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. 2019 Nov 15;43(4):1838–1856. doi: 10.1002/mma.6007

Corrector estimates in homogenization of a nonlinear transmission problem for diffusion equations in connected domains

Victor A Kovtunenko 1,2,, Sina Reichelt 3, Anna V Zubkova 1
PMCID: PMC7027802  PMID: 32103846

Abstract

This paper is devoted to the homogenization of a nonlinear transmission problem stated in a two‐phase domain. We consider a system of linear diffusion equations defined in a periodic domain consisting of two disjoint phases that are both connected sets separated by a thin interface. Depending on the field variables, at the interface, nonlinear conditions are imposed to describe interface reactions. In the variational setting of the problem, we prove the homogenization theorem and a bidomain averaged model. The periodic unfolding technique is used to obtain the residual error estimate with a first‐order corrector.

Keywords: bidomain model, corrector estimates, diffusion problem, nonlinear transmission conditions, periodic unfolding technique

1. INTRODUCTION

We consider coupled linear parabolic equations describing the diffusion of two species in two different phases of one physical domain separated by a thin periodic interface. The coupling of the species arises via nonlinear transmission conditions at the interface, which model surface reactions. Nonlinear interface reactions are relevant, for instance, in electrochemistry, see, eg, Landstorfer et al1 for adsorption and solvation effects at metal‐electrolyte interfaces, and Efendiev et al2 for electro‐chemical reactions in lithium‐ion batteries.

The characteristic length scale of the periodic cell is given by the homogenization parameter ε>0. The main objective is to derive a macroscopic model for vanishing ε, where both phases are connected sets. The limit bidomain model is given via two coupled parabolic equations defined in the macroscopic domain describing the diffusion of the two species in each phase and reactions at the interface. In the case of connected‐connected domains, we exploit the existence of a continuous extension operator from the periodic domain to the whole domain following.3, 4

A qualitative homogenization result for reaction‐diffusion systems with nonlinear transmission conditions has recently been obtained in Gahn et al.5 The limit in the microscopic equations is derived rigorously in the sense of the two‐scale convergence, however, without corrector estimates. There also exists a vast literature on transmission problems with linear interface conditions, eg, Donato et al6 and Donato and Monsurro.7 See references therein for the case of elliptic equations as well as the extensions of the homogenization result to parabolic equations in Jose8 and to nonlinear monotone transmission conditions in Donato and Le Nguyen.9 For the treatment of oscillating third boundary conditions, we refer to Belyaev et al10 and Oleinik and Shaposhnikova.11

Within elecktrokinetic modeling (see Allaire et al12), in previous studies,13, 14, 15, 16 there were considered generalized Poisson‐Nernst‐Planck (PNP) models over two‐phase domains accounting for interface reactions. The corresponding PDE system obeys a structure of the gradient flow; see, eg, other works.17, 18, 19 The paper20 considers the homogenization over a two‐phase domain for static PNP equations and homogeneous interface conditions. In Kovtunenko and Zubkova,21 residual error estimates for the averaged monodomain solution with first‐order correctors were justified under the simplifying assumption that the flux across the interface is of order O(ε 2).

In this paper, however, we are mainly interested in quantitative asymptotic results supported by corrector estimates. There exist many articles on the derivation of error estimates for different classes of reaction‐diffusion systems, eg, other works,22, 23, 24, 25 exploiting a higher regularity of the limit solution and the continuous extension operator from a perforated domain. Moreover, unfolding‐based error estimates have been proven for linear, elliptic transmission problems in Reichelt,26 for reaction‐diffusion systems with linear boundary conditions in perforated domains in Muntean and Reichelt,27 and for systems with nonlinear interface conditions in a two‐phase domain in Fatima et al.28 The latter results are based on the quantification of the periodicity defect for the periodic unfolding operator in Griso,29, 30 and they hold without assuming higher regularity for the corrector problem.

Our approach uses the periodic unfolding method introduced in Cioranescu et sl31 and further refined in Franců32 and Mielke and Timofte.33 To make our error estimates rigorous, we have to assume higher regularity for the limit solutions as well as for the correctors solving the local cell problems. This additional regularity for the limit problem is in line with established homogenization results by, eg, literature.34, 35, 36 Our result provides residual error estimates with a first‐order corrector of order ε , which is (generally) optimal for H 1‐estimates up to an Lipschitz boundary, whereas in Fatima et al,28 the error is of order ε 1/4. For this task, we apply the Poincaré inequality in periodic domains (see Lemma 2) and the uniform extension in connected periodic domains (see Lemma 3).

The paper is structured as follows: In Section 2, we formulate the transmission problem and all relevant assumptions. In Section 3, we prove the existence of solutions to our model and provide a priori estimates. In Sections 4 and 5, we define the periodic unfolding operator and provide important properties as well as first asymptotic results. In Section 6, we state and prove our main result on the residual error estimates.

2. SETTING OF THE TRANSMISSION PROBLEM

For a fixed homogenization parameter ε>0, we consider a macroscopic domain Ω consisting of two subsets Ω1ε, Ω2ε, which are disjoint by a thin interface Γε. The both components Ωiε are assumed to be connected such that |ΩiεΩ|0. By |ΩiεΩ|, we mean the surface measure of points where the boundaries of Ωiε and Ω will meet.

We make the following geometric assumptions.

  • (D1)
    The reference domain ΩRd is a d‐dimensional hyperrectangle, d2, ie, it is
    Ω=k=1d(ak,bk),ak<bkandak,bkR.
    This assumption suffices to split Ω into periodic cells in (D3).
  • (D2)
    The unit cell Y=(0,1)d consists of two open, connected subsets Y 1 and Y 2, which have Lipschitz continuous boundaries ∂Y 1, ∂Y 2 and are disjoint by the interface Γ=∂Y 1∂Y 2. We assume the reflection symmetry, ie,
    Yi{yk=0}=Yi{yk=1}
    for k=1,…,d, i=1,2. This assumption allows us to define periodic functions on Y i in (29). Let n 1 and n 2 denote the unit normal vectors at the respective boundaries ∂Y 1 and ∂Y 2. Every normal is chosen outward from the domain, and it does not depend on scaling by ε.
  • (D3)
    For ε>0, we introduce the decomposition of a point xRd as
    x=εxε+εxε (1)
    into the floor part xεZd and the fractional part xεY. According to (1), let the set of integer vectors
    Iε={λZd|ε(λ+y)Ωfor allyY}
    denote the numbering of local cells inside Ω. We call ε an admissible parameter, if the reference domain Ω from (D1) can be partitioned periodically into the local cells as follows:
    Ω=λIεε(λ+Y). (2)
    For a treatment of small boundary layers, see Reichelt.37, lemma 2.3.3
  • (D4)
    As a consequence of (D1) to (D3), the periodic components Ω1ε and Ω2ε and their interface Γε are determined via
    Ωiε=λIεYiλ,Yiλ=ε(λ+Yi),Γε=Ω1εΩ2ε. (3)
    By this, the outward normal vectors niε at Ωiε coincide with the normal vectors n i at ∂Y i for i=1,2 and do not depend on the scaling ε. The interface Γε is a Lipschitz continuous manifold.

For admissible ε>0, time t∈(0,T) with the final time T>0 fixed, the space variable xΩ1εΩ2ε in the two‐component domain, we consider a nonlinear transmission problem for uiε(t,x), i=1,2, such that

tuiεdiv(Aiεuiε)=0inΩiε, (4a)
Aiεuiε·ni=εgi(u1ε,u2ε)onΓε, (4b)
uiε=0onΩiεΩ, (4c)
uiε=uiinast=0. (4d)

The notation t stands for the time derivative, ∇ for the spatial gradient, and   · ′′ for the scalar product in Rd. Below, we explain in detail the terms entering the system (4). We note that |Γε|=O(1/ε); therefore, the scaling ε in (4b) appears naturally just compensating the longer interface.

  • (A1)
    The diffusivity matrices Ai(y)L(Yi;Rsymd×d), i=1,2, are symmetric, uniformly bounded and elliptic: There exist 0<αβ such that
    α|ξ|2Ai(y)ξ·ξβ|ξ|2for allξRd,a.e.yYi. (5)

The matrices entering (4a) to (4c) are defined as Aiε(x)=Ai{xε} according to the notation (1) and are assumed to be periodic.

In the transmission conditions (4b), the functions gi:R2R, i=1,2, describe interface reactions and are assumed to satisfy

  • (G1)
    the uniform growth condition: there exists K g>0 such that
    |gi(u1,u2)|Kg,for allu1,u2R; (6)
  • (G2)
    the Lipschitz continuity: There exists Lg0 such that
    |gi(u1,u2)gi(v1,v2)|Lg|u1v1|+|u2v2|, (7)
    for all ui,viR, i=1,2.

The linear diffusion equations (4a) are supported by the standard, homogeneous Dirichlet boundary conditions (4c) and the initial data (4d) for given uiinL2(Ω), i=1,2.

We introduce the variational formulation of the problem (4) as follows: find uiεUiε, i=1,2, in the search (solution) space

Uiε={uC(0,T;L2(Ωiε))L2(0,T;H1(Ωiε)):tuL2(0,T;H1(Ωiε)),u=0onΩiεΩ},

satisfying the initial condition (4d) and the nonlinear equation

0Ttuiε,viΩiε+ΩiεAiεuiε·vidxdt=0TΓεεgi(u1ε,u2ε)vidσxdt, (8)

for all test functions v i from the test space

Viε:={vL2(0,T;H1(Ωiε)),v=0onΩiεΩ}.

The notation H1(Ωiε) in Uiε stands for the topologically dual space to H1(Ωiε), and ·,·Ωiε denotes the duality between them.

3. WELL‐POSEDNESS

This section provides the existence of weak solutions in the sense of variational formulation for the microscopic problem (8).

Theorem 1

(Well‐posedness)

  • (i)
    The unique solution uiεUiε to the nonlinear transmission problem (8) exists and satisfies the following a priori estimate:
    uiεUiε2:=uiεC(0,T;L2(Ωiε))2+uiεL2(0,T;H1(Ωiε))2+tuiεL2(0,T;H1(Ωiε))2C1uiinL2(Ωiε)2+C2Kg2+C3,C1,C2,C30, (9)
    uniformly in ε∈(0,ε 0) for ε 0>0 sufficiently small.
  • (ii)
    Under assumptions on positivity of the initial data uiin>0 everywhere in Ω, the solution uiε is positive at least locally in time, and uiε0 at any time under the assumption of the positive production rate from RoubÍček38:
    gi(u1ε,u2ε)(uiε)=0, (10)
    where (uiε)=min(0,uiε) stands for the negative part of the function.
  • (i)

    To prove existence of the solution, we apply the Tikhonov‐Schauder fixed point theorem. We iterate (8) starting with the suitable initialization uim0=uiin, m0N, i=1,2.

    For m>m 0, mN, a solution uimUiε can be found, which satisfies the initial data (4d) and the linearized equations
    0Ttuim,viΩiε+ΩiεAiεuim·vidxdt=0TΓεεgim1vidσxdt, (11)
    for all test functions viViε, using the notation gim1:=gi(u1m1,u2m1) for short. We can test (11) with vi=uim leading to
    0Ttuim,uimΩiε+ΩiεAiεuim·uimdxdt=0TΓεεgim1uimdσxdt. (12)
    We estimate the integral in the right‐hand side of (12) applying weighted Young inequality with a weight 2δKtr>0, the trace theorem (25) below, and the growth condition (6):
    0TΓεεgim1uimdσxdtδεKtr0TΓε(uim)2dσxdt+εKtr4δ0TΓε(gim1)2dσxdtδuimL2(0,T;H1(Ωiε))2+C, (13)
    where C=Ktr4δKg2Tε|Γε|=O(1) with a constant K tr from the trace theorem (25) and K g from (6). Expressing the first term in the left‐hand side of (12) by the chain rule as tuim,uim=12ddtuimL2(Ωiε), using the uniform ellipticity (5) of Aiε and the estimate (13), this follows
    12ddt0TΩiε(uim)2dxdt+(αδ)uimL2(0,T;L2(Ωiε))d2δuimL2(0,T;L2(Ωiε))2+C. (14)
    For δ<α, applying Grönwall inequality, we obtain
    uim(t)L2(Ωiε)2+CδuiinL2(Ωiε)2+Cδe2δtfort(0,T), (15)
    and taking in (14) the supremum over t∈(0,T), we conclude
    uimL(0,T;L2(Ωiε))2+uimL2(0,T;H1(Ωiε))2C1uiinL2(Ωiε)2+C2Kg2+C3,C1,C2,C30.
    Hence, using (6) from (12), it follows tuimL2(0,T;H1(Ωiε))2=O(1) uniformly with respect to m and ε→0, and the continuous embedding of the solution in C(0,T;L2(Ωiε)) holds; see Dautray and Lions.39, p509
    Therefore, the mapping M:UiεUiε defined when solving (11) has compact image, and hence, there exists an accumulation point uiεUiε, i=1,2, and a subsequence still denoted by m such that as m
    uimuiεweakly inUiεanduimuiεstrongly inL2(0,T;L2(Γε)).
    The continuity of M in the weak topology is justified using the Lipschitz continuity of the nonlinear term g i in (7). Applying the fixed point theorem40, section 4.8, theorem 8.1, p293 and the a priori estimate (9) proves the existence of a weak solution of problem (8).
    To prove uniqueness, we consider the difference wiε:=ui1,εui2,ε, i=1,2, of two solutions of (8) with the test function vi=wiε:
    12Ωiε(wiε)2t=0Tdx+0TΩiεAiεwiε·wiεdxdt=Igiε,Igiε:=0TΓεεgi(u11,ε,u21,ε)gi(u12,ε,u22,ε)wiεdσxdt. (16)
    The integral Igiε is estimated due to the Lipschitz continuity (7) as
    |Igiε|εLg0TΓε(|w1ε|2+|w2ε|2)wiεdσxdt. (17)
    Then, collecting the expressions (16) and (17), applying the Cauchy‐Schwarz and Grönwall inequalities, we get
    i=12wiε(t)2i=12wiε(0)2e4KtrLgt=0
    and hence conclude wiε0, which proves ui1,εui2,ε.
  • (ii)
    To prove the nonnegativity of uiε, we decompose the solution into the positive and the negative parts as: uiε=(uiε)+(uiε) and substitute it in the Equation (8) with the test function vi=(uiε). The assumption of the positive production rate (10) together with the uniform ellipticity (5) of Aiε and the nonnegativity of the initial data lead to the estimate:
    supt(0,T)12Ωiε((uiε))2dx+α(uiε)L2(0,T;L2(Ωiε))d212Ωiε((uiε))2t=0dx=0;
    hence, (uiε)0 and uiε0. If uiε(0)=uiin>0 everywhere in Ω, then uiε(t)>0 at least for t sufficiently small, which follows by the continuity of the solution. This completes the proof.

We note that Theorem 1 can be extended for inhomogeneous diffusion equations (4a), where the uniform upper bound is proved in Gurevich and Reichelt41 for reaction functions distributed over domains Ωiε.

4. PERIODIC UNFOLDING TECHNIQUE

Following Cioranescu et al,42 we recall the technique based on the periodic unfolding and averaging operators providing continuous mappings between the components Ωiε and Yi, i = 1,2, up to the boundaries.

Definition 1

For u(x)L2(Ωiε), the unfolding operator Tε:L2(Ωiε)L2(Ω;L2(Yi)), i=1,2, in the domain is defined by

(Tεu)(x,y):=uεxε+εy,forxΩandyYi, (18a)

and for u(x)L2(Ωiε), the operator Tε:L2(Ωiε)L2(Ω;L2(Yi)), i=1,2, is performed on the boundary by

(Tεu)(x,y):=uεxε+εy,forxΩandyYi. (18b)

For φ(x,y)∈L 2(Ω;L 2(Y i)), the averaging operator Tε1:L2(Ω;L2(Yi))L2(Ωiε), i=1,2, in the domain is defined by

(Tε1φ)(x):=1|Y|Yiφεxε+εz,xεdz,forxΩiε, (19a)

and for φ(x,y)∈L 2(Ω;L 2(∂Y i)), the operator Tε1:L2(Ω;L2(Yi))L2(Ωiε), i=1,2, on the boundary is expressed by

(Tε1φ)(x):=1|Y|Yiφεxε+εz,xεdz,forxΩiε. (19b)

Abusing the notation Tε1 is used for a left inverse operator of T ε according to Lemma 1 (i), which is also right inverse in the special cases accounting in Lemma 1 (ii). For those functions that belong to H1(Ωiε), the restriction of the unfolding operator T ε is well‐defined as the mapping H1(Ωiε)L2(Ω;H1(Yi)), and for functions in L 2(Ω;H 1(Y i)), the restriction of the averaging operator Tε1 is well‐defined as L2(Ω;H1(Yi))H1(λIεYiλ), where Yiλ is from (3). We note that the spaces H1(λIεYiλ) and H1(Ωiε) do not coincide because functions from H1(λIεYiλ) are discontinuous while they can have jumps across the interface Γε.

The operator properties are collected below in Lemma 1.

Lemma 1

(Properties of the operators Tε and Tε1) For arbitrary xu(x)H1(Ωiε)L2(Ωiε) and (x,y)↦φ(x,y)∈L 2(Ω;H 1(Y i)∩L 2(∂Y i)), i=1,2, and the extension by zero: ū(x)=u(x) for xΩiε, otherwise ū(x)=0 for xΩΩiε, the following properties hold:

  • (i)

    invertibility of T ε: (Tε1Tε)u(x)=u(x);

  • (ii)
    invertibility of Tε1:
    • (iia)
      (TεTε1φ)(x,y)=φ(y) for x∈Ω, if φ(y) is a constant or periodic function of the argument yY i,
    • (iib)
      (TεTε1ū)(x,·)=(Tε1ū)(x)=|Yi||Y|TεuYi(x) for x∈Ω, where is the average ·Yi=1|Yi|Yi(·)dy;
  • (iii)

    composition rule: Tε(F(u))(x,y)=F(Tεu)(x,y) for any elementary function F;

  • (iv)

    chain rules: εT ε(∇u)(x,y)=∇y(T ε u)(x,y), and (Tε1φ)(x)=Tε1(φ+1εyφ)(x) for xYiλ and φH 1(Ω×Y i);

  • (v)
    integration rules:
    Ωiεu(x)dx=1|Y|Ω×Yi(Tεu)(x,y)dxdy, (20a)
    Ωiεu(x)dσx=1ε|Y|Ω×Yi(Tεu)(x,y)dxdσy; (20b)
  • (vi)
    boundedness of T ε:
    Ωiεu2(x)dx=1|Y|Ω×Yi(Tεu)2(x,y)dxdy, (21a)
    Ωiε|u|2(x)dx=1ε2|Y|Ω×Yi|y(Tεu)|2(x,y)dxdy, (21b)
    Ωiεu2(x)dσx=1ε|Y|Ω×Yi(Tεu)2(x,y)dxdσy. (21c)

The property (iib) follows in a straightforward manner from the calculation of (TεTε1ū)(x,z)=(Tε1ū)(x) for x∈Ω and zY:

1|Y|Yiūεεxε+εzε+εydy=1|Y|Yiūεxε+εydy=Tε1ū(x)

and the fact that Tε1ū=|Yi||Y|TεuYi as a consequence of the definition (19a) if φ(x,y)ū(x) for all φ(x,y)∈L 2(Ω;H 1(Y i)). The proof of the other properties can be found in other studies.20, 21, 31, 42, 43

5. ASYMPTOTIC ANALYSIS

In this section, we collect some auxiliary tools used later in the derivation of the residual error estimates.

Lemma 2

(Poincaré inequality in periodic domains) For u(x)H1(Ωiε), the following Poincaré inequality holds (see, eg, Cioranescu et al42, 43):

uTεuYiL2(Ωiε)2ε2KPuL2(Ωiε)d2,KP>0. (22)

We recall the Poincaré inequality for a function φ(y)∈H 1(Y i) in the unit cell with connected subsets Y i for i=1,2:

Yi(φφYi)2dyKPYi|yφ|2dy,φYi:=1|Yi|Yiφ(y)dy. (23)

Integrating (23) over Ω yields

Ω×Yi|φφYi|2dxdyKPΩ×Yi|yφ|2dxdy

for all φL 2(Ω;H 1(Y i)). Choosing φ=T ε u gives

1|Y|Ω×Yi|TεuTεuYi|2dxdyKP|Y|Ω×Yi|y(Tεu)|2dxdy=KPε2uL2(Ωiε)2.

For the left‐hand side, we use the composition rule (iii) as well as TεTεuYi=TεuYi. For all (x,y)∈Ω×Y i, we have

TεTεuYi(x,y)=Tε(x,z)1|Y|Yiuεxε+εzdz(x,y)=1|Y|Yiuεεxε+εyε+εzdz=1|Y|Yiuεxε+εzdz=TεuYi(x),

while noting that εxε+εyε=xε for all y∈(0,1)d. This shows, in particular, that yTεTεuYi(x,y) is constant for a.e. x∈Ω.

We recall the trace theorem in unit cells for a function φL 2(Ω;H 1(Y i)):

φL2(Yi)2Ktr(φL2(Yi)2+yφL2(Yi)d2)=KtrφH1(Yi)2, (24)

with K tr>0. After the substitution of φ=T ε u for the function u(x)H1(Ωiε), there follows (see, eg, Monsurrò44):

uL2(Ωiε)2Ktr1εuL2(Ωiε)2+εuL2(Ωiε)d2. (25)

In particular, repeating the arguments in the proof of Lemma 2, the trace inequality in periodic domains can be shown:

uTεuYiL2(Ωiε)2εKtr(1+KP)uL2(Ωiε)d2. (26)

Lemma 3

(Uniform extension in connected periodic domains) For u(x)H1(Ωiε), there exists a continuous extension ũH1(Ω) from the connected set Ωiε to Ω such that ũ=u in Ωiε and

ũL2(Ω)2KeuL2(Ωiε)2,ũL2(Ω)d2KeuL2(Ωiε)d2,Ke>0. (27)

If u=0 on ΩiεΩ, then ũH01(Ω) exists satisfying (27).

Indeed, the assertion holds in accordance with previous studies,3, 4, 45, chapter 4 and the zero trace at the boundary Ω is argumented in Höpker.46, theorem 3.5

Below, we recall the auxiliary result from Fellner and Kovtunenko20, lemma 2 and Kovtunenko and Zubkova.21, lemma 4.1

Lemma 4

(Asymptotic restriction from Ω to Ωiε) For given functions u,vH 1(Ω) (which have no jumps across the interface Γε), the asymptotic estimate

Ωiεuvdx|Yi||Y|ΩuvdxεKruH1(Ω)vH1(Ω),Kr>0, (28)

holds as ε→0 for i=1,2.

Based on the geometric assumptions (D1) to (D4), we define the space of periodic functions in the cells Y i by

H#1(Yi):={φH1(Yi):φ(y)|yj=0=φ(y)|yj=1,j=1,,d,foryYiY}. (29)

We set the standard cell problem determining Ni=(N1i,,Ndi)(y), i=1,2, from

divyAi(yNi+I)=0inYi, (30a)
Ai(yNi+I)ni=0onΓ, (30b)
(yNi+I)Ai|yk=0=(yNi+I)Aiyk=1,Ni|yk=0=Ni|yk=1fork=1,,d, (30c)

where the last line in (30c) implies that NkiH#1(Yi) for i=1,2 and k=1,…,d. In (30), the notation yNi(y)Rd×d for yY i stands for the matrix of derivatives with entries (yNi(y))kl=Nkiyl, k,l=1,…,d, and IRd×d denotes the identity matrix. The system (30) admits the weak formulation: find vector‐functions NiH#1(Yi)d such that

YiAi(yNi+I)yφdy=0, (31)

for all test functions φH#1(Yi). A solution of (31) exists, and it is defined up to a constant in Y i.

Based on the solution N i of the cell problem (31), the diffusivity matrices A i admit the following asymptotic representation formulated in the lemma below; see Fellner and Kovtunenko20 and Kovtunenko and Zubkova.21

Lemma 5

(Asymptotic formula for periodic diffusivity matrices)

  • (i)
    For the solution N i of the cell problem (31), the following representation holds:
    Ai(y)(yNi(y)+I)=Ai0+Bi(y), (32)
    with Ai0Rsymd×d given by the averaging
    Ai0:=Ai(yNi+I)Yi, (33)
    and it is a symmetric d‐by‐d matrix:
    There existsa_00such thatξA0ξa_0|ξ|2forξRd. (34)
    The d‐by‐d matrix B i(y) is periodic and has the following divergence form in the cell Y i:
    (Bi)kl=m=1dbklm,m(i),k,l=1,,d,wherebklm,m(i)=bklm(i)ym.
    Its components bklm(i) are skew‐symmetric:
    bklm(i)+bkml(i)=0,k,l,m=1,,d,
    the matrix B i is divergence‐free:
    l,m=1dbklm,lm(i)=0withbklm,lm(i)=2bklm(i)ylym,
    and the average BiYi=0. At the interface, the condition holds:
    (Ai0+Bi)ni=0onΓ. (35)
  • (ii)
    Assume that N iW 1,(Y i)d. For varying function viViε and fixed ui0L2(0,T;H3(Ω)), the following integral form corresponding to the averaged equation (50):
    IAi0:=ΩiεAi0ui0·vidxΓεAi0ui0·nividσx (36)
    with the help of the corrector ui1:=ui0+ε(Tε1Ni)·ui0 is approximated as follows:
    Err0(vi,ε):=0TIAi0ΩiεAiεui1·vidxdt,|Err0(vi,ε)|εKAiL(Yi)NiL(Yi)d+yNiL(Yi)d×d+1ui0L2(0,T;H3(Ωiε))viL2(0,T;H1(Ωiε)),K>0. (37)
  • (i)

    For the vector‐valued solution N i of (31), the representation (32) follows from the Helmholtz theorem; see Zhikov et al.36, section 1.1 The interface condition (35) is obtained after substitution of (32) into (30b).

  • (ii)
    Let viViε and ui0L2(0,T;H3(Ω)) be given. To prove (37), we rewrite IAi0 in (36) in virtue of the integration rules from Lemma 1 in the microvariable y:
    IAi0=1ε2|Y|Ω×Yi(TεAi0)y(Tεui0)·y(Tεvi)dxdyΩ×Γ(TεAi0)y(Tεui0)·ni(Tεvi)dxdσy. (38)

For the constant matrix, the identity Ai0=TεAi0 holds. Then, expressing Ai0 from (32), using the product rule

yNiy(Tεui0)=y(Ni·y(Tεui0))y(y(Tεui0))Ni,

the chain rule εTε(ui0)=y(Tεui0), and the notation of the corrector ui1:=ui0+ε(Tε1Ni)·ui0, we rearrange the following terms:

(TεAi0)y(Tεui0)=(Ai+Ai(yNi)Bi)y(Tεui0)=Aiy(Tεui1)Aiy(y(Tεui0))NiBiy(Tεui0).

Taking into account this formula, IAi0 is performed equivalently by

IAi0=1ε2|Y|Ω×YiAiy(Tεui1))·y(Tεvi)Aiy(y(Tεui0))Ni·y(Tεvi)dxdyΩ×ΓAi0y(Tεui0)·ni(Tεvi)dxdσy+IBi, (39)

with the integral IBi is written component‐wisely as follows:

IBi:=1ε2|Y|Ω×YiBiy(Tεui0)·y(Tεvi)dxdy=1ε2|Y|Ω×Yik,l,m=1dbklm,m(i)(Tεui0),k(Tεvi),ldxdy.

Recalling the definition of B i and the fact that it is divergence‐free, the term IBi is integrated by parts as follows:

IBi=1ε2|Y|Ω×Yik,l,m=1dbklm,m(i)(Tεui0),kl(Tεvi)dxdy1ε2|Y|Ω×YiBiy(Tεui0)·ni(Tεvi)dxdσy. (40)

After substitution of (40) in (39), the integral over Γ disappears due to the interface condition (35). The integral over ∂Y i∖Γ vanishes after rewriting the integral again in macrovariables because of v i=0 on ΩiεΩ and because jumps across the cell boundary of v i and ui0 are zero (by assumed H 3‐, hence, C 1‐smoothness of ui0), while B i is periodic.

The integral over Ω×Y i in (40) can be rewritten using the zero average BiYi=0 as follows:

1ε2|Y|Ω×Yik,l,m=1dbklm,m(i)(Tεui0),kl(Tεvi)dxdy=I1i+I2i,

where

I1i:=1ε2|Y|Ω×Yik,l,m=1dbklm,m(i)(Tεui0),kl(TεviTεviYi)dxdy,
I2i:=1ε2|Y|Ω×YiTεviYik,l,m=1dbklm,m(i)[(Tεui0),kl(Tεui0),klYi]dxdy.

We rewrite I1i and I2i in the macrovariable x in all local cells using the integration rules (20) and (21) and then apply to the result the Cauchy‐Schwarz inequality and the Poincaré inequality (23).

Below, the indices k,l,m will refer to both x as well as y coordinates. We are starting from

I1i=1ε2|Y|Ω×Yik,l,m=1dTε(Tε1bklm,m(i))(Tεui0),klTε(viTεviYi)dxdy=Ωiεk,l,m=1dεTε1bklm(i),mui,kl0(viviYiλ)dx,

where it is for all xΩiε:

TεviYi(x)=1|Yi|Yiviεxε+εzdz=1|ε(λ+Yi)|ε(λ+Yi)vizdz=viYiλ(x)

with λ=xε. First, there are some constants 0<K1K2 such that

|I1i|=λIεYiλk,l,m=1d(εTε1bklm,m(i))ui,kl0(viviYiλ)dxK1BiL(Yi)d×dui0H2(Ωiε)εviL2(Ωiε)dεK2(AiL(Yi)d×dyNiL(Yi)d×d+1)ui0H2(Ωiε)viL2(Ωiε)d. (41)

Similarly, there exists K 3>0 such that

|I2i|K3(AiL(Yi)d×dyNiL(Yi)d×d+1)k,l=1dε(ui,kl0)L2(Ωiε)dviL2(Ωiε). (42)

We substitute in (39) the expression of IB1 from (40) and use (35), such that

IAi01ε2|Y|Ω×YiAiy(Tεui1)·y(Tεvi)dxdy=1ε2|Y|Ω×YiAiy(y(Tεui0))Ni·y(Tεvi)dxdy+I1i+I2i. (43)

Rewriting the integrals in microvariables with the help of the integration rules (20) and (21), the following estimate takes place with K 4>0:

IAi0ΩiεAiεui1·vidx|I1i|+|I2i|+εK4AiL(Yi)d×dNiL(Yi)dui0H2(Ωiε)viL2(Ωiε)d. (44)

Using the estimates (41) and (42), from (44) after integration over time, it follows (37) that proves the assertion of Lemma 5.

With these preliminaries, in the next section, we homogenize the nonlinear transmission problem (8) as ε→0.

6. THE MAIN HOMOGENIZATION RESULT

We state the averaged bidomain diffusion problem determining the functions ui0(t,x), i=1,2, in the time‐space domain (0,T)×Ω from

tui0div(Ai0ui0)=|Γ||Yi|gi(u10,u20)inΩ, (45a)
ui0=0onΩ, (45b)
ui0=uiinast=0, (45c)

where the effective matrices Ai0 are defined in (33). It implies the variational formulation: find ui0U0 in the space

U0={uL(0,T;L2(Ω))L2(0,T;H1(Ω)):tuL2(0,T;H1(Ω)),u=0onΩ},

such that it satisfies the initial condition (45c) and the following nonlinear equation:

0Ttui0,vΩ+ΩAi0ui0·v|Γ||Yi|gi(u10,u20)vdxdt=0, (46)

for all text functions vV0:=L2(0,T;H01(Ω)). In (46), the notation ⟨·,·⟩Ω implies the duality between H 1(Ω) and its topologically dual space H 1(Ω).

The solvability of (46) can be obtained in the same way as for (8) due to the uniform boundedness (6) and the continuity (7) of the nonlinear term g i. Moreover, the a priori estimate like (9) holds (for i=1,2):

ui0U02C1uiinL2(Ω)2+C2Kg2+C3.

In Theorem 2, we need smoothness of the macroscopic solution and the uniform boundedness of N i and of its gradient in order to prove the residual error estimate, which is a standard assumption for cell problems; see, ie, Zhikov et al.36, section 5.6, theorem 5.10 These assumptions might be weekend just to get a two‐scale convergence to the homogenized problem.

Theorem 2

(Residual error estimate) Let the cell problem (31) obey the Lipschitz continuous solution N iW 1,(Y i), and the macroscopic solution be such that ui0L2(0,T;H3(Ω))L(0,T;H1(Ω)), t(ui0)L2(0,T;L2(Ωiε))d, i=1,2. Then the solution uiε of the inhomogeneous problem (8) and the first‐order corrector to the solution ui0 of the averaged problem (46) given by

ui1=ui0+ε(Tε1Ñi)·ui0inΩ, (47)

where ÑiW1,(Y) is a periodic extension of N i to Y, satisfy the residual error estimate:

uiεui1Uiε2Err12(ε)=O(ε), (48)

where Err12 is determined in (66).

We start with derivation of an asymptotic equation for the difference uiεui1 (see (51)). Multiplying the diffusion equation (45a) with a test function viViε, integrating it over (0,T)×Ωiε, it follows the variational equation in two subdomains for i=1,2:

0Ttui0,viΩiεΩiεdiv(Ai0ui0)+|Γ||Yi|gi(u10,u20)vidxdt=0. (49)

The integration by parts in (49) due to the Dirichlet condition (45b) leads to

0Ttui0,viΩiε+ΩiεAi0ui0·vidxΓεAi0ui0·nividσxdt=0TΩiε|Γ||Yi|gi(u10,u20)vidxdt. (50)

We choose vV0 and viViε. With a special choice of v i, it can be equal to v. For test functions vi=vV0Viε, i=1,2, we subtract (50) from the inhomogeneous equation (8):

0Tt(uiεui0),vΩiε+ΩiεAiεuiεAi0ui0·vdx+ΓεAi0ui0·nivdσxdt=0TΓεεgi(u1ε,u2ε)vdσxΩiε|Γ||Yi|gi(u10,u20)vdxdt

and gather the terms as follows:

0Tt(uiεui1),vΩiε+ΩiεAiε(uiεui1)·vdxdtIi(v)=k=03Errk(v,ε), (51)

where the following notation was used

Ii(v):=0TΓεεgi(u1ε,u2ε)vdσx|Γ||Y|Ωgi(u11,u21)vdxdt. (52)

Err0 is given by the formula (37) from Lemma 5, and other residual error functions Errk, k=1,2,3, in the right‐hand side of (51) will be introduced and estimated next.

We use the Cauchy‐Schwarz inequality and the expansion of the time‐derivative of the corrector tui1=t[ui0+ε(Tε1Ni)·ui0] implying that

Err1(v,ε):=0Tt(ui1ui0),vΩiεdt,|Err1(v,ε)|tui1tui0L2(0,T;H1(Ωiε))vL2(0,T;H1(Ωiε))εNiL(Yi)dt(ui0)L2(0,T;H1(Ωiε))dvL2(0,T;H1(Ωiε)). (53)

Applying to gi(u10,u20)v the restriction operator from Lemma 4, then using the boundedness (6) and the Lipschitz continuity (7) for g i leads to

Err2(v,ε):=0T|Γ||Yi|Ωiεgi(u10,u20)vdx|Γ||Y|Ωgi(u10,u20)vdxdt|Err2(v,ε)|εK6KgvL2(0,T;H1(Ω)),K6=Kr|Γ||Yi|T|Ω|, (54)

and the further error function (with K 7=|Γ|L g)

Err3(v,ε):=|Γ||Y|0TΩ(gi(u11,u21)gi(u10,u20))vdxdt,|Err3(v,ε)||Γ|Lg|Y|j=12uj1uj0L2(0,T;L2(Ω))vL2(0,T;L2(Ω))εK7j=12ÑjL(Y)duj0L2(0,T;L2(Ω))dvL2(0,T;L2(Ω)). (55)

In the following, we aim at substitution of v by piecewise constant average Tεv(x):=TεvYj(x) for xΩjε, j=1,2. For this task, we decompose I i in (52) as follows:

Ii(v)=Ji(Tεv)+Err4(v,ε),

with the terms defined as

Ji(Tεv):=1|Y|0TΩ×Γgi(Tεu1ε,Tεu2ε)gi(u11,u21)Tεvdxdσydt,
Err4(v,ε):=0TΓεεgi(u1ε,u2ε)vdσx1|Y|Ω×Γgi(Tεu1ε,Tεu2ε)Tεvdxdσy|Γ||Y|Ωgi(u11,u21)vdx+1|Y|Ω×Γg1(u11,u21)Tεvdxdσydt.

We apply the integration rule (20b) to the first term of Err4 and rewrite the third term using |Γ|=Γdσy. Based on the boundedness (6) of g i, from the Cauchy‐Schwarz inequality, it follows the error estimate

|Err4(v,ε)|=1|Y|0TΩ×Γgi(Tεu1ε,Tεu2ε)(TεvTεv)dxdσydt0TΩ×Γgi(u11,u21)(vTεv)dxdσydtεgi(u1ε,u2ε)L2(0,T;L2(Γε))1|Y|TεvTεvL2(0,T;L2(Ω×Γ))+1|Y|gi(u11,u21)L2(0,T;L2(Ω×Γ))vTεvL2(0,T;L2(Ω×Γ))εK8KgvL2(0,T;L2(Ω))d, (56)

where K8=εT|Γε|Ktr(1+KP)+|Γ||Y|T|Ω|KP. Here, we have used the Poincaré inequality (22), following the trace inequality in periodic domains (26) such that

Ω×Γ(TεvTεv)2dxdσy=j=12Ωjε×Γ(TεvTεvYj)2dxdσyj=12KtrΩjε×Yj(TεvTεvYj)2+|y(Tεv)|2dxdyKtr(1+KP)j=12Ωjε×Yj|y(Tεv)|2dxdyε|Y|Ktr(1+KP)Ω|v|2dx.

Applying Young inequality to J i implies that

|Ji(Tεv)|1|Y|0TΩ×Γ12gi(Tεu1ε,Tεu2ε)gi(u11,u21)2+12Tεv2dxdσydt.

Due to the Lipschitz continuity (7) of g i, using the mean inequality

|Tεuiεui1|22|Tε(uiεui1)|2+2|Tεui1ui1|2,

application of the integration rule (21c) and the trace inequality (25) proceeds further

|Ji(Tεv)|1|Y|0TΩ×Γ2Lg2j=12|Tε(ujεuj1)|2+12Tεv2dxdσydt+Err5(v,ε)=2εLg2j=120TΓε|ujεuj1|2dσxdt+|Γ|2j=120TΩjεTεv2dxdt+Err5(v,ε)2KtrLg2j=12ujεuj1L2(0,T;L2(Ωjε))2+ε2(ujεuj1)L2(0,T;L2(Ωjε))d2+|Γ|2j=121|Yj|2vL2(0,T;L2(Ω))+Err5(v,ε), (57)

because of (see Cioranescu et al43, proposition 2.17)

TεvL2(Ωjε)=|Y||Yj|Tε1vL2(Ω)|Y||Yj|vL2(Ω),

where

Err5(v,ε):=2Lg2|Y|j=120TΩ×ΓTεuj1uj12dxdσydt.

First, we estimate Err5 in (57). Since ui1H1(Ω), according to Griso,29, formula (3.4) the auxiliary estimate for the term in Err5 holds:

Tεuj1uj1L2(Ω×Yj)2ε2Kcuj1L2(Ω)d2,Kc>0.

Therefore, from the trace theorem (24) in Ω×Y j and (21b), we have

1|Y|Tεuj1uj1L2(Ω×Γ)2Ktr|Y|Tεuj1uj1L2(Ω×Yj)2+y(Tεuj1)L2(Ω×Yj)d2ε2Kuuj1L2(Ω)d2,Ku:=KtrKc|Y|+1,

and the term Err5(v,ε) is estimated by

0Err5(v,ε)2ε2Lg2Kuj=12uj1L2(0,T;L2(Ω))d2. (58)

Let η Ω(x) be a smooth cutoff function with a compact support in Ω and equals one outside an ε‐neighborhood of the boundary Ω such that |ηΩ|1 and ε|ηΩ|Cη. For further use, we employ the following functions wiV0Viε expressed equivalently in two ways as

wi:=ũiεui0ε(Tε1Ñi)·ui0ηΩ=ũiεui1+ε(Tε1Ñi)·ui0(1ηΩ), (59)

where ũiεH01(Ω) is the uniform extension of uiεUiε according to Lemma 3.

We will derive the estimates for ũiεui1 with the help of substitution of the test function v=w i from (59) into the expressions for Errk(v,ε), k=0,1,…,5. This implies the following structure of the bounds:

|Errk(wi,ε)|εαkUk, (60)

where the terms are defined by means of

α0:=KAiL(Yi)NiW1,(Yi)d+1,U0:=ui0L2(0,T;H3(Ωiε))wiL2(0,T;H1(Ωiε)),α1:=NiL(Yi)d,U1:=t(ui0)L2(0,T;H1(Ωiε))dwiL2(0,T;H1(Ωiε)),α2:=K6Kg,U2:=wiL2(0,T;H1(Ω)),α3:=K7j=12ÑjL(Y)d,U3:=j=12uj0L2(0,T;L2(Ω))dwjL2(0,T;L2(Ω)),α4:=K8Kg,U4:=wiL2(0,T;L2(Ω))d,α5:=2εLg2Ku,U5:=j=12uj1L2(0,T;L2(Ω))d2,

According to the uniform estimate (9) in Theorem 1 and the continuous extension (27), we have

wiL2(0,T;H1(Ω))23KeuiεL2(0,T;H1(Ωiε))2+3ui0L2(0,T;H1(Ω))2+3εÑiL(Y)dεui0ηΩL2(0,T;H1(Ω))d2=O(1) (61)

following that all α k=O(1) and U k=O(1) for k=0,1,…,5.

The asymptotic equation (51) tested with the function v=w i from (59) leads to

12ddt0TΩiε(uiεui1)2dxdt+0TΩiεAiε(uiεui1)·(uiεui1)dxdt=Ji(Tεwi)+k=04Errk(wi,ε)+Err6(ε)+M(uiεui1) (62)

with the following two terms:

Err6(ε):=0Tt(uiεui1),ε(Tε1Ni)·ui0(1ηΩ)Ωiεdt,M(uiεui1):=0TΩiεAiε(uiεui1)·[ε(Tε1Ni)·ui0(1ηΩ)]dxdt.

We note that M is not an error term; in contrary, it enters with the factor −δ 1 the left‐hand side of the estimate (65) following later.

Err6 is estimated by integration by parts with respect to time

Err6(ε)=0TΩiε(uiεui1)ε(Tε1Ni)·t(ui0)(1ηΩ)dxdtΩiε(uiεui1)ε(Tε1Ni)·ui0(1ηΩ)dxt=0T,

after using Young inequality and the continuous embedding

uiεui1L2(0,T;L2(Ωiε))2Kembuiεui1L(0,T;L2(Ωiε))2, (63)

which implies that

|Err6(ε)|εα6U6,

where

α6:=2+Kemb2NiL(Yi)d,U6:=12+Kembt(ui0)(1ηΩ)L2(0,T;L2(Ωiε))d2+2ui0(1ηΩ)L(0,T;L2(Ωiε))d2+uiεui1L(0,T;L2(Ωiε))2.

The term M(uiεui1) is evaluated by Young inequality with the weight δ 1>0 and using the boundedness property of A i with the upper bound β from (5) as

|M(uiεui1)|=0TΩiεAiε(uiεui1)·{Tε1(yNi)·ui0(1ηΩ)+ε(Tε1Ni)·x(ui0)(1ηΩ)ε(Tε1Ni)·ui0ηΩ}dxdt3βδ123(uiεui1)L2(0,T;L2(Ωiε))d2+Err7(ε),

where

Err7(ε):=3β2δ1yNiL(Yi)d×dui0(1ηΩ)L2(0,T;L2(Ωiε))d2+ε2NiL(Yi)dx(ui0)(1ηΩ)L2(0,T;L2(Ωiε))d×d2+ε2NiL(Yi)dui0·ηΩL2(0,T;L2(Ωiε))2.

It follows

|Err7(ε)|εα7U7,

where

α7:=3β2NiL(Yi)d+yNiL(Yi)d×d,U7:=1δ1ui0(1ηΩ)L2(0,T;L2(Ωiε))d2+εx(ui0)(1ηΩ)L2(0,T;L2(Ωiε))d×d2+εui0·ηΩL2(0,T;L2(Ωiε))2=O(1).

We note that U 7=O(1), in particular, because 1−η Ω≠0 on a O(ε)‐set using the fact that 1−η Ω≠0 on a set of measure O(ε), thus compensating ∇η Ω=O(ε −1) here.

Therefore, using the inequality (57) for J i(⟨T ε w i⟩) and the uniform positive definiteness (33) of A i with the lower bound α>0, from (62), we arrive at the estimate

12Ωiε(uiεui1)2t=0Tdx+α3βδ120TΩiε|(uiεui1)|2dxdt(2KtrLg2+α8)i=12uiεui1L2(0,T;L2(Ωiε))2+2ε2KtrLg2i=12(uiεui1)L2(0,T;L2(Ωiε))d2+k=05|Errk(wi,ε)|+k=68|Errk(ε)|, (64)

where α8:=|Γ|2j=121|Yj|2, and

0Err8(ε):=α8ε(Tε1Ni)·ui0(1ηΩ)L2(0,T;L2(Ωiε))2ε2α8NiL(Yi)dui0L2(0,T;L2(Ωiε))d.

After summation over i=1,2 we rearrange the terms such that

12i=12(uiεui1)(T)L2(Ωiε)2+γi=12(uiεui1)L2(0,T;L2(Ωiε))d2α10i=12uiεui1L2(0,T;L2(Ωiε))2+Err10(ε),Err10(ε):=k=05i=12|Errk(wi,ε)|+2k=69|Errk(ε)|, (65)

where γ:=α4ε2KtrLg23βδ12, α10:=2(KtrLg2+α8), and the error Err9 implies

Err9(ε):=12(uiεui1)(0)L2(Ωiε)2ε2NiL(Yi)dui0(0)L2(Ωiε)d2=O(ε).

After taking the supremum over time, using the embedding theorem (63), we estimate the first term in the left‐hand side of (65) by the lower bound

12i=12(uiεui1)(T)L2(Ωiε)214Kembi=12uiεui1L2(0,T;L2(Ωiε))2+14i=12uiεui1L(0,T;L2(Ωiε))2.

We continue the estimate (65) by taking δ 1 small enough such that γ>0. Therefore, applying Grönwall inequality leads to

i=12(uiεui1)(t)L2(Ωiε)2Err11(ε),Err11(ε):=2Err10(ε)exp(2α10T).

As a consequence, from (65) and the embedding theorem (63), we conclude with the estimate

i=12uiεui1L(0,T;L2(Ωiε))2+i=12(uiεui1)L2(0,T;L2(Ωiε))22Err12(ε),Err12:=2min12,12Kemb,γα10Err11(ε)+Err10(ε)=O(ε), (66)

which finishes the proof.

7. DISCUSSION

Compared with previous results in the literature on multiscale diffusion equations, in the paper, we derived the macroscopic bidomain model that is advantageous for numerical simulation; we first proved the homogenization result supported by residual error estimate of the asymptotic corrector due to the nonlinear transmission condition at the microscopic level, which appears to describe interface chemical reactions.

For further generalization of the obtained result, we suggest to consider the case of connected‐disconnected domains Ω1ε and Ω2ε. While in the connected domain Ω1ε the uniform extension is applicable, the disconnected domain Ω2ε allows a discontinuous Poincaré estimate (see Kovtunenko and Zubkova21).

CONFLICT OF INTEREST

This work does not have any conflicts of interest.

ACKNOWLEDGEMENTS

V.A.K. and A.V.Z. are supported by the Austrian Science Fund (FWF) Project P26147‐N26: “Object identification problems: numerical analysis” (PION). V.A.K. thanks the Russian Foundation for Basic Research (RFBR) joint with JSPS research project 19‐51‐50004 for partial support. S.R. thanks the DFG Collaborative Research Center 910, subproject A5 on pattern formation in systems with multiple scales, for support.

Kovtunenko VA, Reichelt S, Zubkova AV. Corrector estimates in homogenization of a nonlinear transmission problem for diffusion equations in connected domains. Math Meth Appl Sci. 2020;43:1838–1856. 10.1002/mma.6007

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