Abstract
Leakage errors damage a qubit by coupling it to other levels. Over the years, several theoretical approaches to dealing with such errors have been developed based on perturbation arguments. Here we propose a different strategy: we use a sequence of finite rotation gates to exactly eliminate leakage errors. The strategy is illustrated by the recently proposed charge quadrupole qubit in a triple quantum dot, where there are two logical states to encode the qubit and one leakage state. We found an su(2) subalgebra in the three-level system, and by using the subalgebra we show that ideal Pauli x and z rotations, which are universal for single-qubit gates, can be generated by two or three propagators. In addition, the magnitude of detuning fluctuation can be estimated based on the exact solution.
Subject terms: Quantum information, Qubits
Introduction
The physical realization of quantum computer poses an unprecedented challenge to our capabilities of controlling the dynamics of quantum systems. While there have been many attempts to overcome this challenge, the perfect controllability of semiconducting quantum dots makes them promising candidates for universal quantum computation1–6. A universal quantum computer is the ultimate information processor in modern quantum technology, which uses quantum bits (qubits) and quantum circuits to perform computations. A qubit consists of an idealized pair of orthonormal quantum states. However, this idealization neglects other states which are typically present and can mix with those encoding the qubit. Such mixing is termed as leakage. Leakage may be the result of the application of gate operations, or induced by system-bath interactions7–13. Several strategies for combating the leakage errors have been developed for different systems, in particular the semiconducting qubit setup which is the main subject of this work, including analytic pulse shaping10,14 and optimal quantum control15,16. A general leakage-elimination method has also been presented for removing such errors by using simple decoupling and recoupling pulse sequences of the leakage elimination operator (LEO)17. Nonperturbative LEO was recently introduced for nonideal composite pulses, with emphasis on application of three-level nitrogen-vacancy centers18. It is shown that, for a three-level system, the effectiveness of LEOs does not depend on the details of the composite pulses but on the integral of the pulse sequence in the time domain. Recent studies show a significant advantage of a three-level system embedded in a triple quantum dot, which is associated with a decoherence-free subspace (DFS) of a charge quadrupole qubit19. The leakage errors are caused by noise and could be reduced by smoothly-varying short control pulses which are experimentally feasible. The system is modelled by two logical states and a leakage state coupled to one of them. Using perturbation technique and the quasistatic noise approximation, the leakage errors of single qubit operations can be suppressed by simple pulse sequences up to the sixth order in noise amplitude. While it is simple and efficient, the approach needs additional well-controlled pulses, and is only valid for small-amplitude noise. These requirements may not be well satisfied during gate operations, especially when the strength and time-dependence of noise are not negligible in comparison with other control parameters.
Here we consider exactly the same setting as in ref.19, but we are able to solve the inversion exactly by going beyond the first order approximation of that references, by using a simple sequence or circuit of finite rotations (gates). The coupling strength between the logical state and the leakage state is assumed to be static during the operation time, which is experimentally feasible for semiconducting quantum dots20–22. In comparison with the previous work based on the setup19, our solution is not restricted by the magnitude of the fluctuation and provides a clear view of the relation between the fluctuation and the error. In a more practical manner, we apply the approximation in the case when fluctuation is small and evaluate the corresponding error scales, supported by our numerical analysis. Moreover, our exact solution itself also provides an option to reckon noise strength.
Brief Introduction of the Model
We start with a model Hamiltonian represented in the basis spanned by two logical states and one leakage state19,
| 1 |
with
where we use the same notations as in the ref.19. εq and g are independent control parameters for rotations with respect to the z and x directions. Hleak stands for a coupling between the leakage state and one of the logical states, and ζ is the scaled leakage state energy in the absence of coupling23,24. A charge quadrupole (CQ) qubit is formed in three adjacent semiconducting quantum dots sharing a single electron and is embedded in the localized charge basis {|100〉, |010〉, |001〉}, where the basis states denote the electron being in the first, second or the third dot, respectively. The system Hamiltonian reads
| 2 |
where U1,2,3 are the on-site potentials for the three dots. tA,B are tunnel couplings between adjacent dots, and εd = (U1 − U3)/2 (εq = U2 − (U1 + U3)/2) denotes the dipolar (quadrupolar) detuning parameter. A new set of bases consisting of logical qubtis |C〉, |E〉 and a leakage state |L〉 is defined by19,20
| 3 |
and a schematic diagram is presented in Fig. 1. The Hamiltonian in the new basis is transformed into
| 4 |
where a term proportional to the identity has been dropped. is reduced to Eq. (1) under the conditions of ζ = 1, ξ = εd, and . In case that tA = tB and εd = 0 are satisfied, supports a decoherence-free subspace against uniform electric field fluctuations20.
Figure 1.

Schematic diagram of CQ qubits. Adjacent quantum dots are represented in blue. U1,2,3 are on-site potentials, and tA(tB) is the coupling between the left(right) and middle dots. Logical states are denoted by |C〉, |E〉 and leakage state by |L〉. The orange dots are electrons, where the full filled one means a single electron and the half filled ones represent the electron being in an equal superposition of |0〉 and |1〉.
In the triple quantum dot system, εd corresponds to an average dipolar detuning control parameter. Although εd is set to be zero, its fluctuation δεd breaks the DFS and causes leakage. It has been shown that the fluctuation of quadrupolar detuning control parameter is smaller than δεd and is thus neglected. Now we focus on the influence of δεd on the CQ qubit operations. Noise spectrum of δεd is dominated by low-frequency fluctuations which are slow in comparison with gate operations21,22. Therefore δεd is assumed to remain constant during a given gate operation19,23. As a result, unitary operators for x and z rotations can be given by
| 5 |
with arbitrary angles θ and φ. In the bang-bang limit where the control pulses switch instantaneously between two values, the angles are associated with the corresponding bang-bang gate time intervals tz and tx, which are θ = tx(2g/ℏ), φ = tz(εq/ℏ). As shown by Eq. (5), rotation operators are obviously polluted by δεd. Below, we will explain our exact solution to this problem.
Finite Rotations and Exact Elimination of Leakage
To suppress the fluctuation δεd in Ux(g, δεd, θ), we start with the following three matrices
It can be shown that their commutation relations satisfy
indicating that these operators generate an su(2) algebra. An arbitrarily given finite rotation can be represented in an exponential form25
| 6 |
where γ1, γ2, γ3 are three continuous parameters and a linear combination of Mi(i = 1, 2, 3) indicates a specific rotation axis and the corresponding angle. On the other hand, the finite rotation can also be expressed by three Euler’s angles ϕ1, ϕ2 and ϕ3,
| 7 |
The relation between the two sets of parametrizations can be found by setting
| 8 |
where the two sets ϕi and γi (i = 1, 2, 3) are in one-to-one correspondence26. Eq. (8) can be used for generators of the SU(2) group. Now we focus on the decoherence-free subspace in the triple quantum dot, and solve Eq. (8) by setting γ1 = αa, γ2 = αb, γ3 = 0, where a2 + b2 = 1. It is easy to verify that the powers of Mi satisfy
| 9 |
where n is a positive integer, I is the three dimensional identity matrix, and Δ(i) is a matrix whose ith diagonal matrix element is one and all other elements are zeros. Based on the above properties, we can derive an exact matrix equation
| 10 |
representing a system of nine nonlinear equations, among which only three equations are independent. The independent equations determine ϕ1 = ϕ3 and
| 11 |
Therefore angles ϕ1 and ϕ2 can be expressed in terms of α, a and b. Substituting Eq. (8) to Ux(g, δεd, θ), we obtain
| 12 |
where is defined by (). The parameter constraints are
| 13 |
which are obtained from Eq. (11). By reversing Eq. (12) we obtain the ideal gate operator with respect to x axis,
| 14 |
and eliminate the leakage Hleak. Notice that constrains (13) hold for any magnitude of fluctuation δεd. Therefore, one can expand constrains (13) about any specific δεd. In fact, factor δεd can be completely removed in the Taylor expansion of the above constrains. For example, when δεd is relatively small compared to g, the Taylor expansion of constraints (13) in terms of (δεd/g) can be given by
| 15 |
So, approximately one has
| 16 |
Actually, Eq. (16) correspond to the previous results19. If one applies Eq. (16) to perform an x-rotation through , only the values of θ and g are required to be set. Furthermore, the error scales of above approximate control conditions can be given by
| 17 |
where F1 and F2 denote the coefficients of (δεd/g)2 in the expansion of β1 and β2 respectively. The last step in the above expression is also based on Taylor expansion. Seen from Eq. (17), if the x-rotation is performed using Eq. (16), the terms in relation with computational and leakage error scale as (δεd/g)2 and (δεd/g)3 respectively. Therefore, the probability of computational error and leakage error scale as (δεd/g)4 and (δεd/g)6 respectively19. It is worth mentioning that the implementation of objective rotation angle β′2 depends on θ which is the multiplier of g and tx. Then one can enlarge g and shorten tx to further suppress δεd/g for the same given β′2. Besides above example, one can obtain expansions about other points rather than δεd/g = 0 by constraints (13). Due to the mathematical form of the constrains, a singular point exists. Eq. (16) indicate that the value of can be arbitrarily chosen except π. When , θ/4 = π/2 and tan(θ/4) goes to infinity. This can be solved by applying two sequences when β2′ = π/2, which does not change the error scales.
Numerical Results
We firstly show the parameter dependence of exact solution (13) by the surfaces in Fig. 2. We set g/ℏ = 3.0 GHz. tx varies from 0 to 2.0 ns and δεd/g varies from 0 to 0.6. One of our main concern is the ability of rotating a qubit about x-axis under constrains (13), which is given by the domain of β2. Seen from the lower panel of Fig. 2, which is obtained by the second constrain (13), β2 exactly changes from 0 to 2π when δεd = 0 (left subfigure in the lower panel). For the case when δεd is bigger than 0, such as 0.6g/ℏ (right subfigure in the lower panel), one can only obtain a good approximation of the δεd = 0 case when tx is small. Besides, from the upper panel which is obtained by the first constrain (13), we can see that the control parameter β1 is also insensitive to noise, except the neighbour area of singular point tx = 1.05 ns. The left (right) subfigure of the upper panel shows a sectional view of the case when δεd/g = 0 (0.6). In general, one can conclude from the above results that the circuit is insensitive to noise when control time is short. Also, an x-rotation of the CQ qubit through an arbitrary angle can be performed under constrains (13) with one or two sequences (14).
Figure 2.
Surfaces determined by exact solutions in parameter space and four specific sectional graphs. The left (right) column shows the dependence of β1 or β2 on tx when δεd/g is 0 (0.6). The middle column shows the surfaces. The upper panel is obtained by the first Eq. (13) and lower panel is obtained by the second Eq. (13). The curves when δεd/g = 0, 0.2, 0.4, 0.6 are also marked on the surfaces in order to visualize the basic trend.
Next, we show a numerical analysis of the leakage errors of our whole x rotation scheme, with the probability of leakage errors defined by PLC,LE = |〈L|U|C, E〉|2 19. We consider the cases of different types of system noise, i.e., different δεds, and the results are given by Fig. 3. g/ℏ is also set to be 3.0 GHz and β2 is set to be π/2. The control parameter β1 and θ of the circuit (14) applied in all the cases are obtained by solving constrains (13) under above conditions together with the assumption that δεd/ℏ is 0.3 GHz, no matter how it is set in the simulation of a specific evolution. The leakage probabilities are obtained from circuit (14) under quasistatic noise assumption, when system δεd/ℏ (the one used for the simulation of the evolution by the circuit) is 0.1, 0.3, 0.5, or randomly varies from 0.1 to 0.5 GHz in a multi-channel case. The results of δεd/ℏ = 0.1, 0.3, 0.5 GHz are represented by dash-dotted, triangle-dotted, and dashed curves respectively. The solid lines display the results of leakage probabilities of the multi-channel case. In such a case, more than one noise channel is calculated. The δεd/ℏ of a certain channel is static, but randomly varies from 0.1 to 0.5 GHz for different channels. The solid curves in Fig. 3 are obtained by averaging over 100 noise channels. The final leakage probabilities PLC (red curves) and PLE (blue curves) are both below 1.43 × 10−4. The infidelity 1 − F (F is the average gate fidelity27,28) in 2D logical subspace of above cases are below 9.76 × 10−6 which gives the order of the computational error. For this part of results, two conclusions can be drawn. One is that the effectiveness of the circuit (14) does not depend upon an exact knowledge of the noise amplitude. This is indicated by the good performance of the circuit (14) whose parameters are obtained by assuming a fixed value of δεd/ℏ (0.3 GHz), rather than directly using the noise information of corresponding numerical simulation of evolution (system δεd/ℏ = 0.1, 0.5 GHz and random). As for other assumptions of the value of δεd/ℏ, one can also adjust the control parameters of circuit (14) properly according to constrains (13) for a required elimination of leakage. The other is that the changing character of the leakage probabilities of the multi-channel case coincides with that of the single channel case whose system δεd/ℏ is set to be the average of the random one, indicating that multi-channel average will not disturb the effectiveness of the whole process. Therefore, one could expect a stability of circuit (14) in the potential applications.
Figure 3.

The probability of leakage error PLC (red) and PLE (blue) under quasistatic noise approximation. Each condition of the curve is demonstrated by the legend on the right. The dash-dotted, triangle-dotted, and dashed curves show the results when δεd/ℏ = 0.1, 0.3, 0.5 GHz respectively. Solid lines show the average leakage probabilities of the quasistatic noise channels with random magnitude varying from 0.1 to 0.5 GHz.
A noise-free version of constrains (13) requires Taylor expansion. So we numerically analyze an example of such approximation. We consider circuit (14) under Eq. (16). β′2 is set to be π/2. In order to evaluate a case when δεd/g is not relatively big, we set g/ℏ = 0.5 GHz. By replacing the β1 and β2 in circuit (14) by β′1 and β′2, one can calculate PLC,LE. θ and β′1 can be obtained by solving Eq. (16) in the above setup. δεd is also assumed to be constant in one rotation circuit. The results are taken by averaging over different channels where δεd/ℏ randomly varies from 0.15 to 0.45 GHz. The final values of PLC,LE are 1.63 × 10−4 and 4.01 × 10−4, and the infidelity is 2.64 × 10−5. These numbers support the effectiveness of the approximation. Also, we consider the case when δεd/ℏ in circuit (14) changes with time frequently. The simulation is performed by decomposing each exponential operator into a sufficient large number of pieces and δεd/ℏ randomly varies from piece to piece in the range of 0.15 to 0.45 GHz. The final values of average PLC,LE are 7.85 × 10−4 and 1.05 × 10−3 and the infidelity is 2.92 × 10−4, which also shows a insensitivity to the noise.
Estimation of Noise Strength
Based on our exact formula, we can estimate the strength of δεd. For a CQ qubit under noise δεd, an ideal x rotation with angle β2 is generated by experimental parameters β1, θ, g and δεd in terms of the constraints (13). In semiconducting quantum dots, gate operations are implemented by microwave pulses so that θ can be modulated by the pulse width, and g is determined by tunnel couplings tA,B. The spectrum of the noise δεd in range of 5 kHz to 1 MHz has been shown by Hahn echo curves21. Here our derivation suggests a new perspective to look into the noise δεd. An estimation of δεd can be done by following steps. (i) Prepare an initial state, for example |C〉. (ii) Perform the three operations on the right side of Eq. (14) with given g, β1 and θ which has no limitation other than the first Eq. (13). A good approximation can be obtained when g is set to be sufficiently large, such as the first Eq. (16). The resultant operation in the logical subspace is an ideal x rotation. (iii) Measure the output state, and then β2 can be given. (iv) Substitute g, θ and the measurement result of β2 to the second Eq. (13), then δεd is estimated. Our analysis in the previous sections indicates that the first Eq. (13) is mainly in relation with leakage error. So the estimation based on the second Eq. (13) in the logical subspace is little affected by the imperfect control of β1. In experiments on semiconducting quantum dots, state initialization and readout take about 4 ms to 5 ms, and state manipulation needs about 1 ms21. Therefore our estimation is allowed to be performed and repeated for several times and an effective strength curve of δεd in the time domain can be concluded.
Arbitrary Single Qubit Rotation
An arbitrary leakage-free gate can be generated by three ideal x and z rotations. While the ideal x rotation is given by (14), in what follows, we will first show how to generate the ideal z rotation. Let us start with the experimentally available Uz(εq, δεd, ϕ) in Eq. (5). By using the commutation relation [Hz, Hleak] = 0, Uz can be simply decomposed into
| 18 |
Consequently, the leakage-free z rotation can be realized by
| 19 |
is given by and φ′ = −φ/εq. Also, can be implemented by setting εq = 0. Equation (19) shows that only two different gates with the same δεd are needed for the implementation of an ideal z rotation. It does not require the detail of δεd as well.
In general, it is well-known that an arbitrary leakage-free rotation for a single qubit can be implemented by combining Uix and Uiz, i.e., three experimentally-available rotations for x axis and two for z axis, as sketched in Fig. 4. In the above rotation scheme, a conjugate of operator can also be implemented by circuits composed of the su(2) generators that correspond to the short-time evolution when εq or g is set large enough. For example, when g = εq = 12.0 GHz and noise is 0.3 GHz, Uz(0, δεd,φ) can be inverted with infidelity 4.2 × 10−3.
Figure 4.

Circuits for generating Uix and Uiz. The magnitude of applied pulses are εq and g. The operation time tz (t′z) is given through angle φ (φ′) and detuning parameter εq, and tx (t′x) is given by angles θ (β1) and the coupling parameter g.
Conclusion
We provide an exact solution to elimination of leakage errors in a three-level quantum model using simple circuits of gates. The model comprises of two logical states and a leakage state, which can be used to describe a triple quantum dot system supporting a DFS. Encoding qubits in a DFS is a well-known strategy in error suppression for quantum computation, which attracts significant attentions because of its minimal overhead requirements. The concatenation of DFS and the circuits promises to give this approach a twofold resilience, against decoherence and stochastic leakage errors. In comparison with the previous work19, our formalism is based on finite rotations and su(2) subalgebra. Reasonable approximations for application can be obtained from the formula. For example, one will trace back to the results in ref.19 by assuming the noise is relatively small. We numerically analysis the parameter dependence of the exact solution, especially the affection of the noise. Numerical simulation shows that the performance of our circuits does not rely on an accurate knowledge of the noise, and is excellent in a multi-channel model when the noise strength randomly varies from channel to channel, indicating the stability of these circuits. Furthermore we propose an estimation of dipolar detuning control fluctuation to extract strength information of noise. The feasibility of our approach is ensured by the development of sophisticated experimental techniques19,20.
Acknowledgements
We acknowledge grant support from the Spanish MINECO/FEDER Grants FIS2015-69983-P, the Basque Government Grant IT986-16 and UPV/EHU UFI 11/55.
Author Contributions
Y.S. designed the circuit, derived the major formulas and made the numerical analysis. L.-A.W. proposed the origin idea and revised the manuscript. J.-Y.Z. provided insightful advice and important support for this work.
Data Availability
The datasets generated and analysed during the current study are available from the corresponding author on reasonable request.
Competing Interests
The authors declare no competing interests.
Footnotes
Publisher’s note: Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
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Data Availability Statement
The datasets generated and analysed during the current study are available from the corresponding author on reasonable request.

