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. 2020 Dec 15;10:21998. doi: 10.1038/s41598-020-77966-3

Effective field theories for interacting boundaries of 3D topological crystalline insulators through bosonisation

Patricio Salgado-Rebolledo 1,, Giandomenico Palumbo 2, Jiannis K Pachos 1
PMCID: PMC7738686  PMID: 33319789

Abstract

Here, we analyse two Dirac fermion species in two spatial dimensions in the presence of general quartic contact interactions. By employing functional bosonisation techniques, we demonstrate that depending on the couplings of the fermion interactions the system can be effectively described by a rich variety of topologically massive gauge theories. Among these effective theories, we obtain an extended Chern–Simons theory with higher order derivatives as well as two coupled Chern–Simons theories. Our formalism allows for a general description of interacting fermions emerging, for example, at the gapped boundary of three-dimensional topological crystalline insulators.

Subject terms: Topological matter, Topological insulators

Introduction

Time-reversal-invariant topological insulators are among the most well studied topological phases of matter. In three dimensions, they are characterised by suitable topological numbers in the bulk that guarantee the existence of topologically protected massless Dirac fermions on the boundary1,2. Although the topological invariant is a Z2 number, on the slab geometry, it has been shown that robust surface states are given by an odd number of Dirac fermions per boundary3. The situation changes in the case of three-dimensional topological crystalline insulators (TCIs), namely topological insulators characterised by further crystalline symmetries, such as mirror and rotation symmetries411. In particular, for three-dimensional TCIs protected by a single mirror symmetry, one can define the so called mirror Chern number nM on a given two-dimensional plane, which is invariant under the mirror symmetry. These phases host n=|nM| Dirac cones on each boundary5. Recently, mirror-invariant boundary interactions in these systems have been intensively studied by employing several approaches, such as non-linear sigma models12,13, the coupled-wire method for nM=214, Higgs phases for nM=415 and symmetry arguments for nM=816.

Bosonisation represents another important quantum-field-theory approach to study interacting Dirac fermions. It was originally formulated in 1+1 dimensions to map the massive Thirring model to the Sine-Gordon theory17,18 and then extended in higher-dimensional relativistic systems under the name of functional bosonisation19. Although this method has numerous implications that are relevant to condensed matter physics, it has been mainly employed in interacting systems involving a single emergent gauge field.

The goal of this work is to analyse gapped and mirror-broken boundary states in presence of quartic contact interactions between several pieces of fermions. We assume that the interactions are exclusively acting on the boundary, while the bulk of the system is descried by free topological insulating phase. This is similar to the case of 2D time-reversal-invariant topological insulators, where the helical Luttinger liquids appear on the interacting boundary of the system while the 2D bulk states are still related to the free-fermion models20. We introduce then an external magnetic field orthogonal to the surface to induce a Dirac mass that breaks both time-reversal and mirror symmetries and consider generic intra- and inter-species interactions. For simplicity, we fix nM=2, as in14, and employ functional bosonisation. This approach will allow us to map the self-interacting fermion model to free bosonic models. We are interested in obtaining the low energy topological properties of these effective bosonic models for various configuration of inter and intra-species interactions of the original fermionic model.

Our analysis shows that all the resulting effective models contain topological Chern–Simons terms that usually emerge in a variety of T-broken systems such as the quantum Hall states21,22, surface states of three-dimensional topological insulators2 and graphene coupled to external magnetic fields23. However, differently from these previous works, we show the existence of a new exotic phase, characterised by a higher-derivative Chern–Simons term24, when one of the intra-species interaction is switched off. This phase supports a massive U(1) boson and a ghost mode, which is completed decoupled from the bosonic mode, and thus it is a “good ghost”25,26. Moreover, we show the existence of another phase in which the bosonic theory comprises two massive U(1)×U(1) bosons, with a mutual Chern–Simons term, which generalises the well-know Chern–Simons–Maxwell theory to multi-field gauge fields. The topological sector of this phase resembles the effective action studied in Ref.27 in the context of thin-film topological insulators. Importantly, our approach is quite general and can be directly extended to nM>2. This will allow to identify novel topological crystalline phases in presence of very general contact interactions.

Two-fermion interacting system

The starting point of our construction is a (2+1)-dimensional system of two interacting fermion species ψ and χ living on the boundary of 3D topological crystalline insulator with bulk mirror Chern number nM=2. The corresponding effective action is given by

S[χ,ψ]=d3xχ¯iγμμ+mχ+ψ¯iγμμ+mψ+Vχ2χ¯γμχχ¯γμχ+Vχψχ¯γμχψ¯γμψ+Vψ2ψ¯γμψψ¯γμψ, 1

where m=Bzσ3 is the time-reversal broken mass induced by an external magnetic field Bz orthogonal to the surface of the 3D TCI defined on the xy-plane. Here, we use the convention for the Minkowski metric ημν=diag(-,+,+). The gamma matrices are defined in terms of the Pauli matrices as γ0=σ3, γ1=iσ1, γ2=iσ2 and ψ¯=ψγ0, the Dirac conjugate is ψ¯=ψγ0, and the Clifford algebra has the form γμ,γν=-2ημνI2×2. For convenience in the presentation we choose the intra-species coupling constants to be given by Vχ=eχ2 and Vψ=eψ2+ξα2, where eχ, eψ and α are real constants, and ξ=±1, while Vχψ=eχeψ is the inter-species coupling constants.

To analytically determine the behaviour of this interaction system we employ functional bosonisation. This is a powerful approach that will allows us to identify the equivalent bosonic theory describing our model in the low-energy regime. By defining kμ=χ¯γμχ, jμ=ψ¯γμψ, the corresponding generating functional has the form

Z=Dχ¯DχDψ¯Dψexpid3x[χ¯iγμμ+mχ+ψ¯iγμμ+mψ+12eχkμ+eψjμeχkμ+eψjμ+ξα22jμjμ]. 2

In order to integrate out the fermion field χ, we follow19,28 (see also2931) and express the third term in the action as

expi2d3xeχkμ+eψjμeχkμ+eψjμ=Daexpid3x-12aμaμ+aμeχkμ+eψjμ, 3

where aμ is an Hubbard–Stratonovich vector field. By replacing this back into the generating functional Z, we obtain

Z=Dχ¯DχDψ¯DψDaexpid3x[χ¯γμ(iμ+eχaμ)+mχ+ψ¯γμiμ+eψaμ+mψ+ξα22jμjμ-12aμaμ]. 4

We now integrate out χ to obtain an effective bosonic action Γ[a]. In the large mass limit, it can be approximated as3234

Γ[a]=-ilogdetγμ(iμ+eχaμ)+msmeχ28πd3xϵμνρaμνaρ, 5

where sm=m|m|=sign(m) and ϵμνρ is the (2 + 1)-dimensional Levi-Civita symbol with ϵ012=1. Therefore we can write

Z=Dψ¯DψDaexpiSeff[ψ,a], 6

where

Seff[ψ,a]=d3x-12aμaμ+smeχ28πϵμνρaμνaρ+ψ¯γμiμ+eψaμ+mψ+ξα22jμjμ. 7

The action (7) holds for general values of the parameters eχ, eψ, α and ξ. The first two terms are purely given in terms of the vector field aμ. They correspond to the self dual action resulting from a single fermionic species, χ, introduced in35,36. The total action Seff is an extension to that self-dual model having the field aμ coupled to a self-interacting fermionic field ψ. In the following we consider specific configurations of these couplings and extract the behaviour of the model in each case.

Pauli term and higher-derivative Chern–Simons action

In this section we show that for a particular value of the couplings the fermionic system (1) can be described in the low energy limit by a single fermion field non-minimally coupled to an effective U(1) gauge field. In particular, this coupling configuration gives rise to a higher-derivative Chern–Simons theory24. We start our analysis of (7) by considering the interpolating action

SI[ψ,a,A]=d3x[-12aμaμ+ϵμνρaμνAρ-2πsmeχ2ϵμνρAμνAρ+eψaμjμ+ψ¯iγμμ+mψ+ξα22jμjμ], 8

which is given in terms of the Dirac fermion field ψ, the vector field aμ and a new gauge field Aμ. The path integral of SI[ψ,a,A] is equivalent to the functional integral associated to the effective action (7). By integrating out the field Aμ in (8), we obtain

ZI=Dψ¯DψDaDAexpiSI[ψ,a,A]=Dψ¯DψDaexpiSeff[ψ,a], 9

where Seff is given by (7). On the other hand, by integrating out the vector field aμ in the interpolating action (8) we find

ZI=Dψ¯DψDAexpiSeffdual[ψ,A], 10

where the action Seffdual[ψ,A] is given by

Seffdual[ψ,A]=d3x-14FμνFμν-2πsmeχ2ϵμνρAμνAρ+ψ¯iγμμ+mψ+eψψ¯σμνFμνψ+12eψ2+ξα2jμjμ. 11

In this dual effective action Seffdual[ψ,A] the field Fμν=μAν-νAμ is the field strength associated to the gauge potential Aμ and we have also used the standard definition σμν=i4[γμ,γν]=12ϵμνργρ.

The action Seffdual[ψ,A] is dual to Seff[ψ,a], so it faithfully describes the original system (1). The advantage of Seffdual[ψ,A] is that it is given in terms of the gauge field Aμ rather than the vector field aμ and thus it is easier to identify its topological character. From (11) we observe that the effective action (7) can be dualised to a Chern–Simons–Maxwell model coupled to the fermion field ψ by means of the Pauli term. Note that, after using the interpolating action, the coupling of the self interaction for ψ has been shifted back to the original value it had in (1). By directly comparing (1) and (11), we see that we can interpret the Pauli coupling as the low energy description of the mixed interaction term Vχψψ¯γμψχ¯γμχ. The duality between (11) and (7) has been previously established on-shell by eliminating the field aμ or Aμ from the interpolating action (8) by means of their corresponding field equations37,38.

Higher derivative Chern–Simons theory: the eψ2+ξα2=0 case

We now consider the action (7) for the case where α2=eψ20 and ξ=-1, which corresponds to Vψ=0 in (1). In that case, the action (7) does not describe free fermions so that they cannot be integrated out. Moreover for ξ=-1 we cannot employ a similar relation to (3) in order to linearise the interactions. In this case the self interaction in the dual action (11) vanishes and the effective theory takes the form of a fermion non-minimally coupled to the field strength Fμν by means of the Pauli term. Defining the Hodge dual of the curvature Fμ=12ϵμνρFνρ the action takes the form

Seffdual[ψ,A]=d3x12FμFμ-2πsmeχ2ϵμνρAμνAρ+ψ¯γμiμ+eψFμ+mψ. 12

In other words, the Pauli term couples the magnetic moment of the fermions with the magnetic field3941. Note that in 2+1 dimensions the magnetic moment is a scalar leading to the coupling term eψkμFμ seen in (12).

To analyse the properties of (12) we integrate out the fermions ψ. As shown in4244 the Pauli term can be obtained starting from the standard minimal coupling in the Dirac action ψ¯γμAμψ and shifting the gauge field Aμ into the generalised connection AμAμ+eψFμ. We can then integrate out ψ in (12) by using the result (5) for the generalised connection and then set Aμ=0, i.e

Γ[Aμ+eψFμ]|Aμ=0=-ilogdetγμ(iμ+Aμ+eψFμ)+m|Aμ=0smeψ28πd3xϵμνρFμνFρ. 13

By using this result, which is also compatible with Ref.45, the corresponding effective action takes the form

Seffdual[A]=d3x12FμFμ-2πsmeχ2ϵμνρAμνAρ+smeψ28πϵμνρFμνFρ. 14

It is important to remark that, even though the higher-derivative term in the above action looks like a Chern–Simons form, it is not topological as it depends on the space-time metric. Indeed, as shown in24, up to boundary terms one can write

ϵμνρFμνFρ=ϵμνρAμνAρ. 15

Thus, this term leads to a non-vanishing contribution to the energy-momentum tensor, which is a signature of its non-topological nature.

As it has been shown in24, the action (14) includes a ghost mode. Now we will show that this model admits a description in which the ghost is decoupled from the physical degree of freedom. In order to do so, we follow46 and decompose the vector potential in terms of new variables X and Y as follows

A0=1-2X,Ai=1-2εijjY. 16

The effective action (14) then becomes

Seffdual[X,Y]=d3x12YY+smeψ28πXY-2πsmeχ2XY+12X2. 17

We can now integrate out the field X in the corresponding partition function Z=DXDYeSeffdual[X,Y], which yields an effective action for Y given by

Seffdual[Y]=-12eψ28π2d3xY-m+2-m-2Y,m±2=128πeψ221+eψ22eχ2±1+eψ2eχ2. 18

This higher derivative scalar field action can be expressed in terms of two Klein–Gordon fields φ± defined by

φ±=eψ28π-m2Y|m+2-m-2|. 19

The action then takes the form25,26

Seffdual[φ+,φ-]=d3x12φ+-m+2φ+-12φ--m-2φ-. 20

Hence, the field redefinition (19) allows us to express (14) as the action for two decoupled massive Klein–Gordon fields, φ+ and φ-. The field φ+ is a physical Klein–Gordon field, while φ- is a ghost. Since the ghost fields is totally decoupled from the physical degree of freedom, the physical spectrum is not affected by it. In this sense we have a “good” ghost25 emerging in our theory. From (19) we see that m+2>0 for any values of eψ and eχ. On the other hand, m-2 can be positive or negative depending on the values of the couplings eψ and eχ, implying that the ghost φ2 can be also a tachyon. Thus, this theory shares similar features with the Chern–Simons–Maxwell theory47 that describes a single propagating massive bosonic mode. In our case, the effect of the higher-derivative term is to renormalise the topological mass of the boson.

Single and mutual Chern–Simons theories

In this section we show that, besides the Chern–Simons and Maxwell terms, suitable choices of the parameters in the starting action (1) lead to an effective description of the system that includes a mutual Chern–Simons term48.

Single Chern–Simons theory: the α=0 case

The case α=0 corresponds to interaction couplings in (1) that satisfy VχVψ=Vχψ2. In this case we can define the four-spinor Ψ=(ψ,χ)T and the corresponding current Jμ=Ψ¯ΓμΨ, where Γμ=I2×2γμ. The generating functional (2) then boils down to

Z=DΨ¯DΨexpid3xΨ¯iΓμμ+mΨ+12eΨ2JμJμ, 21

where eΨ2=eχ2+eψ2. Since this is a standard Thirring model for Ψ we can linearise the interactions by introducing a vector field aμ19, so that by means of Gaussian integration we implement the replacement eΨ2JμJμ-12aμaμ+eψaμJμ in (21). Using (5) to integrate out Ψ, the low energy behaviour of this system is captured by the following effective action

Seff[ψ,a]=d3x-12aμaμ+smeΨ28πϵμνρaμνaρ. 22

This result can be also obtained from (7) by setting α=0 in and subsequently integrating out ψ. Following35,36, we can dualise this action to a Chern–Simons–Maxwell theory

Seffdual[A]=d3x-14FμνFμν-MAϵμνρAμνAρ. 23

Hence, for the specific case where α=0 the system becomes formally equivalent to a single species self-interacting fermion that gives rise to a Chern–Simons theory with coupling MA=2πsm/(eχ2+eψ2). This theory describes massive bosons that only mediate short-range interactions47.

Mutual Chern–Simons theories: the ξ=1, α0 case

The choice of parameters ξ=1 and α0 corresponds to the action (1) with VψVχ>Vχψ2. In this case the effective action (7) becomes

Seff[ψ,a]=d3x-12aμaμ+smeχ28πϵμνρaμνaρ+ψ¯γμiμ+eψaμ+mψ+α22jμjμ, 24

so one can integrate out ψ directly. Following similar steps as above, we use (3) to linearise the self interaction in the path integral associated to (24) by introducing a new vector field bμ. Subsequently, using (5) with the replacement aμaμ+αeψbμ leads to

Seff[a,b]=d3x-12aμaμ-12bμbμ+sm(eχ2+eψ2)8πϵμνρaμνaρ+smα28πϵμνρbμνbρ+smeψα4πϵμνρaμνbρ. 25

In this action both aμ and bμ are vector fields. In order to turn them into gauge fields we employ the interpolating action procedure. Consider the interpolating path integral (see appendix A in supplementary information)

ZI=DADBDaDbexpid3x-12aμaμ-12bμbμ+ϵμνρaμνAρ+ϵμνρbμνBρ-mA2ϵμνρAμνAρ+mIϵμνρAμνBρ-mB2ϵμνρBμνBρ, 26

where the masses mA, mB and mI are to be fixed in term of the couplings constants in (25). Integrating out the fields Aμ and Bμ leads exactly to the functional integral of the action (25), i.e.

ZI=DaDbexp{iSeff[a,b]}, 27

provided the masses mA, mB and mI are given by

mA=4πsmeχ2,mB=4πsmα21+eψ2eχ2,mI=4πsmαeχ2eψ. 28

The dual theory is obtained by integrating out the vector fields aμ and bμ in (26), which yields

ZI=DADBexpid3x-14FμνFμν-14GμνGμν-mA2ϵμνρAμνAρ+mIϵμνρAμνBρ-mB2ϵμνρBμνBρ, 29

where we have introduced a second field strength, Gμν=μBν-νBμ. Interestingly, for α2=eχ2+eψ2, there appears an emergent Z2 symmetry that exchanges the gauge fields, i.e.

Z2:AμBμ,BμAμ. 30

This theory describes two massive bosons and generalises the Chern–Simons–Maxwell theory47, which is defined for a single U(1) gauge field and the double-Maxwell-BF theory4951. The latter, defined for mA=mB=0, has been employed to study the Meissner effect in two-dimensional superconductors/superfluids that preserve time-reversal symmetry. In this context, the two massive bosons can be interpreted as massive modes related to an effective London penetration length50.

Here, we give a physical interpretation of our model by neglecting the Maxwell terms and focusing on the topological sector

Seffdual[A,B]=-d3xϵμνρmA2AμνAρ-mIAμνBρ+mB2BμνBρ, 31

which is dominant at large distances. By a suitable rescaling of the gauge fields, this topological action formally coincides with that one derived in Ref.27 in thin-film topological insulators. In this context, our T-broken action would describe an emergent quantum anomalous Hall state induced by interactions. In fact, the presence of sm in all the three coefficients mA, mB and mI is the signature of the presence of a common Chern number encoded in those terms that changes sign when the external Zeeman field is flipped. There are however important physical differences with respect to Ref.27. In that work, the Aμ field is identified with an external electromagnetic field and the two fermion species live on different boundaries, such that only in the thin-film limit the effective 2D model for the boundary contain both species.

Finally, note that the effective action in (31) can be further reduced by integrating out the gauge field Bμ, which yields the Chern–Simons action we met in (23) with the same mass MA=2πsm/(eχ2+eψ2). Therefore, at the level of the topological affective action, integrating out Bμ is equivalent to set α=0 in the original action (1). On the other hand, if we choose to integrate the gauge field Aμ, we obtain the Chern–Simons term of (23) for the field Bμ with MB=2πsm/α2. This result corresponds to setting eψ=eχ=0 in (1), which eliminates the interaction between ψ and χ and keeping only the Thirring self-interaction for ψ with coupling α2.

Response to external electromagnetic field

In this subsection we probe the system in Eq. (24) by introducing an external electromagnetic potential Aμ. This requires to modify action (1) by minimally coupling the fermions ψ and χ to Aμ as follows

S[χ,ψ,A]=S[χ,ψ]+qd3x(jμ+kμ)Aμ. 32

Repeating the steps outlined in the previous section leads to the generalization of the effective action (25) to the following one

Seff[a,b,A]=Seff[a,b]+smq4πd3xϵμνρqAμνAρ+(eχ+eψ)Aμνaρ+αAμνbρ. 33

The interpolating path integral (26) is then modified as

ZI=DADBDaDbexpid3x-12aμaμ-12bμbμ+ϵμνρaμνAρ+ϵμνρbμνBρ-2πsmeχ2ϵμνρAμνAρ-2eψαAμνBρ+eχ2+eψ2α2BμνBρ+qeχϵμνρAμνAρ+eχ-eψαAμνBρ, 34

and the dual action (31) is generalized to

Seffdual[A,B,A]=Seffdual[A,B]+qeχϵμνρAμνAρ+qα1-eψeχϵμνρAμνBρ. 35

Integrating out the fields Aμ and Bμ in the corresponding path integral reduces (35) to the following action

S~effdual[A]=q2sm4πd3xϵμνρAμνAρ, 36

which is given only in terms of Aμ. Varying this action with respect to Aμ we obtain the current

Jμ=δS~effdualδAμ=q2sm4πϵμνρFνρ. 37

This clearly shows a topological Hall response of our system in presence of an external electromagnetic field. This current is sensitive to the sign sm of the generated mass m, but it is insensitive to the particular values of the interaction couplings, eχ, eψ and α.

Domain walls and chiral bosons

We now show that our effective topological field theory in Eq. (31) allows us to describe the 1D gapless modes trapped along defect lines (namely, 1D domain walls) that we can add on the 2D gapped boundary. In fact, defect lines behave as an effective spacial boundary for the 2 + 1-D bosonic model in Eq. (31) and the CS/CFT correspondence52 allows us to derive the chiral boson action associated to the 1D modes53. For this action, we can define the following new fields

A±=A±eχ2+eψ2αB. 38

In this way, the effective action takes the form of two decoupled Chern–Simons terms

S~effdual=d3xϵμνρκ+Aμ+νAρ++κ-Aμ-νAρ-, 39

where we have defined

κ±=-πsmeχ21±eψeχ2+eψ2. 40

Following52, we adopt coordinates (txy) and consider the generalized axial gauge

At±-vAx±=0. 41

The Gauss law Fxy=0 leads to locally pure gauge configurations

Ax±=xΦ±,Ay±=yΦ±, 42

which can be implemented directly in the action (39) and leads to

Sedge=dtdxκ+tΦ+xΦ+-vxΦ+2+κ-tΦ-xΦ--vxΦ-2. 43

Therefore, the 1D dynamics is described by two chiral bosons, which are determined by the parameters κ± and velocity v53. Importantly, these chiral modes trapped along the line defects can be eventually measured in experiments.

Conclusions

In this article we have studied the effect interactions have on two Dirac fermions in 2+1 dimensions. As we are interested in the topological properties of this system we employed the bosonisation method in order to obtain the corresponding effective gauge theories. As we vary the fermion couplings with intra-species interactions, Vχ and Vψ, and inter-species interactions Vχψ we obtain a variety of topological theories that correspond to different phases of the model. When one of the fermionic species does not self-interact, Vψ=0, then the system is described by a Chern–Simons theory with a higher-derivative term. With the appropriate field reparametrisation this theory can be written in terms of a physical scalar field and a “good ghost” that completely decouples from the physical spectrum. Hence, it gives a well behaved topological theory, which shares similar features with the Chern–Simons–Maxwell theory and the topological mass is renormalised by the higher-derivative term. Beyond this particular regime, when we take VχVψ>Vχψ2 the action is given in terms of two coupled Chern–Simons theories that describes two propagating massive bosons. In this case the system is described by an emergent quantum anomalous Hall state induced by interactions and the two interacting massive Dirac fermions can be mapped to the two massive bosons. Moreover, for a particular choice of the coupling constants, there appears an emergent Z2 symmetry. In terms of physical observables, we have shown that by coupling the interacting model to an external electromagnetic field, the semiclassical currents are related to a topological Hall response. Moreover, by adding suitable domain walls on the gapped boundary, there appear propagating 1D modes trapped along the domain walls (i.e. defect lines). This is due to the well-known CS/CFT correspondence, where the CFT describes the 1D chiral modes, which can be in principle measured in experiments. Our method does not have a simple interpretation in the case where VχVψ<Vχψ2 so an alternative approach needs to be taken. We leave this case for a future investigation. Finally, note that our approach can be naturally generalised in various ways. One can consider multi-species interactions described by multi-U(1) gauge fields. This paves the way to study the interacting boundaries of 3D topological crystalline insulators for nM>2 through functional bosonisation. Moreover, one can consider multi-SU(N) non-Abelian generalisation of the gauge fields along the lines of Ref.54.

Supplementary information

Acknowledgements

We would like to thank J. Gomis for useful discussions. This work was supported by the ERC through the Starting Grant project TopoCold and the EPSRC Grant EP/R020612/1. Statement of compliance with EPSRC policy framework on research data: This publication is theoretical work that does not require supporting research data. PS-R acknowledges the School of Physics and Astronomy of the University of Leeds for hospitality and support as invited researcher.

Author contributions

J.K.P. designed the research. G.P. implemented the application to crystalline topological insulators. J.K.P. and G.P. wrote the main manuscript. P.S.-R. performed the main calculations. All authors discussed the results and reviewed the manuscript.

Competing interests

The authors declare no competing interests.

Footnotes

Publisher's note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Supplementary information

is available for this paper at 10.1038/s41598-020-77966-3.

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