamiltonian (8) in the form Ψn,m(x,q)=Ψn(x)Ψm(q), where

Ψn(x)=CneR2x2Hn(xR),Ψm(q)=Cmes2q2Hm(qs), 12

and where Hn, Hm are Hermite polynomials, R=1σκ, s=Λσ, and the normalization coefficients

Cn=12nn!πR1/4,Cm=12mm!πs1/4. 13

We then find Ψ(x,q,t)=Sˆ1Ψ(x,q,t). As a result, Ψ(x,q,t)=n,mAn,meiEn,mtΨn,m(x,q), where the wave function Ψn,m(x,q)=Sˆ1Ψn,m(x,q). The action of the operator Sˆ1 on the function Ψn,m(x,q) is not an obvious problem. For this, for example, the wave function Ψn(x) must be represented in the form of a Fourier integral Ψn(x)=12πan(p)exp(ip1σκx)dp, where for the inverse Fourier transform we obtain an(p) = Cn(−i)nexp(−p2/2) and only then and only then can the operator Sˆ1 act. As a result, we get

Ψn,m(x,q)=CnCm(i)n2πep22Hn(p)eix(pRαq)es2(q+pγR)2×Hm(s(q+pγR))dp. 14

Function (14) can be calculated analytically using the table integral35, but the result is complicated enough without doing further analysis. It will be shown later that for calculating probabilities and quantum entanglement, the analytic form of the function (14) is not required, so this calculation is not given here.

Consider the Fourier integral for the wave function Ψ(x, q, t) in the form Ψ(p,q,t)=12πΨ(x,q,t)exp(ipx)dx. After a simple calculation we find that

Ψ(p,q,t)=n,mAn,meiEn,mtΨn,m(p,q),

where

Ψn,m(p,q)=cncmin(sR)1/4e12R(pαq)2Hn(1R(pαq))×es2(q(1+αγ)γp)2Hm(s(q(1+αγ)γp)), 15

and where cn=(2nn!π)1,cm=(2mm!π)1. We show that the Fourier transform of the wave function can also be used, like the wave function itself, to calculate the probabilities. We expand the wave function in the eigenfunctions of the unperturbed system in the form Ψ(x,q,t)=m1,m2am1,m2(t)Φm1(x)eiEm1tΦm2(q)eiEm2t, where Em1,Em2 are the energy of states, with quantum numbers m1, m2, respectively, for a noninteracting oscillator in the state |m1〉 and a free electromagnetic field in the Fock state |m2〉 and am1,m2(t) is the probability amplitude for finding the system in state Φm1(x),Φm2(q) at time t. By the definition of probability wm1,m2=|am1,m2(t)|2 is the probability of detecting a system in the state m1, m2 at time t. Carrying out the Fourier transform over this decomposition (as shown above), we obtain Ψ(p,q,t) = im1m1,m2am1,m2(t)eiEm1teiEm2tΦm1(p)Φm2(q). Using the orthogonality condition, we obtain am1,m2(t) = (i)m1eiEm1teiEm2tΦm1(p)Φm2(q)|Ψ(p,q,t) = (i)m1n,mAn,meiΔEn,mtΦm1(p)eiEm1tΦm2(q)eiEm2t|Ψn,m(p,q), where ΔEn,m=En,mEm1Em2.

In order to calculate am1,m2(t) must be known An,m; these are sought from the initial conditions of the problem Ψ(p,q,0)=12πΨ(x,q,0)exp(ipx)dx. Assume that at the initial instant of time t = 0 the system was in the state Ψ(x,q,0)=Φs1(x)Φs2(q). The initial state of the system is a noninteracting oscillator in the state |s1〉 and a free electromagnetic field in the Fock state |s2〉. As a result, Ψ(p,q,0)=is1Φs1(p)Φs2(q) and using the orthogonality properties of Ψn,m(p,q)|Ψn,m(p,q)=δn,nδm,m (δn,n is the Kronecker symbol), we obtain

An,m=is1Ψn,m(p,q)|Φs1(p)Φs2(q). 16

If in the expression (16) the coefficient An,m is renamed so that it reflects information about the state from which it is calculated An,mAn,ms1,s2, we then obtain

am1,m2(t)=n,mAn,ms1,s2An,mm1,m2eiΔEn,mt. 17

Next, we make a simplification, based on the fact that the parameter β entering expression (17) is a small quantity. Indeed, for a realistic microcavity or focal volume36, this value is of the order of 10−5–10−3, although it is usually even less. It can be seen from expressions (7), (9) and (15) that the quantum entanglement of the system will be significant if the parameter ε is a finite value. Since β1, and ε is a finite quantity, we get ω ≈ ωc ≈ ω, and Δω = ω − ωc is less than or of order β. We write out expression (15) retaining the main terms under the condition β1 and ω ≈ ωc ≈ ω

Ψn,m(p,q)=incncmexp(σ2(pαq)2)×Hn(σ(pαq))exp(σ2(q+αp)2)Hm(σ(q+αp)), 18

where σ in this case will be σ = (1 + α2)−1, and α=εε2+1. The parameter α is the main parameter of the problem under consideration and α ∈ (−1, 1), and σ ∈ (1/2, 1). It should be noted that the wave function (18) can be obtained by rotating the orthogonal coordinate system [the coordinates (p, q) → (p′, q′), where p=pcosθqsinθ, and q=qcosθ+psinθ] by an angle θ corresponding to the value tgθ = α.

In order to calculate (16) with the wave function (18), the results of previous research17 must be used where an integral of this kind was calculated. As a result, we obtain

An,ms1,s2=is1n(1)s2+mαs2+mn!m!(1+α2)s1+s22s1!s2!Pm((1+s1+s2),ns2)(2+α2α2), 19

where Pa(b,c)(x) is the Jacobi polynomial. In expression (19), as was shown in the previous study in calculating the integral17, the condition s1 + s2 = m + n is fulfilled. If the condition s1 + s2 = m + n is satisfied, then m1 + m2 = m + n is executed, which means s1 + s2 = m1 + m2. This is a very important condition; as will be shown below, its use permits the calculation of the Schmidt modes.

Thus, the probability amplitude for detecting a system in the state |m1〉 |m2〉 during the evolution of the system from the state |s1〉 |s2〉 is obtained in the analytical form and is determined by the expressions (10), (19) and

am1,m2(t)=n=0s1+s2An,s1+s2ns1,s2An,s1+s2nm1,m2eiΔEn,s1+s2nt. 20

In the expression (20), up accurate to an inessential phase, ΔEn,s1+s2n for β1 can be replaced by ΔEn,s1+s2nδn, where δ=βω(α+ε). In addition, the wave function Ψ(x, q, t) is accurate to an inessential phase, and taking into account the fact that s1 + s2 = m1 + m2, it can be represented in the form

Ψ(x,q,t)=m1=0s1+s2am1,s1+s2m1(t)Φm1(x)Φs1+s2m1(q). 21

Schmidt’s Modes and Quantum Entanglement

According to Schmidt’s theorem31,32, the wave function of the system can be expanded in the form Ψ=kλkuk(x)vk(q), where uk(x) is the wave function of the pure state 1 of the system, vk(p) is the wave function of the pure state 2 of the system, and where λk is the Schmidt mode and is an eigenvalue of the reduced density matrix, i.e. ρ1(x,x)=kλkuk(x)uk(x) or ρ2(q,q)=kλkvk(q)vk(q). Having found the Schmidt mode λk, the measure of the quantum entanglement of the system can be calculated. To do this, various measures of entanglement can be used, for example, the Schmidt parameter31,32 K=(kλk2)1 or Von Neumann entropy33,34 SN=kλkln(λk). The main difficulty in calculating quantum entanglement is the search for λk for a quantum-dynamic system.

Using expression (21), the definition of the reduced density matrix can be obtained

ρ1(x,x)=m1=0s1+s2|am1,s1+s2m1(t)|2Φm1(x)Φm1(x),ρ2(q,q)=m1=0s1+s2|am1,s1+s2m1(t)|2Φs1+s2m1(q)Φs1+s2m1(q), 22

from which it follows that λk=|ak,s1+s2k(t)|2, and SN=k=0s1+s2λkln(λk).

We now present the results of quantum entanglement for the Von Neumann entropy SN. As an example, in Fig. 2 we consider the dependences of SN = SN(δt) on the dimensionless parameter for α = (1, 3/4, 1/2, 1/10, 1/100) and four variants of photon numbers s2 and oscillator s1. Calculation of entropy, for negative values of α, is not necessary, since λk is an even function λk(α) = λk(−α). From this it follows that λk, and hence the probability |am1,m2(t)|2, of detecting a system in the state |m1〉 |m2〉 is a continuous function; nonetheless, α for ε = 0 is interrupted. Indeed, if λk(α) = λk(−α), then α can be replaced by α → |α|, where |α|=ε2+1|ε|, which is a continuous function.

Figure 2.

Figure 2

The results of calculating the Von Neumann entropy SN = SN(δt) for α = (1, 3/4, 1/2, 1/10, 1/100) and (a) s1 = 0, s2 = 10; (b) s1 = 5, s2 = 10; (c) s1 = 10, s2 = 10; (d) s1 = 20, s2 = 10.

Conclusion

It can be seen from formula (20) and Fig. 2 that the entropy SN = SN(δt) is a 2π periodic function, i.e. SN(δt) = SN(δt + 2π). It is also interesting to note that when δ ~ β, the value is small; therefore, in order for the system to have a large quantum entanglement, it takes t ~ 1/β. The system will quickly go into a quantum-entangled state in the case when ωc is distinguishable from ω, but when β1 from expression (7) it is clear that α1 and γ1, so the quantum entanglement will be small. As a result, we can say that to achieve a large quantum entanglement of the system, ωc ≈ ω is necessary, with Δω = ωc − ω less or about β, but the time for large quantum entanglement must be large t ~ 1/β. In the opposite case (ωc, as distinct from ω), the system quickly becomes a quantum-entangled state, but the quantum entanglement is very small. Quantum entanglement will be a large value in the case of s1+s21, for example, when the number of photons is large. It is known that the Von Neumann entropy has the maximum value max{SN} = ln N, where N is the number of nonzero eigenvalues; in our case, therefore, max{SN} = ln(s1 + s2) (which is well illustrated by the Fig. 2). The advantage of the problem under investigation is that the quantum entanglement is not limited to the framework of the model and can take arbitrarily large values for a certain choice of s1 and s2. The presented method can be an intensive source of quantum-entangled electrons with photons. To characterize the intensity (or probability) of quantum-entanglement, the Schmidt parameter or the Von Neumann entropy is most often used. For example, if we compare the quantum entanglement on the basis of the Schmidt parameter, we get that the presented method can give more orders of magnitude more quantum entanglement than at SPDC. Indeed, the Schmidt parameter for SPDC in practice can be no more than ten37, in theory can reach several hundred38, but in our case this parameter is unlimited. For example, for s1 ~ 106 or s2 ~ 106, and also α ~ 1, the Schmidt parameter is easy to calculate and at the maximum it can reach K ~ 106. It should also be added that the study of the quantum entanglement of the system under consideration is possible only on the basis of an exact solution of the Schrodinger equation (1). Other approaches, for example, using the Jaynes-Cummings model to solve the problem under consideration would not be possible, since our task is multilevel. An experimental realization of this method of quantum entanglement of an electron with an electromagnetic field is possible. To do this, it is sufficient to place an electron in a magnetic field and irradiate such a system with a non-classical electromagnetic field. The methods for obtaining nonclassical states of the electromagnetic field are well known. In order for quantum entanglement to be essential, it is necessary to select the parameters of the electromagnetic field so that α ~ 1 (see (7)) for ω ≈ ωc, and also to choose large values of quantum numbers s1 and s2.

In summary, a system consisting of a quantum harmonic oscillator interacting with a quantized electromagnetic field has been studied. The main result of this work is that it should now be possible to obtain in an analytic form the main characteristics of such a system as well as the probability of transitions and the Schmidt mode; quantum entanglement could also be studied further using, the Von Neumann entropy, and such a system could also be used as an intensive source of quantum-entangled photons with an electron.

Acknowledgements

This work was supported by the grant of the President of the Russian Federation (grant No. MK-6289.2018.2) and the Northern (Arctic) Federal University named after M.V. Lomonosov.

Author Contributions

Dmitry N. Makarov conceived a project and it was carried out by himself.

Competing Interests

The author declares no competing interests.

Footnotes

Publisher's note: Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

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