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. 2023 Jan 24;10(2):552–553. doi: 10.1021/acsphotonics.2c01805

Correction to “Terahertz Magnon-Polaritons in TmFeO3

Kirill Grishunin, Thomas Huisman, Guanqiao Li, Elena Mishina, Theo Rasing, Alexey V Kimel, Kailing Zhang, Zuanming Jin, Shixun Cao, Wei Ren, Guo-Hong Ma , Rostislav V Mikhaylovskiy
PMCID: PMC9936624  PMID: 36820327

The first error is a misprint in eq 5 from the original paper. The correct formula for the permeability of TmFeO3 is

graphic file with name ph2c01805_m001.jpg 5C

where ω0 is the resonant frequency, Δω is the absorption line width, and Δμ is the effective oscillator strength. The graphic of Inline graphic, which is shown in Figure 3 in the original paper, is not affected by this misprint, as the correct formula was used to plot it.

The second error was discovered in the Terahertz Emission section, and here we decided to provide the full derivation.

The system of the Maxwell equations in the frequency domain (eqs 6 and 7) should be corrected to

graphic file with name ph2c01805_m003.jpg 6C
graphic file with name ph2c01805_m004.jpg 7C

The corresponding wave equation (eq 8 from the original paper) will become the following:

graphic file with name ph2c01805_m005.jpg 8C

In the 1D case it simplifies to

graphic file with name ph2c01805_m006.jpg 9C

where Inline graphic is the wave vector.

The solution of eq 9C has the following form:

graphic file with name ph2c01805_m008.jpg 11C

where Inline graphic is a partial (forced) solution, k0 is the wave vector in air, k1 is the wave vector in the material, and d is the thickness of the sample.

Taking the partial solution in the form Inline graphic, it is found from eq 9C that

graphic file with name ph2c01805_m011.jpg 12C

where Inline graphic is the effective optical penetration decay and Inline graphic is used for the simplification of notation.

By integrating Maxwell’s equations over an infinitesimal length crossing the interfaces and taking the limit as the thicknesses of the transition regions go to zero, one gets the boundary conditions:

graphic file with name ph2c01805_m014.jpg

Using eq 11C, these boundary conditions lead to the following system of equations:

graphic file with name ph2c01805_m015.jpg 13C

Solving these equations for A3, we obtain the solution for the spectrum of the THz radiation emitted from the slab:

graphic file with name ph2c01805_m016.jpg 14C

where Inline graphic. It should be noted that if α = 0 and μ = 1 the formula corresponds to the formula derived in the ref 23 from the original paper.

The eq 14C has the same structure as eq 14 from the original paper, and the error results in swapping coefficients in front of the real and imaginary part.

We plot Figures 6C and 8C using the correct formula. The new calculated data do not differ significantly from original data and exhibit the same features.

Figure 6C.

Figure 6C

(a) Geometry of THz generation in a slab of orthoferrite and the electromagnetic waves relevant to the problem of light−matter interaction; (b) Calculated and measured Fourier amplitudes EFT of the electric field for radiation generated in the TmFeO3 sample slab by a laser pulse at 40 K; (c) The time traces corresponding to the spectra shown in (b).

Figure 8C.

Figure 8C

(a) Calculated transmission beating spectra for the region between the THz pulse and its echo in the time-domain range for different crystal thicknesses; (b) emission spectra for different crystal thicknesses.


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