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. 2021 Feb 8;6(7):5009–5018. doi: 10.1021/acsomega.0c06143

Effect of Sulfur Deposition on the Horizontal Well Inflow Profile in the Heterogeneous Sulfur Gas Reservoir

Mingren Shao , Qi Yang , Bo Zhou , Shuhui Dai §, Ting Li ∥,⊥,*, Faraj Ahmad #
PMCID: PMC7905943  PMID: 33644609

Abstract

graphic file with name ao0c06143_0014.jpg

A semianalytical coupled reservoir/wellbore model based on the volumetric source for horizontal wells of sulfur gas reservoirs is presented, which considers sulfur deposition and permeability heterogeneity. Compared to the results without considering the sulfur deposition effect, the results of this paper model is better fitted to field production data and average relative errors of two simulated results are 8.37% (considering sulfur deposition) and 23.38% (not considering sulfur deposition). Based on the model, we perform sensitivity in terms of various sulfur depositions, producing pressure drop, and permeability contrast. Results show that the production decreases with increased sulfur deposition, and the flow rate along the wellbore in the horizontal well decreases because of sulfur deposition. The production without and with sulfur deposition increases with increased producing pressure drop, while the production without sulfur deposition is higher. Also, higher producing pressure drop causes a higher nonuniform inflow profile along the horizontal well. Sulfur deposition can reduce a nonuniform biased inflow profile along the horizontal well in heterogeneous sulfur gas reservoirs, but the horizontal well production is reduced. Therefore, sulfur deposition is crucial for the production prediction and inflow profile along the horizontal well in heterogeneous sulfur gas reservoirs.

Introduction

Sulfur deposition has attracted increasing attention because it harms production in sulfur gas reservoirs. Sulfur deposition tends to occur when the temperature and pressure of high sulfur gas reservoirs change. The gas reservoir pressure drops, as the gas production increases; hence, sulfur saturation in the sulfur gas decreases.16 Based on sulfur saturation, some mathematical models were built to predict the influence of sulfur deposition on the gas inflow profile of horizontal wells,79 but these models are based on vertical wells. Furthermore, few researchers are concerned about the horizontal well inflow profile in heterogeneous sulfur gas reservoirs.

Over the past few decades, many researchers have focused on horizontal well oil/gas inflow along the horizontal wells,1012 and this problem involves complex reservoir seepage, wellbore flow, and their relationship.1320 Penmatcha and Aziz15 and Ozkan et al.16 developed reservoir/well models by the point source function to predict the flow rate and pressure distribution along the horizontal wellbore, and the point source function was also widely used for transient pressure analysis in other gas reservoirs such as the coalbed methane gas reservoir,1719 but the solution of the point source function has the characteristic of singularity.20 Vicente et al.21 developed a three-dimensional implicit simulator to solve the coupling equation between the reservoir and wellbore. The numerical model can be used to analyze the flow rate and pressure distribution of horizontal wells accurately and deeply, and they need more data and more computation time than analytical solution and semi-analytical solution. Ouyang and Huang22 presented a coupled reservoir/wellbore model using experimental results, but did not consider porous media seepage in the reservoir. Karimifard and Durlofsky23 proposed a new method to consider the interaction between a wellbore model and a reservoir model. However, the boundary conditions in the wellbore model are constants, and this leads to erroneous results in applications.

Souza et al.24 proposed a numerical model to simulate the coupling of the wellbore and reservoir, which takes into account factors such as wellbore length, isotropy and anisotropy, completion scheme, and formation damage near the wellbore area. However, this method needs longer computational time than the analytical method and semianalytical method.2528 The volumetric source method25 was proposed to evaluate the inflow profile for horizontal well completion with inflow control devices, and computational efficiency and high accuracy were obtained. The reservoir/well model of Furui was improved by Adesina et al.,29 who considered the pressure drop caused by acceleration. However, the influence of formation damage near the well area has not been effectively solved. Moreover, less attention was focused on the effects of sulfur deposition on the horizontal well inflow profile in the heterogeneous sulfur gas reservoir.

Sulfur Deposition Damage Model

For sulfur gas reservoir development, the main effects of sulfur deposition are the decrease of the porosity and the decrease of the permeability. It is assumed that the pressure change in time dt is dp and the change in sulfur solubility is dC. During the dt time, the volume of the precipitated solid sulfur in the saturated gas stream is given as follows

graphic file with name ao0c06143_m001.jpg 1

where Vs is the precipitated sulfur volume (m3); q is the flow rate (m3); Bg is the gas volume factor (m3/m3); C is the sulfur solubility in gas (g/m3); p is the reservoir pressure (MPa); t is the production time (d); T is the gas reservoir temperature (K); and ρs is the density of the solid sulfur (2.07 g/cm3).

The deposition amount of the sulfur element in the reservoir can be calculated by eq 1. The deposited solid sulfur clogs the rock pores, and so, the relationship between porosity changes and time can be expressed as30

graphic file with name ao0c06143_m002.jpg 2

where m = ((dC/dp)TμgBg2/k0).where ϕ is the porosity after sulfur deposition, which is dimensionless; ϕ0 is the initial porosity, which is also dimensionless; a is the laboratory coefficient, and its empirical value is −6.842; h is the net thickness (m); r is the sulfur deposition radius (m); μg is the gas viscosity (mPa·s); and k0 is the initial permeability (10–3 μm2).

The relationship between sulfur deposition saturation and porosity is given as

graphic file with name ao0c06143_m003.jpg 3

where Ss is sulfur deposition saturation.

By integrating eq 3, sulfur saturation can be expressed as

graphic file with name ao0c06143_m004.jpg 4

Sulfur deposition affects not only saturation but also the formation permeability. Based on the results reported by Robert,9 the formation permeability and the sulfur deposition saturation can be expressed as

graphic file with name ao0c06143_m005.jpg 5

where k is the permeability after sulfur deposition (10–3 μm2).

Therefore, the permeability after sulfur deposition can be expressed as

graphic file with name ao0c06143_m006.jpg 6

Semianalytical Model and Solution

Assumptions

As we can see in Figure 1, the sulfur gas reservoir is assumed to be a homogeneous reservoir. The gas reservoir (big box) and volumetric source (small box) are shaped as a cuboid box. There are five closed boundaries and one constant pressure boundary on the big box. The surface of the source (small box) is parallel to the gas reservoir. The horizontal well exists in the middle of the big box and fully penetrates the sulfur gas reservoir. It is assumed that the flow in the sulfur gas reservoir is a single steady flow, and the gas flow conforms to Darcy’s law. Sulfur is precipitated in the form of elementary substances during the production process.

Figure 1.

Figure 1

Schematic diagram of the box gas reservoir and horizontal well.

Reservoir Flow Model

As shown in Figure 1, the sulfur gas reservoir model is described by the following parameters: the sizes of the sulfur gas reservoir are xe, ye, and ze. In the heterogeneous sulfur gas reservoir, the gas production intensity of a volume source is q. The sizes of the volumetric source are 2wx, 2wy, and 2wz in three directions, and the center coordinate is (cx, cy, cz). Based on the abovementioned assumption, the diffusion equation of the gas flow in the sulfur gas reservoir can be expressed as

graphic file with name ao0c06143_m007.jpg 7

Boundary conditions

graphic file with name ao0c06143_m008.jpg 8
graphic file with name ao0c06143_m009.jpg 9
graphic file with name ao0c06143_m010.jpg 10
graphic file with name ao0c06143_m011.jpg 11

where

graphic file with name ao0c06143_m012.jpg 12
graphic file with name ao0c06143_m013.jpg 13
graphic file with name ao0c06143_m014.jpg 14
graphic file with name ao0c06143_m015.jpg 15

H(xx0) is the Heaviside function

graphic file with name ao0c06143_m016.jpg 16

where ψi is the original pseudopressure of the gas reservoir, MPa; ψg is the pseudopressure at any point of the sulfur gas reservoir, MPa; qg is the volumetric source strength of the sulfur gas reservoir, m3/d; Vsource is the geometry size of the volumetric source, m3; k0 is the reservoir permeability, μm2; p is the reservoir pressure at any point of the sulfur gas reservoir, MPa; pini is the original gas reservoir pressure, MPa; μg is the gas viscosity, mPa·s; Z is the deviation factor of the sulfur gas reservoir; psc is the pressure under surface standard conditions, MPa; Tsc is the temperature under surface standard conditions, K; and T is the gas reservoir temperature, K.

The solution of the diffusion equation of the gas flow in the sulfur gas reservoir can be written by eq 16. A detailed derivation process of the solution for the diffusion equation based on the volumetric source model in this section can be found in the Appendix.19,20

graphic file with name ao0c06143_m017.jpg 17

In this study, the cylindrical horizontal well is equivalent to a rectangle shape (Figure 1). The rectangle is divided into N parts (Figure 2), and each part is regarded as a volumetric sink, the length of part i is Li, the wellbore radius is rw, and the coordinates of i is (xi, yi, zi). Therefore, the coordinates of part i and dimensions of three directions are as follows

graphic file with name ao0c06143_m018.jpg 18
graphic file with name ao0c06143_m019.jpg 19
graphic file with name ao0c06143_m020.jpg 20

Figure 2.

Figure 2

Schematic of the horizontal well and gas reservoir division.

Corresponding to the division of horizontal wells, the gas reservoir is also divided into N parts, as shown in Figure 2. According to the superposition principle, the pressure drop at any point M(x,y,z) in the sulfur gas reservoir is obtained by the following equation

graphic file with name ao0c06143_m021.jpg 21

It is assumed that there is no cross flow between the two adjacent sulfur reservoir segments and that the point M(x,y,z) is located in the center of part i. According to eq 21, the pressure drop of point M can be expressed as

graphic file with name ao0c06143_m022.jpg 22

Eq 13 is substituted into eq 22 to obtain the pressure of part i

graphic file with name ao0c06143_m023.jpg 23

The sk* approach31 was presented to model reservoir permeability heterogeneity near the wellbore region. s is a constant background permeability and k* is the effective skin along the horizontal well. The skin factor caused by the reservoir heterogeneity by Hawkins’ method32 can be expressed as

graphic file with name ao0c06143_m024.jpg 24

Substituting the eq 24 into the eq 23, the pressure of part i for the sulfur gas reservoir is

graphic file with name ao0c06143_m025.jpg 25

Substituting eq 16 into the eq 25, the eq 25 is converted as

graphic file with name ao0c06143_m026.jpg 26

Wellbore Flow Model

In this study, a single fluid is assumed to flow between two nodes, as shown in Figure 3. As shown in Figure 3, the mass conservation equation can be expressed as:

graphic file with name ao0c06143_m027.jpg 27

Figure 3.

Figure 3

Flow model in the horizontal wellbore.

According to eq 27, the following equation can be obtained as follows:

graphic file with name ao0c06143_m028.jpg 28

The conservation equation can be written as follows:

graphic file with name ao0c06143_m029.jpg 29

Let Inline graphic, and τwi and eq 28 are substituted into eq 29 to obtain the pressure drop

graphic file with name ao0c06143_m031.jpg 30

where the friction coefficient f can be written as33

graphic file with name ao0c06143_m032.jpg 31

The ranges Re ≤ 2300, 2300 < Re < 4000, and Re ≥ 4000 correspond to laminar flow, transition flow, and turbulent flow, respectively.

The properties of the gas (pressure, density, and gas flow rate) by the ideal gas can be expressed as

graphic file with name ao0c06143_m033.jpg 32
graphic file with name ao0c06143_m034.jpg 33

Assuming that the fluid flow near the wellbore is uniform, the gas velocity of part i from the sulfur gas reservoir to the wellbore can be expressed as

graphic file with name ao0c06143_m035.jpg 34

From eqs 2734, the pressure drop of the wellbore can be expressed as

graphic file with name ao0c06143_m036.jpg 35

where Zi is the deviation factor of part i.

It is to be noted that the frictional pressure drop is the first item, and the acceleration pressure drop is the second and third items.

Coupled Model and Solution

As shown in Figure 4, gas reservoir seepage and wellbore flow are coupled to study the influence of the horizontal well inflow profile in the heterogeneous sulfur gas reservoir.

Figure 4.

Figure 4

Coupling diagram of gas reservoir seepage and wellbore flow.

For production control

graphic file with name ao0c06143_m037.jpg 36

For bottom-hole pressure control

graphic file with name ao0c06143_m038.jpg 37

where Qmax is the maximum production, m3/d and pwf,min is the minimum bottom hole pressure, Mpa.

The coupled model is constituted by eqs 2637. Because the model is nonlinear, this model can be solved by the Newton Raphson method. The detailed solution process is shown in Figure 5.

Figure 5.

Figure 5

Calculation flow chart for the model.

Results and Discussion

The effectiveness and application of the reservoir wellbore coupling model proposed in this paper are illustrated by a horizontal well of a sulfur gas reservoir. Basic parameters of the sulfur gas reservoir and horizontal well are shown in Table 1 and Figure 6. The comparison of the results is shown in Figure 7. The results of this paper model compared to the results of the model without considering the effect of sulfur deposition indicate that the new reservoir/wellbore model with sulfur deposition is better fitted to sulfur gas field data, and the average relative errors of the two simulation results are 8.37 and 23.38%, respectively. It shows that sulfur deposition in the sulfur gas reservoir is an important phenomenon that cannot be ignored.

Table 1. Basic Parameters of the Sulfur Gas Reservoir and Horizontal Well.

parameters value
sulfur gas reservoir length [m] 980
sulfur gas reservoir width [m] 600
top depth of the reservoir [m] 6730.3
porosity[fraction] 0.16
initial pressure [MPa] 70
gas density [kg/m3] 0.69
horizontal well length [m] 980
reservoir thickness [m] 60
horizontal well radius [mm] 120
gas viscosity [mPa·s] 0.026
wellbore roughness [m] 0.04

Figure 6.

Figure 6

Permeability along the horizontal well.

Figure 7.

Figure 7

Comparison to field data.

Figures 8 and 9 illustrate production changes with sulfur deposition and the inflow profile of the horizontal well, respectively. For a horizontal well with a producing pressure drop of 3 Mpa, the production decreases with increased sulfur deposition. Also, the flow rate along the horizontal well decreases because the sulfur deposition is higher, which results in a lower flow rate along the horizontal well.

Figure 8.

Figure 8

Production changes with sulfur deposition.

Figure 9.

Figure 9

Influence of sulfur deposition.

Figure 10 illustrates the influence of producing pressure drop. The production both without and with sulfur deposition increases with increased producing pressure drop, while the production without sulfur deposition is higher. Figure 11 illustrates the flow rate without and with sulfur deposition along the horizontal well. The effect of sulfur deposition on the high part of the permeability is greater than that of the low part of the permeability with the increase in the production differential pressure. Also, higher producing pressure drop causes a higher nonuniform inflow profile along the horizontal well.

Figure 10.

Figure 10

Influence of producing pressure drop.

Figure 11.

Figure 11

Inflow profile of the horizontal well in the sulfur gas reservoir.

As shown in Table 2, the permeability of the three groups is set with different permeability contrasts (Jk). Figure 12 illustrates the bigger difference of the permeability contrast in production without and with sulfur deposition and the greater nonuniform inflow profile along the horizontal well in heterogeneous sulfur gas reservoirs. Also, sulfur deposition can reduce the nonuniform biased inflow profile along the horizontal well in heterogeneous sulfur gas reservoirs, but the production of horizontal wells is reduced.

Table 2. Distribution of Horizontal Permeability.

  permeability [10–3 μm2]
distance from the heel [m] Jk = 2.7 Jk = 8.7 Jk = 17.8
6760.3 2.601 3.179 3.05
6834.9 2.601 3.179 9.248
6894.9 2.601 3.179 1.0716
6940.9 3.468 3.757 4.046
6986.9 3.5102 3.6414 5.9245
7032.9 2.8033 3.179 0.8381
7078.9 1.9074 3.8148 1.6785
7124.9 3.757 0.8959 1.8785
7170.9 1.6005 1.6473 3.3235
7216.9 3.3235 3.8726 5.1
7262.9 2.9854 2.89 4.02
7308.9 3.5547 2.89 0.5202
7354.9 3.3524 1.6404 4.4217
7400.9 3.1501 1.1849 3.4391
7446.9 3.4969 4.9997 2.601
7492.9 2.1964 2.5744 1.445
7538.9 3.3501 0.578 2.023
7584.9 3.3056 2.312 0.8381
7630.9 3.2657 2.5432 2.89
7676.9 2.3987 4.3639 1.445
7728.3 1.3762 4.5373 0.6069

Figure 12.

Figure 12

Influence of the permeability contrast.

Conclusions

A new semianalytical model based on the volumetric source method for horizontal wells in sulfur gas reservoirs is developed. The production and the inflow performance of a horizontal well are simulated based on the new model. Compared with the results without considering the effect of sulfur deposition, the calculation results of the new reservoir/wellbore model with sulfur deposition are better fitted to sulfur gas field data, and the average relative errors of the two simulation results are 8.37% and 23.38%, respectively. Based on the model, we determine sensitivity in terms of various sulfur depositions, producing pressure drop, and permeability contrast. The results in detail are stated as follows:

  • (1)

    The production decreases with increased sulfur deposition under a certain pressure. Also, the flow rate along the horizontal well decreases because sulfur deposition is higher, which results in a lower flow rate along the horizontal well.

  • (2)

    The production without and with sulfur deposition increases with increased producing pressure drop, while the production without sulfur deposition is higher. With the increase of producing pressure drop, the effect of sulfur deposition on the high part of the permeability is greater than that of the low part of the permeability. Also, higher producing pressure drop results in a bigger nonuniform inflow profile along the horizontal well.

  • (3)

    The bigger difference of the permeability contrast in production without and with sulfur deposition and the greater nonuniform inflow profile along the horizontal well in heterogeneous sulfur gas reservoirs are illustrated. Also, sulfur deposition can reduce the nonuniform biased inflow profile along the horizontal well in heterogeneous sulfur gas reservoirs, but the production of horizontal wells is reduced.

Acknowledgments

This work was financially supported by the Foundation of State Key Laboratory of Petroleum Resources and Prospecting, China University of Petroleum, Beijing (no. PRP/open-1901).

Appendix19,20

From eqs 69, the characteristic equation can be expressed as

graphic file with name ao0c06143_m039.jpg A.1

Let E = =X(x)Y(y)Z(z), according to separation variables, eq A.1 can be transformed as three one-dimensional eigenvalue problems

graphic file with name ao0c06143_m040.jpg A.2

where

graphic file with name ao0c06143_m041.jpg A.3

Based on eq 16, the characteristics values of three one-dimensional eigenvalue problems are

graphic file with name ao0c06143_m042.jpg A.4
graphic file with name ao0c06143_m043.jpg A.5
graphic file with name ao0c06143_m044.jpg A.6

According to eqs A.4A.6, the characteristic value of three one-dimensional eigenvalue problems is

graphic file with name ao0c06143_m045.jpg A.7

The corresponding characteristic function system of three one-dimensional eigenvalue problems is

graphic file with name ao0c06143_m046.jpg A.8

The 2-norm of eigen function of the characteristic function is

graphic file with name ao0c06143_m047.jpg A.9

where

graphic file with name ao0c06143_m048.jpg A.10

Taking eqA.9 of the characteristic function system as transformation kernel, the model established in this paper is solved through orthogonal transformation. The corresponding orthogonal transformation can be described as follows

graphic file with name ao0c06143_m049.jpg A.11

Based on eqA.9, the inverse transformation of eq 27 is as follows

graphic file with name ao0c06143_m050.jpg A.12

Using orthogonal transformation in eqA.12, eqs 711 can be converted as

graphic file with name ao0c06143_m051.jpg A.13

Substituting eqA.13 into eqA.12, the solution of the model in this paper is

graphic file with name ao0c06143_m052.jpg A.14

where

graphic file with name ao0c06143_m053.jpg A.15
graphic file with name ao0c06143_m054.jpg A.16
graphic file with name ao0c06143_m055.jpg A.17

The authors declare no competing financial interest.

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